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ZOBOV, V. E.
AUTOCORRELATION FUNCTIONS OF THE ANISOTROPIC HEISENBERG PARAMAGNET IN THE APPROXIMATION OF A SELF-CONSISTENT FLUCTUATING FIELD / V. E. ZOBOV // Theor. Math. Phys. - 1990. - Vol. 84, Is. 1. - P. 751-757, DOI 10.1007/BF01017200. - Cited References: 10 . - ISSN 0040-5779

РУБ Physics, Multidisciplinary + Physics, Mathematical
Рубрики:
RELAXATION
Аннотация: The method proposed earlier for investigating the dynamics of the isotropic Heisenberg paramagnet at high temperatures is generalized to the anisotropic case. A system of nonlinear integrodifferential equations relating the three autocorrelation functions of the x, y, and z components of an individual spin is obtained. A solution of the system is sought in the form of series in powers of the time and is investigated on the plane of the complex time variable. The coefficients of the series up to the tenth order for the xy model and the model with truncated dipole interaction are calculated, and the parameters of the singular points nearest the origin are determined from them.

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Доп.точки доступа:
Зобов, Владимир Евгеньевич
}
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Averyanov, E. M.
Splitting of polarized impurity fluorescence bands in the steady-state spectrum of an isotropic solution / E. M. Averyanov // JETP Letters. - 1994. - Vol. 59, Is. 1. - P. 23-26. - Cited References: 12 . - ISSN 0021-3640

РУБ Physics, Multidisciplinary
Рубрики:
RELAXATION
Аннотация: A difference is predicted between the peaks, nu(VV) and nu(VH), Of the polarized components J(VV)(nu) and J(VH)(nu) in the steady-state spectrum of impurity fluorescence in an isotropic solution. This difference would result from a temporal correlation between an orientational Brownian diffusion of excited fluorescing molecules and a structural relaxation of the surrounding matrix molecules.

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Доп.точки доступа:
Аверьянов, Евгений МихайловичAver'yanov
}
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Observation of mixed two-phase state in Eu0.7Pb0.3MnO3 single crystal by magnetic resonance method / N. V. Volkov [et al.] // Physica B. - 2002. - Vol. 324, Is. 1-4. - P. 254-260, DOI 10.1016/S0921-4526(02)01397-2. - Cited References: 19 . - ISSN 0921-4526

РУБ Physics, Condensed Matter
Рубрики:
OPTIMALLY DOPED MANGANITES
   COLOSSAL MAGNETORESISTANCE
   PARAMAGNETIC ANOMALIES
   CURIE-TEMPERATURE
   LA1-XCAXMNO3
   RELAXATION
   SEPARATION
Кл.слова (ненормированные):
manganites -- CMR -- magnetic resonance -- phase separation -- CMR -- Magnetic resonance -- Manganites -- Phase separation -- Europium compounds -- Ferromagnetic materials -- Paramagnetic resonance -- Phase separation -- Phase transitions -- Manganites -- Single crystals
Аннотация: The magnetic resonance measurements show that the mixed two-phase state takes place in the Eu0.7Pb0.3MnO3 single crystal. The coexistence of the magnetic phases is observed in vicinity of the magnetic phase transition, where the sample exhibits the effect of the CMR. The frequency-field dependencies of the spectra allow to conclude that these phases are paramagnetic and ferromagnetic ones. Moreover, the study of the frequency dependencies shows the sensitivity of the mixed-phase state to the external magnetic field. This suggests that the scenario of the phase separation is realized in this case and the mixed two-phase state is not related to simple chemical inhomogeneity. (C) 2002 Elsevier Science B.V. All rights reserved.

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Держатели документа:
RAS, SB, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
ИФ СО РАН
L.V. Kirensky Institute of Physics SB RAS, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Volkov, N. V.; Волков, Никита Валентинович; Petrakovskii, G. A.; Петраковский, Герман Антонович; Vasiliev, V. N.; Velikanov, D. A.; Великанов, Дмитрий Анатольевич; Sablina, K. A.; Саблина, Клара Александровна; Patrin, K. G.; Патрин, Константин Геннадьевич
}
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Two-phase paramagnetic-ferromagnetic state of La0.7Pb0.3MnO3 single-crystal lanthanum manganite / N. V. Volkov [et al.] // Phys. Solid State. - 2002. - Vol. 44, Is. 7. - P. 1350-1354, DOI 10.1134/1.1494635. - Cited References: 17 . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
COLOSSAL MAGNETORESISTANCE
   MAGNETIC-RESONANCE
   DOPED MANGANITES
   LA1-XCAXMNO3
   SEPARATION
   TRANSITION
   RELAXATION
   EPR
Аннотация: Two phases, paramagnetic and ferromagnetic, were shown by the magnetic resonance method to coexist below the temperature T-C in La0.7Pb0.3MnO3 single crystals exhibiting colossal magnetoresistance. The magnetic resonance spectra were studied in the frequency range 10-78 GHz. The specific features in the behavior of the spectral parameters were observed to be the strongest at the temperatures corresponding to the maximum magnetoresistance in the crystals. The concentration ratios of the paramagnetic and ferromagnetic phases in the samples were found to be sensitive to variations in temperature and external magnetic field. This behavior suggests realization of the electronic phase separation mechanism in the system under study. (C) 2002 MAIK "Nauka/Interperiodica".

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Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Siberian Div, Krasnoyarsk 660036, Russia
ИФ СО РАН
Kirensky Institute of Physics, Siberian Division, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Volkov, N. V.; Волков, Никита Валентинович; Petrakovskii, G. A.; Петраковский, Герман Антонович; Vasil'ev, V. N.; Sablina, K. A.; Саблина, Клара Александровна
}
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High-frequency dielectric spectra from liquid crystals of series nCB and nOCB / B. A. Belyaev [et al.] // Tech. Phys. - 2002. - Vol. 47, Is. 4. - P. 470-473, DOI 10.1134/1.1470597. - Cited References: 8 . - ISSN 1063-7842

РУБ Physics, Applied
Рубрики:
DECIMETER WAVELENGTH RANGE
   RELAXATION
   SPECTROSCOPY
   PHASES
Аннотация: The design of a resonant frequency-tunable high-sensitivity microstrip sensor is suggested. The permittivity dispersion of liquid crystals of two homologic series, alkylcyanobiphenyls (7CB and 8CB) and alkyloxycyanobiphenyls (7OCB and 8OCB), is studied at frequencies of 100-900 MHz. The dielectric spectra are shown to be the sum of the Debye relaxation and dielectric resonances observed at f approximate to 160, 280, 360, 450, 550, and 650 MHz. The dielectric resonances are present in the spectra of all the samples in both the nematic and isotropic phase. The substitution of an oxygen atom (series nOCB) for a carbon atom (series nCB) in liquid crystal molecules has a minor effect on the dielectric resonance frequencies but changes the resonance intensities and splits some of the resonance lines. (C) 2002 MAIK "Nauka / Interperiodica".

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Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Siberian Div, Krasnoyarsk 660036, Russia
ИФ СО РАН
Kirenskii Institute of Physics, Siberian Division, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Belyaev, B. A.; Беляев, Борис Афанасьевич; Drokin, N. A.; Дрокин, Николай Александрович; Shabanov, V. F.; Шабанов, Василий Филиппович; Shepov, V. N.; Шепов, Владимир Николаевич
}
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Specific features of the approximation of the dielectric spectra of alkylcyanobiphenyl liquid crystals / B. A. Belyaev [et al.] // Phys. Solid State. - 2003. - Vol. 45, Is. 3. - P. 598-602, DOI 10.1134/1.1562253. - Cited References: 16 . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
DECIMETER WAVELENGTH RANGE
SERIES
RELAXATION
Аннотация: The frequency dependences of the longitudinal and transverse permittivities of oriented nematic liquid crystals belonging to the alkylcyanobiphenyl group nCB (n = 5-8) are measured in the relaxation region in the meter and decimeter wavelength ranges. It is established that the dispersion of the longitudinal permittivity is well approximated by the sum of two Debye processes with different relaxation times. The frequency dependence of the transverse permittivity is represented by the dispersion relation with a continuous distribution of relaxation times in a specified time range. It is demonstrated that, in the high-frequency range (f 200 MHz), in which the dielectric spectra exhibit a number of weakly pronounced dispersion features, the total dispersion of the permittivity is adequately described by the sum of relaxation and resonance processes. (C) 2003 MAIK "Nauka/Interperiodica".

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Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Siberian Div, Krasnoyarsk 660036, Russia
ИФ СО РАН
Kirensky Institute of Physics, Siberian Division, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Belyaev, B. A.; Беляев, Борис Афанасьевич; Drokin, N. A.; Дрокин, Николай Александрович; Shabanov, V. F.; Шабанов, Василий Филиппович; Shepov, V. N.; Шепов, Владимир Николаевич
}
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Zobov, V. E.
The coordinate of the singular point of generating functions of clusters in the high-temperature dynamics of spin lattice systems with axially symmetric interaction / V. E. Zobov, M. A. Popov // Theor. Math. Phys. - 2003. - Vol. 136, Is. 3. - P. 1297-1311, DOI 10.1023/A:1025603416535. - Cited References: 25 . - ISSN 0040-5779

РУБ Physics, Multidisciplinary + Physics, Mathematical
Рубрики:
CONSISTENT FLUCTUATING FIELD
   NUCLEAR-DOUBLE-RESONANCE
   HEISENBERG PARAMAGNET
   LINE SHAPE
   RELAXATION
   SPECTRUM
   APPROXIMATION
   CRYSTALS
   MOMENT
   CAF2
Кл.слова (ненормированные):
spin dynamics -- singular points -- expansion over the reciprocal space dimension -- Expansion over the reciprocal space dimension -- Singular points -- Spin dynamics
Аннотация: We investigate generating functions for equipped trees composed of double bonds of two sorts on a hypercubic lattice of dimension d with built-in fragments. Rules for constructing these clusters are chosen to ensure the estimate for coefficients of power series in time for the longitudinal and transverse autocorrelation functions of the spin system with axially symmetric interaction. We derive a system of two equations for the tree-generating functions and an equation for the generating functions of chains leading from the root to a fragment in a tree using the Bethe approximation and under the condition that mainly bonds of one sort are taken into account. For the face-centered hypercubic lattice, we find the First terms of the 1/d expansion for the coordinate of the singular point of the generating function in both the anisotropic and the isotropic cases taking fragments in the forms of a triangle from four bonds and a four-fold bound pair into account. The obtained result is written in terms of ratios of lattice sums and is generalized to nuclear spin systems with dipole-dipole interaction. The theoretical value of the singular-point coordinate agrees well with the experimental value calculated from the tail of the absorption spectrum of the nuclear magnetic resonance in a barium fluoride monocrystal.

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Держатели документа:
Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Novosibirsk, Russia
Krasnoyarsk State Univ, Krasnoyarsk, Russia
ИФ СО РАН
Kirenskii Institute of Physics, Siberian Branch, RAS, Russian Federation
Krasnoyarsk State University, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Popov, M. A.; Зобов, Владимир Евгеньевич
}
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Unusual disorder effects in superconducting LaFeAs1-delta O0.9F0.1 as revealed by As-75 NMR spectroscopy / F. . Hammerath [et al.] // Phys. Rev. B. - 2010. - Vol. 81, Is. 14. - Ст. 140504, DOI 10.1103/PhysRevB.81.140504. - Cited References: 52. - This work has been supported by the DFG, through FOR 538, SPP 1458 and Contract No. Be1749/12. G. L. acknowledges support from the A. v. Humboldt-Stiftung. M. M. K. acknowledges support from RFBR under Grant No. 09-02-00127, RAS program on "Low temperature quantum phenomena" and President of Russia MK-1683.2010.2. S. L. D. thanks H. Kontani, K. Kuroki, K. Kikoin, and M. Kulic for useful discussions. . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
GAPS
   BA0.6K0.4FE2AS2
   RELAXATION
   SCATTERING
Аннотация: We report As-75 nuclear magnetic resonance measurements of the spin-lattice relaxation in the superconducting (SC) state of LaFeAsO0.9F0.1 and As-deficient LaFeAs1-delta O0.9F0.1. The temperature behavior of 1/T-1 below T-c changes drastically from a T-3 dependence for LaFeAsO0.9F0.1 to a T-5 dependence for the As-deficient sample. These results, together with the previously reported unexpected increase in Tc and the slope of the upper critical field near Tc for the As-deficient sample, are discussed in terms of nonuniversal SC gaps in Fe pnictides and the effect of As deficiency as an exotic case where nonmagnetic "smart" impurities even stabilize an s(+/-)-wave superconductor or within a scenario of a disorder-driven change to s(++) superconductivity.

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Держатели документа:
Inst Solid State Res, D-01171 Dresden, Germany
Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany
Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
Institute for Solid State Research, IFW Dresden, P.O. Box 270116, D-01171 Dresden, Germany
Max-Planck-Institut fur Physik Komplexer Systeme, D-01187 Dresden, Germany
L.V. Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences, 660036 Krasnoyarsk, Russian Federation
Department of Physics, University of Florida, Gainesville, FL 32611, United States

Доп.точки доступа:
Hammerath, F.; Drechsler, S. L.; Grafe, H. J.; Lang, G.; Fuchs, G.; Behr, G.; Eremin, I.; Korshunov, M. M.; Коршунов, Максим Михайлович; Buchner, B.
}
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Quantum nonequilibrium approach for fast electron transport in open systems: Photosynthetic reaction centers / M. . Pudlak [et al.] // Phys. Rev. E. - 2011. - Vol. 84, Is. 5. - Ст. 51912, DOI 10.1103/PhysRevE.84.051912. - Cited References: 34. - This work is partly supported by the Slovak Academy of Sciences in the framework of Center of Excellence NANOFLUID, VEGA Grants No. 2/0069/10, No. FIS2008-00781/FIS (Spain), and RFBR No. 11-02-00086 (Russia). . - ISSN 1539-3755

РУБ Physics, Fluids & Plasmas + Physics, Mathematical
Рубрики:
BACTERIUM RHODOPSEUDOMONAS-VIRIDIS
   PRIMARY CHARGE SEPARATION
   AMINO-ACID-SEQUENCE
   BACTERIOPHEOPHYTIN
   RELAXATION
   SUBUNIT
   DONOR
   MODEL
Кл.слова (ненормированные):
Electron transfer -- External fields -- Fast electron transport -- Initial conditions -- Non equilibrium -- Path-integral -- Perturbation theory -- Photosynthetic reaction center -- Second orders -- Time convolution -- Vibrational modes -- Electron transitions -- Perturbation techniques -- Quantum chemistry -- Photosynthesis
Аннотация: Creation of electrons or excitons by external fields in a system with initially statistically independent unrelaxed vibrational modes leads to an initial condition term. The contribution of this term in the time convolution generalized master-equation approach is studied in the second order of the perturbation theory in path-integral formalism. The developed approach, applied for the analysis of dynamics in the photosynthetic reaction center, exhibits the key role of the initial condition terms at the primary stage of electron transfer.

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Держатели документа:
[Pudlak, M.
Pincak, R.] Slovak Acad Sci, Inst Expt Phys, Kosice 04353, Slovakia
[Pichugin, K. N.] LV Kirenskii Inst Phys, Krasnoyarsk 660036, Russia
[Nazmitdinov, R. G.] Univ Illes Balears, Dept Fis, ES-07122 Palma De Mallorca, Spain
[Nazmitdinov, R. G.] Joint Inst Nucl Res, Bogoliubov Lab Theoret Phys, Dubna 141980, Russia
ИФ СО РАН
Institute of Experimental Physics, Slovak Academy of Sciences, 04353 Kosice, Slovakia
Kirensky Institute of Physics, Akademgorodok 50/38, 660036 Krasnoyarsk, Russian Federation
Departament de Fisica, Universitat de les Illes Balears, ES-07122 Palma de Mallorca, Spain
Bogoliubov Laboratory of Theoretical Physics, Joint Institute for Nuclear Research, 141980 Dubna, Russian Federation

Доп.точки доступа:
Pudlak, M.; Pichugin, K. N.; Пичугин, Константин Николаевич; Nazmitdinov, R. G.; Pincak, R.
}
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10.

Short-range correlations and their thermal hysteresis in the paramagnetic phase of YFe3(BO3)(4) / L. . Rebbouh [et al.] // Phys. Rev. B. - 2011. - Vol. 83, Is. 14. - Ст. 140406, DOI 10.1103/PhysRevB.83.140406. - Cited References: 21. - This work was supported by grants from the Natural Sciences and Engineering Research Council of Canada and the Canada Foundation for Innovation. J.M.C. acknowledges support from the Canada Research Chairs program. . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
MOSSBAUER-SPECTRA
GDFE3(BO3)(4)
RELAXATION
Аннотация: Neutron diffraction and Mossbauer spectroscopy have been used to examine the connections between long-and short-range magnetic order in the rare-earth iron ferroborate YFe3(BO3)(4). We establish the presence of short-range magnetic order in the pseudo-one-dimensional Fe-spin chains of the FeO6 octahedra while the ferroborates are in their (long-range) paramagnetic phase. The short-range order exists at temperatures several times the Neel temperature. In addition, we observe thermal hysteresis of the short-range ordered Fe spins. The observed Fe-spin dynamics are suggestive of the presence of solitons within the domains that form in the Fe-spin chains.

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Держатели документа:
[Rebbouh, L.
Desautels, R. D.
Cadogan, J. M.
van Lierop, J.] Univ Manitoba, Dept Phys & Astron, Winnipeg, MB R3T 2N2, Canada
[Ritter, C.] Inst Laue Langevin, F-38042 Grenoble, France
[Temerov, V.
Pankrats, A.] RAS, LV Kirenskii Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia
ИФ СО РАН
Department of Physics and Astronomy, University of Manitoba, Winnipeg, MB R3T 2N2, Canada
Institut Laue-Langevin, Boite Postale 156, F-38042 Grenoble, France
L. V. Kirenskii Institute of Physics, Siberian Branch of RAS, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Rebbouh, L.; Desautels, R. D.; Ritter, C.; Cadogan, J. M.; Temerov, V.; Pankrats, A. I.; Панкрац, Анатолий Иванович; van Lierop, J.
}
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11.

Theoretical study of the diffusion of lithium in crystalline and amorphous silicon / A. S. Fedorov [et al.] // JETP Letters. - 2012. - Vol. 95, Is. 3. - P. 143-147, DOI 10.1134/S0021364012030058. - Cited References: 28. - We are grateful to the Institute of Computational Modeling, Siberian Branch, Russian Academy of Sciences; the Interdepartmental Supercomputer Center, Russian Academy of Sciences; and the Computer Center, Siberian Federal University, for the use of their computer clusters for performing all calculations. This work was supported by the Ministry of Education and Science of the Russian Federation (federal program "Human Capital for Science and Education in Innovative Russia" for 2009-2013). . - ISSN 0021-3640

РУБ Physics, Multidisciplinary
Рубрики:
ACCELERATED MOLECULAR-DYNAMICS
   AB-INITIO
   INFREQUENT EVENTS
   SIMULATION
   RELAXATION
   HYDROGEN
   POINTS
   SI
Аннотация: The effect of the lattice deformation on potential barriers for the motion of a lithium atom in crystalline silicon has been studied through ab initio density functional calculations. A new universal method of calculating the diffusion coefficient of an admixture in amorphous solid media through the activation mechanism has been proposed on the basis of these data. The method is based on the calculation of the statistical distribution of potential barriers for the motion of an admixture atom between minima depending on the position of neighboring atoms. First, the amorphous structure, which is generated by annealing from the crystalline structure with vacancies, has been simulated. Then, the statistical distribution of the potential barriers in the amorphous structure for various local environments of the admixture atoms has been calculated by means of linear regression with the parameters determined for barriers in crystalline silicon subjected to different deformations. The diffusion coefficient of the admixture has been calculated from this distribution by using the Arrhenius formula. This method has been tested by the example of crystalline and amorphous silicon with admixture of lithium atoms. The method demonstrates that the diffusion of lithium in amorphous silicon is much faster than that in crystalline silicon; this relation is confirmed experimentally.

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Публикация на русском языке Теоретическое исследование диффузии лития в кристаллическом и аморфном кремнии [Текст] / А. С. Федоров [и др.] // Письма в Журн. эксперим. и теор. физ. : Наука, 2012. - Т. 95 Вып. 3-4. - С. 159-163

Держатели документа:
[Fedorov, A. S.
Popov, Z. I.
Ovchinnikov, S. G.] Russian Acad Sci, Kirensky Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia
[Kuzubov, A. A.] Siberian Fed Univ, Krasnoyarsk 660041, Russia

Доп.точки доступа:
Fedorov, A. S.; Федоров, Александр Семенович; Popov, Z. I.; Попов, Захар Иванович; Kuzubov, A. A.; Кузубов, Александр Александрович; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич
}
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12.

    Effects of composition modulation on the luminescence properties of Eu3+ doped Li1-xAgxLu(MoO4)2 solid-solution phosphors / F. Cheng [et al.] // Dalton Trans. - 2015. - Vol. 44, Is. 41. - P. 18078-18089, DOI 10.1039/c5dt02760h. - Cited References: 42. - The present work was supported by the National Natural Science Foundations of China (Grant No. 51272242, 51572023, 51511130035), Natural Science Foundations of Beijing (2132050), the Program for New Century Excellent Talents in University of Ministry of Education of China (NCET-12-0950), Beijing Nova Program (Z131103000413047), Beijing Youth Excellent Talent Program (YETP0635), the Funds of the State Key Laboratory of Rare Earth Resource Utilization, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences (RERU2015022), and the excellent tutor section of the Fundamental Research Funds for the Central Universities of China University of Geosciences, Beijing (2-9-2015-028). This work was also partly supported by the Russian Foundation for Basic Research (Grant No. 15-52-53080 GFEN_a). . - ISSN 1477-9226
   Перевод заглавия: Влияние модуляции состава на люминесцентные свойства твердотельного люминофора Li1-xAgxLu(MoO4)2 допированного Eu3+

РУБ Chemistry, Inorganic & Nuclear
Рубрики:
RED PHOSPHORS
   PHOTOLUMINESCENCE PROPERTIES
   ENERGY-TRANSFER
   WHITE LEDS
   IONS
   NA
   POLYMORPHISM
   TUNGSTATES
   RELAXATION
   MOLYBDATES
Аннотация: Double molybdate scheelite-type solid-solution phosphors Li1−xAgxLu1−y(MoO4)2:yEu3+ were synthesized by the solid state reaction method, and their crystal structures and luminescence properties were investigated in detail. The composition modulation and structural evolution of this series of samples were studied and the selected AgEu(MoO4)2, AgLu(MoO4)2, LiLu(MoO4)2 and LiEu(MoO4)2 phases were analyzed based on the Rietveld refinement. Depending on the variation of the Li/Ag ratio in Li1−xAgxLu1−y(MoO4)2:yEu3+ phosphors, the difference in the luminescence properties of Li1−xAgxLu1−y(MoO4)2:yEu3+ phosphors was ascribed to two factors, one reason could be assigned to the coupling effect and the nonradiative transition between the energy levels of LixAg1−xLu(MoO4)2 matrices and the activator Eu3+, another could be due to the near ultraviolet energy absorption and transmission efficiency between the charge-transfer (CT) band of O2−–Mo6+ and the 4f → 4f emissive transitions of Eu3+. The ultraviolet-visible diffuse reflection spectra (UV-vis DRS) and Raman spectra analysis were also used to verify the above mechanism.

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Держатели документа:
School of Materials Sciences and Technology, China University of Geosciences, Beijing, China
School of Materials Sciences and Engineering, University of Science and Technology Beijing, Beijing, China
Laboratory of Crystal Physics, Kirensky Institute of Physics, SB RAS, Krasnoyarsk, Russian Federation
Department of Physics, Far Eastern State Transport University, Khabarovsk, Russian Federation
Beijing National Laboratory for Molecular Sciences, State Key Laboratory of Rare Earth Materials Chemistry and Applications, College of Chemistry and Molecular Engineering, Peking University, Beijing, China

Доп.точки доступа:
Cheng, F.; Xia, Zhiguo; Molokeev, M. S.; Молокеев, Максим Сергеевич; Jing, X.
}
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13.

Morozov, E. V.
Probing flocculant-induced asphaltene precipitation via NMR imaging: from model toluene-asphaltene systems to natural crude oils / E. V. Morozov, O. N. Martyanov // Appl. Magn. Reson. - 2016. - Vol. 47, Is. 2. - P. 223-235, DOI 10.1007/s00723-015-0741-9. - Cited References:46. - This research was performed with the financial support of Russian Science Foundation (project no. 15-19-00119). . - ISSN 0937-9347. - ISSN 1613-7507

РУБ Physics, Atomic, Molecular & Chemical + Spectroscopy
Рубрики:
PETROLEUM ASPHALTENES
   MOLECULAR-DYNAMICS
   AGGREGATION
   MICROSCOPY
   SCATTERING
   RESONANCE
   SEDIMENTATION
   ASSOCIATION
   CALORIMETRY
   RELAXATION
Аннотация: An nuclear magnetic resonance (NMR) imaging approach for studying flocculant-induced asphaltene precipitation processes is introduced in this report. Unlike commonly accepted techniques, which primarily measure aggregation processes on the submicron scale (the level of asphaltene molecules and their aggregates), NMR imaging demonstrates the capability to obtain new useful information about bulk system behavior on the macro scale. To reveal the capabilities of the method, the model toluene-asphaltene system and two samples of natural crude oils with different chemical composition and physical properties (such as asphaltene content and density) were employed for experiments. The process of colloidal suspension formation and two different patterns of its evolution were observed depending on both the asphaltene content and the flocculant concentration. In the first pattern, the flocculant-induced precipitation leads to the slow uniform compacting of the suspension and descent of the sedimentation front, whereas the second pattern is characterized by sediment accumulation and the upwards drift of the front. It was found that the behavior of the precipitated asphaltenes in the model system correlates well with those observed in natural crude oils. The results achieved in this work are in agreement with the data obtained previously via other techniques. Thus, NMR imaging proved to be an efficient method for probing flocculant-induced precipitation in crude oils.

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Держатели документа:
Russian Acad Sci, Inst Chem & Chem Technol, Siberian Branch, Akademgorodok 50-24, Krasnoyarsk 660036, Russia.
Russian Acad Sci, Kirensky Inst Phys, Siberian Branch, Akademgorodok 50-24, Krasnoyarsk 660036, Russia.
Russian Acad Sci, Siberian Branch, Boreskov Inst Catalysis, Pr Ak Lavrentieva 5, Novosibirsk 630090, Russia.
Novosibirsk State Univ, Pirogova St 2, Novosibirsk 630090, Russia.

Доп.точки доступа:
Martyanov, O. N.; Морозов, Евгений Владимирович; Russian Science Foundation [15-19-00119]
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14.

    Lundin, A. A.
    Asymptotic similarity of time correlation functions and shape of the 13C and 29Si NMR spectra in diamond and silicon / A. A. Lundin, V. E. Zobov // J. Exp. Theor. Phys. - 2018. - Vol. 127, Is. 2. - P. 305-315, DOI 10.1134/S1063776118080216. - Cited References: 47. - We thank V.A. Atsarkin, V.V. Demidov, F.S. Dzheparov, and E. B. Feldman for the discussion of our results. This work was supported by a subsidy allocated by the Institute of Chemical Physics of the Russian Academy of Science for the State assignment, theme 0082-2018-0005, code TSITIS AAAA-A18-118020690203. . - ISSN 1063-7761. - ISSN 1090-6509
Рубрики:
SPIN SYSTEMS
   LINE-SHAPES
   RELAXATION
   SOLIDS
   PARAMAGNETS
   RESONANCE
Аннотация: Based on the proposed theory, we have investigated the shape of the NMR absorption spectra for 13C and 29Si nuclei in diamond and silicon crystals attributable to the internuclear dipole–dipole interaction. In accordance with the available experimental data, we have considered both crystals with a 100% content of magnetoactive isotopes and crystals with a comparatively low dilution by nonmagnetic nuclei. The time correlation functions (the first of which is the Fourier transform of the NMR spectrum) arising in an infinite chain of coupled differential equations are shown to be mutually similar with a slight time delay. The proposed theory allows the spectrum to be calculated analytically. The results obtained agree satisfactorily with the experimental ones. It is noted that the mutual similarity of the time correlation functions is probably a corollary of the development of dynamical chaos in the system.

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Публикация на русском языке Лундин, Андрей Арнольдович. Асимптотическое подобие временных корреляционных функций и форма спектров ЯМР 13C и 29Si в алмазе и кремнии [Текст] / А. А. Лундин, В. Е. Зобов // Журн. эксперим. и теор. физ. - 2018. - Т. 154 Вып. 2. - С. 354–367

Держатели документа:
Russian Acad Sci, Semenov Inst Chem Phys, Vorobevskoe Sh 26, Moscow 117977, Russia.
Russian Acad Sci, Kirensky Inst Phys, Fed Res Ctr, Krasnoyarsk Sci Ctr,Siberian Branch, Akademgorodok 50, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Zobov, V. E.; Зобов, Владимир Евгеньевич; Institute of Chemical Physics of the Russian Academy of Science [0082-2018-0005, TSITIS AAAA-A18-118020690203]
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15.

    Zobov, V. E.
    On the effect of an inhomogeneous magnetic field on high-frequency asymptotic behaviors of correlation functions of spin lattices / V. E. Zobov, M. M. Kucherov // JETP Letters. - 2018. - Vol. 107, Is. 9. - P. 553-557, DOI 10.1134/S002136401809014X. - Cited References: 39 . - ISSN 0021-3640. - ISSN 1090-6487
Рубрики:
HEISENBERG PARAMAGNET
   SYSTEMS
   TIME
   RELAXATION
   DYNAMICS
   SPECTRA
Аннотация: Singular points of spin autocorrelation functions on the imaginary time axis, which determine the arguments of exponential high-frequency asymptotic behaviors, have been analyzed. It has been shown that randomly distributed inhomogeneous magnetic fields expand the wings of spectra of autocorrelation functions and, thereby, intensify the heating of a system subjected to variable magnetic fields, which are used to create effective Hamiltonians or at the saturation of inhomogeneously broadened EPR lines.

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Публикация на русском языке Зобов, Владимир Евгеньевич. О влиянии неоднородного магнитного поля на высокочастотные асимптотики корреляционных функций спиновых решеток [Текст] / В. Е. Зобов, М. М. Кучеров // Письма в Журн. эксперим. и теор. физ. - 2018. - Т. 107 Вып. 9-10. - С. 578-582

Держатели документа:
Russian Acad Sci, Siberian Branch, Fed Res Ctr KSC, Kirensky Inst Phys, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Inst Space & Informat Technol, Krasnoyarsk 660074, Russia.

Доп.точки доступа:
Kucherov, M. M.; Зобов, Владимир Евгеньевич
}
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16.

Mironov, V. L.
Spectroscopic Multirelaxation Dielectric Model of Thawed and Frozen Arctic Soils Considering the Dependence on Temperature and Organic Matter Content / V. L. Mironov, I. V. Savin // Izv. Atmos. Ocean. Phys. - 2019. - Vol. 55, Is. 9. - P. 986-995, DOI 10.1134/S0001433819090305. - Cited References: 16 . - ISSN 0001-4338. - ISSN 1555-628X

РУБ Meteorology & Atmospheric Sciences + Oceanography
Рубрики:
SMOS BRIGHTNESS TEMPERATURES
RELAXATION
BOREAL
Кл.слова (ненормированные):
dielectric model -- moisture -- temperature -- organic soil -- remote sensing -- wet soil
Аннотация: A temperature spectroscopic dielectric model of moist soils developed on the basis of measurements of six samples of thawed and frozen Arctic soils with different contents of organic matter, from 30 to 90%, is presented. This model allows predicting complex permittivity values of moist soil that are in a good agreement with dielectric measurements. It is applicable in a frequency range from 0.05 to 15 GHz, a temperature range from ‒30° to +25°C, and a moisture range from 0.009 to 1.001 g/g. It can be recommended for use in remote sensing algorithms of moisture and temperature of soil using space radiometric and radar data.

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Публикация на русском языке Миронов, Валерий Леонидович. Спектроскопическая многорелаксационная диэлектрическая модель талых и мерзлых арктических почв, учитывающая зависимости от температуры и содержания органического вещества [Текст] / В. Л. Миронов, И. В. Савин // Исслед. Земли из космоса. - 2019. - № 1. - С. 62-73

Держатели документа:
Russian Acad Sci, Kirensky Inst Phys, Siberian Branch, Krasnoyarsk, Russia.

Доп.точки доступа:
Savin, I. V.; Савин, Игорь Викторович; Миронов, Валерий Леонидович
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17.

Markevich, I. A.
Impedance Spectroscopy Study of a Polymer Composite with Carbon Nanotubes in Contact with an Electrolyte / I. A. Markevich, N. A. Drokin, G. E. Selyutin // Tech. Phys. - 2019. - Vol. 64, Is. 9. - P. 1324-1329, DOI 10.1134/S1063784219090093. - Cited References: 14 . - ISSN 1063-7842. - ISSN 1090-6525

РУБ Physics, Applied
Рубрики:
BEHAVIOR
CONDUCTIVITY
RELAXATION
Кл.слова (ненормированные):
impedance spectroscopy -- nanotubes -- electrolyte
Аннотация: The measured frequency dependence of the electric impedance of a composite based on ultra-high molecular weight polyethylene reinforced with carbon nanotubes in contact with an electrolyte is presented. The behavior of the active and reactive impedance components, permittivity, and conductivity in the frequency range from 0.1 Hz to 120 MHz is analyzed. An equivalent electric circuit simulating the dispersion of the impedance of the polymer composite making contact with the electrolyte is proposed. The formation of a double electric layer at the interface between the polymer composite and electrolyte layer is demonstrated and the electrical characteristics of this layer are determined.

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Публикация на русском языке Маркевич И. А. Исследование методом импедансной спектроскопии полимерного композита с углеродными нанотрубками в контакте с электролитом [Текст] / И. А. Маркевич, Н. А. Дрокин, Г. Е. Селютин // Журн. техн. физ. - 2019. - Т. 89 Вып. 9. - С. 1400-1405

Держатели документа:
Russian Acad Sci, Krasnoyarsk Sci Ctr, Inst Chem & Chem Technol, Siberian Branch, Krasnoyarsk 660036, Russia.
Russian Acad Sci, Krasnoyarsk Sci Ctr, Kirensky Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Drokin, N. A.; Дрокин, Николай Александрович; Selyutin, G. E.
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