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Weak ferromagnetism in copper metaborate CuB2O4 / G. A. Petrakovskii [et al.] // Phys. Solid State. - 1999. - Vol. 41, Is. 7. - P. 1157-1161, DOI 10.1134/1.1130957. - Cited References: 10 . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
SUSCEPTIBILITY
Аннотация: CuB2O4 single crystals have been grown and their magnetic and resonance properties have been investigated for the first time. The temperature dependence of the susceptibility was found to contain features at T = 21 and 10 K. The CuB2O4 single crystal transformed at T = 21 K to a weakly ferromagnetic state. The sharp drop in susceptibility at T 10 K is caused by a transition of the magnetic system of CuB2O4 to an antiferromagnetic state. The effective magnetic moment of the Cu2+ ion, determined from the high-temperature part of the magnetic susceptibility, is 1.77 mu(B). The room-temperature g factors are, respectively, 2.170 and 2.133 for magnetic field parallel and perpendicular to the c axis of the crystal. The antiferromagnetic resonance parameters in the weakly ferromagnetic and antiferromagnetic phases were measured. (C) 1999 American Institute of Physics. [S1063-7834(99)02907-X].

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Публикация на русском языке Слабый ферромагнетизм в метаборате меди CuB2O4 [Текст] / Г. А. Петраковский, К. А. Саблина, Д. А. Великанов [и др.] // Физ. тверд. тела. - 1999. - Т. 41 Вып. 7. - С. 1267-1271

Держатели документа:
Russian Acad Sci, LV Kirensky Phys Inst, Siberian Branch, Krasnoyarsk 660036, Russia
ИФ СО РАН
L. V. Kirenskii Institute of Physics, Siberian Branch, Russian Academy of Sciences, 660036 Krasnoyarsk, Russian Federation

Доп.точки доступа:
Petrakovskii, G. A.; Петраковский, Герман Антонович; Sablina, K. A.; Саблина, Клара Александровна; Velikanov, D. A.; Великанов, Дмитрий Анатольевич; Vorotynov, A. M.; Воротынов, Александр Михайлович; Volkov, N. V.; Волков, Никита Валентинович; Bovina, A. F.; Бовина, Ася Федоровна
}
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    Structural and magnetic alteration of Cu2GaBO5 forced by Mn3+ doping / E. Moshkina, E. Eremin, D. Velikanov [et al.] // J. Alloy. Compd. - 2022. - Vol. 902. - Ст. 163822, DOI 10.1016/j.jallcom.2022.163822. - Cited References: 43. - The study was supported by the Russian Science Foundation (Grant No. 21-72-00130) . The specific heat measurements were supported by the subsidy allocated to Kazan Federal University for the state assignment in the sphere of scientific activities (Project No.Journal of Alloys and Compounds 902 (2022) 163822 0671-2020-0 050) . The magnetic measurements, powder X-ray and EDX data were obtained using the analytical equipment of Krasnoyarsk Regional Center of Research Equipment of Federal Research Center "Krasnoyarsk Science Center SB RAS". The X-ray single-crystal experiment was done using the equipment of the Research and Education Centre "Molecular Design and Environmentally Safe Technologies" at NSU. The authors acknowl-edge Prof. Rushana Eremina and Dr. Tatyana Gavrilova for the valu-able discussion of the obtained results . - ISSN 0925-8388. - ISSN 1873-4669
   Перевод заглавия: Структурная и магнитная перестройка Cu2GaBO5, вызванная допированием Mn3+

РУБ Chemistry, Physical + Materials Science, Multidisciplinary + Metallurgy & Metallurgical
Рубрики:
CRYSTAL-STRUCTURE
SUSCEPTIBILITY
Кл.слова (ненормированные):
Ludwigites -- Flux growth -- Magnetic susceptibility -- Spin glass state
Аннотация: To study the gradual change of the structure and the magnetic state of the ludwigite Cu2GaBO5 upon Mn3+ doping, single crystals of Cu2Ga1−xMnxBO5 (x = 0.55, 0.7, 0.8) with the size up to 3 × 3 × 10 mm3 were grown using the flux technique. The phase homogeneity and crystal structure of the obtained compounds were investigated by the powder and single crystal X-ray diffraction. All the samples possessed the monoclinic-distorted ludwigite structure with the P21/c space group. The study of the actual Cu/Ga/Mn composition by the EDX (energy-dispersive X-ray spectroscopy) technique revealed the lower Mn content in all the samples and the refined formulas were Cu2Ga0.47Mn0.53BO5, Cu1.92Ga0.5Mn0.58BO5 and Cu2Ga0.32Mn0.68BO5, respectively. Despite the high manganese content, the concentration transition (from Cu2GaBO5 to Cu2MnBO5) and change of the monoclinic angle did not occur, but strong Me-O octahedra distortions exceeding those both in the parent ludwigites Cu2GaBO5 and Cu2MnBO5 were found. The study of the thermodynamic and magnetic properties revealed the low-temperature magnetic phase transition inherited from the parent Cu2GaBO5 in all the samples. However, the nature and ordering type for the compounds with different Mn content were different: there was a complex transformation of the magnetic state from the partially ordered AFM (antiferromagnetically) in Cu2Ga0.47Mn0.53BO5, through the spin glass state, to the combined spin glass/ordered state in Cu2Ga0.32Mn0.68BO5 with the appearance of magnetic anisotropy. The evident dependence of Tc (phase transition temperature) on the magnetic field was found as well as its decrease at the nonzero magnetic field in the samples with x = 0.53 and 0.68.

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Держатели документа:
Kirensky Inst Phys, Krasnoyarsk 660036, Russia.
Siberian State Univ Sci & Technol, Krasnoyarsk 660037, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Far Eastern State Transport Univ, Dept Phys, Khabarovsk 680021, Russia.
Novosibirsk State Univ, Novosibirsk 630090, Russia.
Inst Geol & Mineral, Novosibirsk 630090, Russia.
Kazan Fed Univ, Inst Phys, Kazan 420008, Russia.
Russian Acad Sci, Fed Res Ctr, Krasnoyarsk Sci Ctr, Siberian Branch, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Moshkina, E. M.; Мошкина, Евгения Михайловна; Eremin, E. V.; Еремин, Евгений Владимирович; Velikanov, D. A.; Великанов, Дмитрий Анатольевич; Bovina, A. F.; Бовина, Ася Федоровна; Molokeev, M. S.; Молокеев, Максим Сергеевич; Seryotkin, Y.; Cherosov, M.; Batulin, R.; Nemtsev, I. V.; Немцев, Иван Васильевич; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Russian Science FoundationRussian Science Foundation (RSF) [21-72-00130]; Kazan Federal University [0671-2020-0 050]
}
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Aplesnin, S. S.
Static and dynamic magnetic properties of coupled spin-1/2 antiferromagnetic chains / S. S. Aplesnin // J. Phys.: Condens. Matter. - 2000. - Vol. 12, Is. 37. - P. 8191-8207, DOI 10.1088/0953-8984/12/37/316. - Cited References: 21 . - ISSN 0953-8984

РУБ Physics, Condensed Matter
Рубрики:
ONE-DIMENSIONAL ANTIFERROMAGNETS
   SYSTEMS
   SUSCEPTIBILITY
   EXCITATIONS
   SR2CUO3
   CA2CUO3
   KCUF3
Кл.слова (ненормированные):
Computational methods -- Copper compounds -- Correlation methods -- Functions -- Magnetic field effects -- Magnetic properties -- Magnetization -- Monte Carlo methods -- Quantum theory -- Specific heat -- Thermal effects -- Excitation spectroscopy -- Interchain coupling -- Intrachain couplings -- Mean-field approximation -- Spin-spin correlation function -- Spinons -- Antiferromagnetic materials
Аннотация: Calculations of the thermodynamic quantities, and the spectra of spinons, triplet excitations, and two-particle spin-singlet (Delta S-z = 0, +/- 1) excitations for a weakly coupled antiferromagnetic S = 1/2 spin chain are made using a mean-field approximation for the interchain couplings (J(2)) by the quantum Monte Carlo method. The mass gaps in these excitation spectra are estimated as functions of the interchain coupling. The critical held H-c, and the temperatures at which the spinon and singlet gaps close (T-1 and T-2, respectively) are obtained. Some peculiarities of the staggered magnetization, the specific heat, and the spin-spin correlation function are found at T-1 = 0.9J(2), T-2 = 1.5J(2), H-c = 3.8J(2), as determined by linear function fitting for J(2)/J(1) < 0.15 The intrachain and interchain couplings, and the staggered magnetization for KCuF3, Sr2CuO3, and Ca2CuO3 are estimated, and mass gaps are predicted to exist in the spectra of the spinons and the singlet two-particle excitations.

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Держатели документа:
Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
ИФ СО РАН
L V Kirensky Institute of Physics, Siberian Br. Russ. Acad. of Sci., Krasnoyarsk, 660036, Russian Federation

Доп.точки доступа:
Аплеснин, Сергей Степанович
}
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    Spin-glass behavior in single crystals of hetero-metallic magnetic warwickites MgFeBO4, Mg0.5Co0.5FeBO4, and CoFeBO4 / A. Arauzo [et al.] // J. Magn. Magn. Mater. - 2015. - Vol. 392. - P. 114-125, DOI 10.1016/j.jmmm.2015.05.006. - Cited References:36. - This work has been financed by the MINECO Project MAT11/23791, MAT2014-53921-R and DGA IMANA project E-34, Russian Foundation for Basic Research (project Nr. 13-02-00958, 13-02-00358 and 14-02-31051-mol-a), Council for Grants of the President of the Russian Federation (project Nr. NSh-2886.2014.2 and SP-938.2015.5). The work of one of coauthors (M.S.P.) was supported by the program of Foundation for Promotion of Small Enterprises in Science and Technology ("UMNIK" program). . - ISSN 0304-8853. - ISSN 1873-4766
   Перевод заглавия: Спин-стекольное поведение в монокристаллах гетерометаллических магнитных варвикитов MgFeBO4, Mg0.5Co0.5FeBO4 и CoFeBO4

РУБ Materials Science, Multidisciplinary + Physics, Condensed Matter
Рубрики:
SYSTEMS
   CHAIN
   Fe
   SUSCEPTIBILITY
   Fe2OBO3
   ENERGY
Кл.слова (ненормированные):
Warwickites -- Spin glass -- Entanglement -- Exchange interaction
Аннотация: Magnetic properties of heterometallic warwickites MgFeBO4, Mg0.5Co0.5FeBO4, and CoFeBO4 are presented, highlighting the effect of Co substitution on the magnetic properties of these compounds. The analysis of magnetization and heat capacity data has shown that these compounds exhibit a spin-glass transition below TSG=10, 20 and 22 K, respectively. Using zero field ac susceptibility as entanglement witness we find that the low dimensional magnetic behavior above TSG show quantum entanglement behavior χ(Τ)∝T−α(Τ) up to TE≈130 K. The α parameters have been deduced as a function of temperature and Co content, indicating the existence of random singlet phase in this temperature region. Above TE the paramagnetism is interpreted in terms of non-entangled spins giving rise to Curie–Weiss paramagnetism. The different intra- and inter-ribbon exchange interaction pathways have been calculated within a simple indirect coupling model. It is determined that the triangular motifs in the warwickite structure, together with the competing interactions, induce frustration. The spin-glass character is explained in terms of the substitutional disorder of the Mg, Fe and Co atoms at the two available crystallographic sites, and the frustration induced by the competing interactions. The Co substitution induces uniaxial anisotropy, increases the absolute magnetization and increases the spin-glass freezing temperature. The entanglement behavior is supported in the intermediate phase irrespective of the introduction of anisotropy by the Co substitution.
Представлены магнитные свойства гетерометаллических варвикитов MgFeBO4, Mg0.5Co0.5FeBO4 и CoFeBO4, с выделением эффекта замещения Co на магнитные свойства этих соединений. Анализ данных намагниченности и теплоемкости показал, что эти соединения обладают спин-стекольным переходом ниже TSG=10, 20 и 22 К соответственно. Используя нулевого поля для переменной восприимчивости, мы находим, что низкоразмерных магнитное поведение выше TSG показать квантовая запутанность поведение χ (Τ) αT? α (Τ) до TEE130 К. Параметры α были выведены в зависимости от температуры и содержание Со, что указывает на существование случайного синглетного фазы в этой области температур. Над TE в Парамагнетизм интерпретируется в терминах перепутывания спинов, приводящих к парамагнетизму Кюри-Вейсса. Различные внутри- и обменного взаимодействия между направлениями были рассчитаны в модели простой косвенной связи. Установлено, что треугольные мотивы в структуре варвикита, вместе с конкурирующими взаимодействиями, вызывают фрустрацию. Характер спинового стекла объясняется в условиях беспорядка замещения атомов Mg, Fe и Co в двух доступных кристаллографических позициях, и фрустрацию, индуцированную конкурирующими взаимодействиями. Замена Со вызывает одноосную анизотропию, увеличивает абсолютную намагниченность и повышает температуру замерзания спинового стекла. Запутанность Поведения поддерживается в промежуточной фазе, независимо от анизотропии из-за введения замещения Со.

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Держатели документа:
Univ Zaragoza, Serv Med Fis, Zaragoza 50009, Spain
LV Kirenskii Inst Phys, Krasnoyarsk 660036, Russia
Siberian Fed Univ, Krasnoyarsk 660074, Russia
RAS, Shubnikov Inst Crystallog, Moscow 119333, Russia
Siberian State Aerosp Univ, Krasnoyarsk 660014, Russia
Univ Zaragoza, CSIC, Inst Ciencia Mat Aragon, Zaragoza 50009, Spain
Dept Fis Mat Condensada, Zaragoza 50009, Spain

Доп.точки доступа:
Arauzo, A.; Kazak, N. V.; Казак, Наталья Валерьевна; Ivanova, N. B.; Иванова, Наталья Борисовна; Platunov, M. S.; Платунов, Михаил Сергеевич; Knyazev, Yu. V.; Князев, Юрий Владимирович; Bayukov, O. A.; Баюков, Олег Артемьевич; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Lyubutin, I. S.; Frolov, K. V.; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Bartolome, J.; MINECO Project [MAT11/23791, MAT2014-53921-R]; DGA IMANA project [E-34]; Russian Foundation for Basic Research [13-02-00958, 13-02-00358, 14-02-31051-mol-a]; Council for Grants of the President of the Russian Federation [NSh-2886.2014.2, SP-938.2015.5]; program of Foundation for Promotion of Small Enterprises in Science and Technology ("UMNIK" program)
}
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    Ignatchenko, V. A.
    Spectral properties of waves in superlattices with 2D and 3D inhomogeneities / V. A. Ignatchenko, D. S. Tsikalov // J. Exp. Theor. Phys. - 2011. - Vol. 113, Is. 2. - P. 232-244, DOI 10.1134/S1063776111080061. - Cited References: 24. - This study was supported in part by the program of the Presidium of the Russian Academy of Sciences (grant no. 27.1), Federal Targeted Program (State contract no. 02.740.11.0220), and Targeted Programs "Development of the Higher School Scientific Potential" in 2009-2010 and 2011 years. . - ISSN 1063-7761
Рубрики:
X-RAY REFLECTION
   PERTURBED FIELDS
   MULTILAYERS
   SUSCEPTIBILITY
   PROPAGATION
   INTERFACES
   SCATTERING
   SYSTEM
Аннотация: We investigate the dynamic susceptibility and one-dimensional density of states in an initially sinusoidal superlattice containing simultaneously 2D phase inhomogeneities simulating correlated rough-nesses of superlattice interfaces and 3D amplitude inhomogeneities of the superlattice layer materials. The analytic expression for the averaged Green's function of the sinusoidal superlattice with two phase inhomogeneities is derived in the Bourret approximation. It is shown that the effect of increasing asymmetry in the peak heights of dynamic susceptibility at the Brillouin zone boundary of the superlattice, which was discovered earlier [15] upon an increase in root-mean-square (rms) fluctuations, also takes place upon an increase in the correlation wavenumber of inhomogeneities. However, the peaks in this case also become closer, and the width and depth of the gap in the density of states decrease thereby. It is shown that the enhancement of rms fluctuations of 3D amplitude inhomogeneities in a superlattice containing 2D phase inhomogeneities suppresses the effect of dynamic susceptibility asymmetry and leads to a slight broadening of the gap in the density of states and a decrease in its depth. Targeted experiments aimed at detecting the effects studied here would facilitate the development of radio-spectroscopic and optical methods for identifying the presence of inhomogeneities of various dimensions in multilayer magnetic and optical structures.

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Держатели документа:
[Ignatchenko, V. A.
Tsikalov, D. S.] Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia

Доп.точки доступа:
Tsikalov, D. S.; Цикалов, Денис Сергеевич; Игнатченко, Вальтер Алексеевич
}
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Shalaev, V. M.
Small-particle composites .2. Nonlinear optical properties / V. M. Shalaev, E. Y. Poliakov, V. A. Markel // Phys. Rev. B. - 1996. - Vol. 53, Is. 5. - P. 2437-2449, DOI 10.1103/PhysRevB.53.2437. - Cited References: 45 . - ISSN 0163-1829

РУБ Physics, Condensed Matter
Рубрики:
FRACTAL CLUSTERS
   RAMAN-SCATTERING
   SUSCEPTIBILITY
   CONDUCTIVITY
   EXCITATIONS
   COLLOIDS
   LIGHT
Аннотация: Strong fluctuations of local fields may result in very large optical nonlinearities in small-particle composites. Enhancement associated with particle clustering is found for a number of optical processes, including four-wave mixing (FWM), third-harmonic generation (THG), Raman scattering, and nonlinear refraction and absorption in Kerr media. Field fluctuations and optical nonlinear susceptibilities are especially large in fractal clusters. The enhancement of optical processes is expressed in terms of the resonant linear absorption by collective dipolar eigenmodes in a cluster, and quality factors, q, of the modes (q much greater than 1). It is shown that the susceptibility of a composite material consisting of random small-particle clusters is proportional to q(3) for Raman scattering and the Kerr optical nonlinearity, and to q(4) and q(6) for THG and FWM, respectively. For all of these processes, a spectral dependence of the effective susceptibility is found. Broad-scale numerical simulations of the optical response in small-particle composites are performed to complement the theory. The simulations are in reasonable agreement with available experimental data.

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Держатели документа:
LV KIRENSKII INST PHYS,KRASNOYARSK 660036,RUSSIA
RUSSIAN ACAD SCI,INST AUTOMAT & ELECTROMETRY,NOVOSIBIRSK 630090,RUSSIA
ИФ СО РАН

Доп.точки доступа:
Poliakov, E. Y.; Markel, V. A.
}
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Size effects in the formation of an uncompensated ferromagnetic moment in NiO nanoparticles / S. I. Popkov [et al.] // J. Appl. Phys. - 2019. - Vol. 126, Is. 10. - Ст. 103904, DOI 10.1063/1.5109054. - Cited References: 54. - This study was supported by the Ministry of Science and Higher Education of the Russian Federation and by the Russian Foundation for Basic Research, Government of the Krasnoyarsk Territory, and Krasnoyarsk Territorial Foundation for Support of Scientific and R&D Activities, project: "Magnetic Reversal of Magnetic Nanoparticles in Strong Pulsed Magnetic Fields-A New Approach to the Study of Dynamic Effects Associated with the Magnetization of Magnetic Nanoparticles," Project No. 18-42-240012. . - ISSN 0021-8979. - ISSN 1089-7550

РУБ Physics, Applied
Рубрики:
MAGNETIC-PROPERTIES
   TEMPERATURE
   SUSCEPTIBILITY
   NANOFERRIHYDRITE
Аннотация: The magnetic properties of samples of NiO nanoparticles with average sizes of 23, 8.5, and 4.5 nm were investigated. Using the magnetization curves measured in strong (up to 250 kOe) pulsed magnetic fields, the contributions of the free spin and ferromagnetic subsystems were extracted. It has been found that the ferromagnetic contribution increases with a decrease in the nanoparticle size and is proportional to the fraction of uncompensated exchange-coupled spins. It is demonstrated that the uncompensated spins form in the antiferromagnetic NiO oxide due to an increase in the fraction of surface atoms in the nanoparticles with decreasing particle size and defects in the bulk of particles.

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Держатели документа:
Russian Acad Sci, Kirensky Inst Phys, Fed Res Ctr, Krasnoyarsk Sci Ctr,Siberian Branch, Krasnoyarsk 660036, Russia.
Russian Acad Sci, Siberian Branch, Boreskov Inst Catalysis, Novosibirsk 630090, Russia.

Доп.точки доступа:
Popkov, S. I.; Попков, Сергей Иванович; Krasikov, A. A.; Красиков, Александр Александрович; Dubrovskiy, A. A.; Дубровский, Андрей Александрович; Volochaev, M. N.; Волочаев, Михаил Николаевич; Kirillov, V. L.; Martyanov, O. N.; Balaev, A. D.; Балаев, Александр Дмитриевич; Ministry of Science and Higher Education of the Russian Federation; Russian Foundation for Basic Research, Government of the Krasnoyarsk Territory [18-42-240012]; Krasnoyarsk Territorial Foundation [18-42-240012]
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Ignatchenko, V. A.
Partial restoration of the wave spectrum of a superlattice due to cross correlations between one- and three-dimensional inhomogeneities / V. A. Ignatchenko, Y. I. Mankov // Phys. Rev. B. - 2007. - Vol. 75, Is. 23. - Ст. 235422, DOI 10.1103/PhysRevB.75.235422. - Cited References: 32 . - ISSN 1098-0121

РУБ Physics, Condensed Matter
Рубрики:
ELASTIC MEDIUM THEORY
   PERIODIC MULTILAYERS
   SPIN-WAVES
   LOCALIZATION
   SYSTEMS
   SUSCEPTIBILITY
   DISORDER
   MEDIA
Аннотация: Effects of cross correlations between one-dimensional (1D) and three-dimensional (3D) random inhomogeneities on the wave spectrum in sinusoidal superlattices are studied theoretically. The situation when the gap in the spectrum (the forbidden zone) at the first Brillouin zone boundary of the superlattice is closed under the action of the 1D inhomogeneities is considered. The phenomenon of the partial opening of this gap is found when the 3D inhomogeneities cross correlated with the 1D inhomogeneities add to the superlattice. The appearance of the logarithmic resonance in the center of the forbidden zone under the action of the cross correlations is shown. The physical nature of the effects in the wave spectrum of the superlattice that are caused by the cross correlations and the relation of these effects with the asymptotic properties of the correlation function of inhomogeneities are discussed.

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Держатели документа:
SB RAS, LV Kirensky Inst Phys, Krasnoyarsk 660036, Russia
ИФ СО РАН
L. V. Kirensky Institute of Physics, SB RAS, 660036 Krasnoyarsk, Russian Federation

Доп.точки доступа:
Mankov, Y. I.; Игнатченко, Вальтер Алексеевич
}
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10.

Averyanov, E. M.
Orientation ordering and critical behavior of discoid nematics / E. M. Averyanov // Zhurnal Eksperimentalnoi Teor. Fiz. - 1996. - Vol. 110, Is. 5. - P. 1820-1840. - Cited References: 55 . - ISSN 0044-4510