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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zhou, Guojun, Guo, Shaoqiang, Zhao, Jing, Molokeev M. S., Liu, Quanlin, Zhang, Junying, Xia, Zhiguo
Заглавие : Unraveling the mechanochemical synthesis and luminescence in MnII-based two-dimensional hybrid perovskite (C4H9NH3)2PbCl4
Место публикации : Sci. China Mater. - 2019. - Vol. 62, Is. 7. - P.1013-1022. - ISSN 2095-8226, DOI 10.1007/s40843-018-9404-4. - ISSN 2199-4501(eISSN)
Примечания : Cited References: 40. - The present work was supported by the National Natural Science Foundation of China (91622125, 51722202 and 51572023) and the Natural Science Foundation of Beijing (2172036), and Molokeev M acknowledges the support of the Russian Foundation for Basic Research (17-52-53031). The DFT calculation was carried out at the National Supercomputer Center in Tianjin, and the calculations were performed on TianHe-1(A).
Предметные рубрики: DOPANT ENERGY-TRANSFER
EMISSION
EXCITON
MODEL
Аннотация: The mechanochemical route is a facile and fast way and has received much attention for developing versatile advanced functional materials. Herein, we reported a mechanochemical synthesis for incorporating divalent manganese ions (MnII) into a two-dimensional (2D) hybrid perovskite (C4H9NH3)2PbCl4. The mild external stimuli originating from the grinding at room temperature enabled the formation of MnII-doped 2D hybrid perovskites, and rapidly changed the luminescence characteristics. The photoluminescence analyses show that the violet and orange emissions are attributed to (C4H9NH3)2Pb1–xMnxCl4 band-edge emission and the T1→6A1 transition of Mn2+ resulting from an efficient energy transfer process, respectively. Site preference and distribution of the doped Mn2+ cations on the locations of Pb2+ were analyzed. The formation energy calculated by the density functional theory (DFT) indicates that the Mn2+ ions can rapidly enter the crystal lattice due to the unique 2D crystal structure of the hybrid perovskite. Such a case of mechanochemical synthesis for the 2D hybrid perovskite motivates many novel emerging materials and the related applications.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Su, Binbin, Molokeev M. S., Xia, Zhiguo
Заглавие : Mn2+-Based narrow-band green-emitting Cs3MnBr5 phosphor and the performance optimization by Zn2+ alloying
Место публикации : J. Mater. Chem. C. - 2019. - Vol. 7, Is. 36. - P.11220-11226. - ISSN 2050-7526, DOI 10.1039/c9tc04127c. - ISSN 2050-7534(eISSN)
Примечания : Cited References: 24. - The present work was supported by the National Natural Science Foundations of China (Grant No. 51722202, 51972118 and 51572023), Natural Science Foundations of Beijing (2172036) and the Guangdong Provincial Science & Technology Project (no. 2018A050506004).
Предметные рубрики: THERMAL-STABILITY
BACKLIGHT
EMISSION
Аннотация: To discover new narrow-band green-emitting phosphors is a challenge for backlighting light-emitting diodes (LEDs) used in liquid crystal displays (LCDs). The synthesis and optical properties of Cs3MnBr5 are demonstrated herein. The intrinsic Mn2+ luminescence without concentration quenching leads to intense green emission at 520 nm with narrow full width at half maximum of 42 nm and high photoluminescence quantum yield (PLQY) of 49% under the excitation at 460 nm. When a small amount of Zn2+ is introduced into Cs3MnBr5, the luminescence intensity decreases slightly. However, the thermal stability of Cs3MnBr5 is improved from 82% to 87% with the intensity values at 423 K compared to that at 298 K. The white LED device fabricated using Cs3Mn0.96Zn0.04Br5 (green) and K2SiF6:Mn4+ (red) phosphors with a blue LED chip exhibit a high luminous efficiency (107.76 lm W-1) and wide color gamut (101% National Television System Committee standard (NTSC) in Commission Internationale de L'Eclairage (CIE) 1931 color space), demonstrating its potential application in wide color gamut LCD backlights.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Yang, Xiang, Zhang, Y.u., Zhang, Xuejie, Chen, Jian, Huang, Haisen, Wang, Dongsheng, Chai, Xirong, Xie, Gening, Molokeev M. S., Zhang, Haoran, Liu, Yingliang, Lei, Bingfu
Заглавие : Facile synthesis of the desired red phosphor Li2Ca2Mg2Si2N6:Eu2+ for high CRI white LEDs and plant growth LED device
Место публикации : J. Am. Ceram. Soc. - 2020. - Vol. 103, Is. 3. - P.1773-1781. - ISSN 0002-7820, DOI 10.1111/jace.16858. - ISSN 1551-2916(eISSN)
Примечания : Cited References: 34. - National Natural Science Foundations of China, Grant/Award Number: 21671070 and 51802101; Project GDUPS; Natural Science Foundation of Guangdong Province, Grant/Award Number: 2018A030310217; Guangzhou Science & Technology Project, Grant/Award Number: 201704030086; Guangdong Provincial Special Fund for Modern Agriculture Industry Technology Innovation Teams; National Undergraduate Innovation and Entrepreneurship Training Program granted for Gening Xie, Grant/Award Number: 201910564035
Предметные рубрики: IN-GLASS
LUMINESCENCE
PERFORMANCE
EFFICIENT
EMISSION
ROUTE
Аннотация: The red emission with suitable peak wavelength and narrow band is acutely required for high color rendering index (CRI) white LEDs without at the cost of the luminous efficacy. Herein, the Li2Ca2Mg2Si2N6:Eu2+ red phosphor was prepared with facile solid‐state method using Ca3N2, Mg3N2, Si3N4, Li3N, and Eu2O3 as the safety raw materials under atmospheric pressure for the first time, which shows red emission peaking at 638 nm with full width at half maximum (FWHM) of 62 nm under blue light irradiation and becomes the desired red phosphor to realize the balance between luminous efficacy and high CRI in white LEDs. The morphology, structure, luminescence properties, thermal quenching behavior, and chromaticity stability of the Li2Ca2Mg2Si2N6:Eu2+ phosphor are investigated in detail. Concentration quenching occurs when the Eu2+ content exceeds 1.0 mol%, whereas high‐temperature photoluminescent measurements show a 32% drop from the room‐temperature efficiency at 423 K. In view of the excellent luminescence performances of Li2Ca2Mg2Si2N6:Eu2+ phosphor, a white LEDs with CRI of 91 as a proof‐of‐concept experiment was fabricated by coating the title phosphor with Y3Al5O12:Ce3+ on a blue LED chip. In addition, the potential application of the title phosphor in plant growth LED device was also demonstrated. All the results indicate that Li2Ca2Mg2Si2N6:Eu2+ is a promising red‐emitting phosphor for blue LED‐based high CRI white LEDs and plant growth lighting sources.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Alekseev K. N., Erementchouk M. V., Kusmartsev F. V.
Заглавие : Direct-current generation due to wave mixing in semiconductors
Место публикации : Europhys. Lett. - 1999. - Vol. 47, Is. 5. - P.595-600. - ISSN 0295-5075, DOI 10.1209/epl/i1999-00430-0
Примечания : Cited References: 34
Предметные рубрики: BLOCH OSCILLATOR
SUPERLATTICES
PHOTOCURRENT
TRANSPORT
FREQUENCY
FIELD
RECTIFIERS
EMISSION
CHAOS
GAAS
Аннотация: We describe an effect of the generation of direct current which may arise in semiconductors or semiconductor microstructures due to a mixing of coherent electromagnetic radiations of commensurate frequencies. The effect is, in essence, due to a nonparabolicity of the electron energy bands and is stronger in systems where this nonparabolicity is greater. We have made exact calculations in the framework of the Kane model, applicable to narrow-gap semiconductors and the tight-binding model which we employ for a description of a semiconductor superlattice.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zhang, Ningzi, Molokeev M. S., Liu, Quanlin, Xia, Zhiguo
Заглавие : Pure red upconversion luminescence and optical thermometry of Er3+ doped sensitizer-rich SrYbInO4 phosphors
Место публикации : J. Mater. Chem. C. - 2018. - Vol. 6, Is. 27. - P.7361-7366. - ISSN 2050-7526, DOI 10.1039/c8tc02565g. - ISSN 2050-7534(eISSN)
Примечания : Cited References:34. - The present work was supported by the National Natural Science Foundation of China (Grant 91622125, 51722202 and 51572023) and the Natural Science Foundations of Beijing (2172036), and M. Molokeev acknowledges support of the Russian Foundation for Basic Research (17-52-53031).
Предметные рубрики: TEMPERATURE-SENSING BEHAVIOR
EMISSION
NANOCRYSTALS
LANTHANIDE
Аннотация: Er3+ doped sensitizer-rich SrYbInO4 upconversion phosphors with an orthorhombic structure (Pnma) were synthesized by using a high temperature solid state reaction and their phase structure, site occupation and microstructure have been analyzed. Interestingly, upon the excitation from 980 nm pulsed laser diodes, the SrYbInO4:Er3+ phosphor emitted a nearly pure red emission on account of the 4F9/2 → 4I15/2 transition of Er3+. Additionally, based on the pump power dependence of the upconversion intensity and the schematic diagram of the energy levels, the upconversion mechanism in this system was verified in a two-photon process. The temperature-dependent behaviors of the as-synthesized sample demonstrated the potential for applications in optical thermometry.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Pankin P. S., Vetrov S. Ya., Timofeev I. V.
Заглавие : Tamm plasmon in a structure with the nanocomposite containing spheroidal core-shell particles
Коллективы : Russian Foundation for Basic Research; Government of the Krasnoyarsk Territory; Krasnoyarsk Territorial Foundation [17-42-240464]; Scholarship of the President of the Russian Federation [SP-227.2016.5]
Место публикации : J. Opt.: IOP, 2019. - Vol. 21, Is. 3. - Ст.035103. - ISSN 2040-8978, DOI 10.1088/2040-8986/ab04d8. - ISSN 2040-8986(eISSN)
Примечания : Cited References: 49. - This study was supported by the Russian Foundation for Basic Research, the Government of the Krasnoyarsk Territory, and the Krasnoyarsk Territorial Foundation for Support of Scientific and R&D Activities, project No. 17-42-240464. P S P acknowledges the support of the Scholarship of the President of the Russian Federation No. SP-227.2016.5.
Предметные рубрики: DIMENSIONAL PHOTONIC CRYSTAL
ENHANCEMENT
EMISSION
STATES
Ключевые слова (''Своб.индексиров.''): tamm plasmon--nanocomposite--photonic crystal--core-shell particles
Аннотация: Spectral peculiarities of the structure consisting of a photonic crystal coated with a nanocomposite (NC) have been investigated. The NC used contains spheroidal nanoparticles with a dielectric core and a metallic shell, which are uniformly dispersed in a transparent matrix. The spectral manifestation of the observed Tamm plasmon polariton (TPP) and Fabry-Perot mode has been examined. A significant polarization sensitivity of the spectra upon variation in the nanoparticle shape has been demonstrated. The dispersion curves presented for the TPP and Fabry-Perot mode are shown to be in good agreement with the spectra obtained by the transfer matrix method.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Yun, Xiangyan, Zhou, Jun, Zhu, Yaohui, Molokeev M. S., Jia, Yetong, Wei, Chao, Xu, Denghui, Sun, Jiayue
Заглавие : Thermometry and up-conversion luminescence of Ln3+ (Ln = Er, Ho, Tm)-doped double molybdate LiYbMo2O8
Место публикации : J. Mater. Sci.: Mater. Electron. - 2020. - Vol. 31, Is. 21. - P.18370-18380. - ISSN 0957-4522, DOI 10.1007/s10854-020-04382-8. - ISSN 1573-482X(eISSN)
Примечания : Cited References: 41. - This work is supported by the National Natural Science Foundation of China (No. 21576002 and 61705003) and Beijing Technology and Business University Research Team Construction Project (No. PXM2019_014213_000007)
Предметные рубрики: TEMPERATURE SENSING BEHAVIOR
OPTICAL THERMOMETRY
EMISSION
PHOSPHOR
Аннотация: The discovery of stable and highly sensitive up-conversion (UC) phosphors using the fluorescence intensity ratio (FIR) is a significant challenge in the field of optical temperature sensor. Er3+/Ho3+/Tm3+-doped LiYbMo2O8 UC phosphors with excellent luminescence properties were successfully synthesized through a high-temperature solid-state reaction, and the crystal structure and UC luminescence properties were discussed in detail. The UC process has been investigated by spectra pump power dependence and further explained via the energy level diagram. All emission processes about Er3+ ions and Ho3+ ions are two-photon processes and the blue emission process about Tm3+ ions is a combination of two-photon process and three-photon process. Thermal sensing performances depended on FIR technology were estimated and the sensitivities of LiYb1−xMo2O8:xLn3+ included absolute sensitivity (Sa) and relative sensitivity (Sr) can produce particular change rules with the temperature, which can serve as excellent candidates for applications in optical temperature sensing. With the increase of temperature, the maximum values of Sr of LiYb1−xMo2O8:xLn3+ are 1.16% K−1 (0.05Er3+), 0.25% K−1 (0.01Ho3+), and 0.51% K−1 (0.01Tm3+), respectively. In addition, the Sa value of LiYb0.95Mo2O8:0.05Er3+ phosphor will reach the maximum (1.08% K−1) at 475 K, while the maximum values of Sa of LiYb0.99Mo2O8:0.01Ho3+ and LiYb0.99Mo2O8:0.01Tm3+ are 0.16% K−1, 0.14% K−1.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Deng, Chenkai, Hao, Shiqiang, Liu, Kunjie, Molokeev M. S., Wolverton, Christopher, Fan, Liubing, Zhou, Guojun, Chen, D.a., Zhao, Jing, Liu, Quanlin
Заглавие : Broadband light emitting zero-dimensional antimony and bismuth-based hybrid halides with diverse structures
Коллективы : Beijing Municipal Natural Science FoundationBeijing Natural Science Foundation [2182080]; National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [51972021, 51702329]; Fundamental Research Funds for the Central UniversitiesFundamental Research Funds for the Central Universities [FRF-IDRY-19-005]; RFBRRussian Foundation for Basic Research (RFBR) [19-52-80003]; Department of Energy, Office of Science Basic Energy SciencesUnited States Department of Energy (DOE) [DE-SC0014520]
Место публикации : J. Mater. Chem. C. - 2021. - Vol. 9, Is. 44. - P.15942-15948. - ISSN 2050-7526, DOI 10.1039/d1tc04198c. - ISSN 2050-7534(eISSN)
Примечания : Cited References: 52. - This work was supported by Beijing Municipal Natural Science Foundation (2182080) and the National Natural Science Foundation of China (51972021 and 51702329). The work was partly supported by the Fundamental Research Funds for the Central Universities (FRF-IDRY-19-005) and by the RFBR according to the research project No. 19-52-80003. S. H. and C. W. (DFT calculations) acknowledge support from the Department of Energy, Office of Science Basic Energy Sciences under Grant DE-SC0014520. Access to QUEST, the supercomputing resources facilities at Northwestern University, is also acknowledged
Предметные рубрики: CRYSTAL-STRUCTURE
LONE-PAIR
EMISSION
PEROVSKITES
TIN
LUMINESCENCE
Аннотация: Low-dimensional organic–inorganic metal halides have recently attracted extensive attention because of their various structures and distinguished photoelectric properties. Herein, we report a series of new zero-dimensional organic–inorganic hybrid metal halides: (TMEDA)3Bi2Cl12·H2O, (TMEDA)3Bi2Br12·H2O, (TMEDA)3Sb2Br12·H2O, and (TMEDA)5Sb6Cl28·2H2O [TMEDA = N,N,N′·trimethylethylenediamine]. (TMEDA)3M2X12·H2O (M = Bi or Sb, X = Cl or Br) crystallizes in the monoclinic space group P21/n, and (TMEDA)5Sb6Cl28·2H2O crystallizes in the orthorhombic space group Pnma. (TMEDA)3M2X12 possesses a zero-dimensional structure with the metal halide ions of [MBr6]3− isolated by the organic TMEDA2+ cations. Interestingly, the (TMEDA)5Sb6Cl28·2H2O structure consists of a combination of corner-connected octahedra [Sb4Cl18]6− and edge-shared [Sb2Cl10]4−, which is quite rare. The light emission of all these compounds was measured, and (TMEDA)3Sb2Br12·H2O exhibits the most intense luminescence. Upon 400 nm ultraviolet light excitation, (TMEDA)3Sb2Br12·H2O exhibited strong broadband yellow emission centered at 625 nm with a full-width at half-maximum of ∼150 nm originating from self-trapped excitons. This work suggests the possibility of new types of hybrid halides by introducing different metal centers and probing the structural evolution and photoluminescent properties, serving as a reference for the relationship between structure and luminescent performance and demonstrating their potential use as phosphors in light-emitting diodes.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Liu, Gaochao, Molokeev M. S., Xia, Zhiguo
Заглавие : Structural rigidity control toward Cr3+-based broadband near-infrared luminescence with enhanced thermal stability
Коллективы : International Cooperation Project of the National Key Research and Development Program of China [2021YFE0105700]; National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [51972118, 51961145101]; Guangzhou Science & Technology Project [202007020005]; Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program [2017BT01X137]; RFBRRussian Foundation for Basic Research (RFBR) [19-52-80003]
Место публикации : Chem. Mat. - 2022. - Vol. 34, Is. 3. - P.1376-1384. - ISSN 0897-4756, DOI 10.1021/acs.chemmater.1c04131. - ISSN 1520-5002(eISSN)
Примечания : Cited References: 59. - This work was supported by the International Cooperation Project of the National Key Research and Development Program of China (2021YFE0105700) , National Natural Science Foundation of China (Nos.: 51972118 and 51961145101) , Guangzhou Science & Technology Project (202007020005) , and the Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program (2017BT01X137) . This work was also funded by RFBR according to the research Project No. 19-52-80003
Предметные рубрики: PHOSPHOR
PHOTOLUMINESCENCE
EFFICIENT
EMISSION
CR3+
Аннотация: Broadband near-infrared (NIR) light sources based on phosphor-converted light-emitting diodes (pc-LEDs) are desirable for biochemical analysis and medical diagnosis applications; however, the development of target NIR phosphor is still a challenge. Herein, broadband NIR phosphors, Cr3+-activated CaSc1–xAl1+xSiO6 (λem = 950 nm), are designed and optimized by chemical substitution toward enhanced quantum efficiency and thermal stability. Structural and spectral analyses along with density functional theory calculations reveal that Sc3+/Al3+ substitution contributes to enhancing the structural rigidity and the local symmetry of the [Sc/AlO6] octahedron so that the nonradiative relaxation of Cr3+ emission centers is suppressed significantly. The as-fabricated phosphor-in-glass-based NIR LED light source demonstrates great potential in the detection of alcohol concentration. This study provides a local structure design principle for exploring NIR phosphors with enhanced thermal stability and will also stimulate further studies on material discovery and quantitative analysis of NIR spectroscopy.
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Li, Mingze, Molokeev M. S., Zhao, Jing, Xia, Zhiguo
Заглавие : Optical functional units in zero-dimensional metal halides as a paradigm of tunable photoluminescence and multicomponent chromophores
Место публикации : Adv. Opt. Mater. - 2020. - Vol. 8, Is. 8. - Ст.1902114. - ISSN 2195-1071, DOI 10.1002/adom.201902114
Примечания : Cited References: 38. - This work was supported by the National Natural Science Foundation of China (Nos. 51961145101, 51722202, and 51972118), Fundamental Research Funds for the Central Universities (D2190980), the Guangdong Provincial Science & Technology Project (2018A050506004), and this work was also funded by RFBR according to the Research Project No. 19-52-80003
Предметные рубрики: PEROVSKITES
LUMINESCENCE
ABSORPTION
EMISSION
Аннотация: Zero-dimensional (0D) organic–inorganic hybrid luminescent metal halides have many promising optoelectronic applications; however, the single building unit in the 0D framework restricts their multimode optical control and photoluminescence tuning. Thus, it remains urgent but challenging to rationally design distinct anionic polyhedral with different optical functions and further expand this family by an equivalent cation substitution and halogen replacement. Herein, (C9NH20)9[Pb3X11](MX4)2 (X = Br and Cl, M = Mn, Fe, Co, Ni, Cu, and Zn) is successfully synthesized verifying the rationality of the design philosophy, and the optical characterizations demonstrate the effects of X‐position anions and M‐position cations on luminescence process. Intriguingly, both [Pb3X11]5− and [MX4]2− perform as inorganic building units in this 0D system and optically active centers, in which the former leads to high‐efficiency broad‐band yellow/green emission originating from self‐trapped excitons and the as‐observed multicomponent chromophores are derived from the absorption of the latter in the visible light region. The present work highlights the importance of different optical functional units showing synergistic effects on the physical properties and inspires future studies to explore multifunctional application of 0D luminescent metal halides.
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