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Anisotropic thermal expansion and electronic transitions in the Co3BO5 ludwigite / N. Kazak, A. Arauzo, J. Bartolome [et al.] // Dalton Trans. - 2022. - Vol. 51, Is. 16. - P6345-6357, DOI 10.1039/d2dt00270a. - Cited References: 57. - We are grateful to the Russian Foundation for Basic Research (project no. 20-02-00559 and 21-52-12033) for supporting this paper. This work was performed within the framework of the budget project no. 0287-2021-0013 for the Institute of Chemistry and Chemical Technology SB RAS. We acknowledge the financial support from the Spanish Ministry of Economy, Industry and Competitiviness (MINECO), (Grant No. MAT2017-83468-R) and from the regional Government of Aragón (E12-20R RASMIA project) . - ISSN 1477-9226
Кл.слова (ненормированные):
Activation energy -- Anisotropy -- Cobalt compounds -- Crystal structure -- Electric conductivity -- Electronic properties -- Magnetic moments -- Magnetic susceptibility -- Negative thermal expansion
Аннотация: The investigations of the crystal structure, magnetic and electronic properties of Co3BO5 at high temperatures were carried out using powder X-ray diffraction, magnetic susceptibility, electrical resistivity, and thermopower measurements. The orthorhombic symmetry (Sp.gr. Pbam) was observed at 300 K and no evidence of structural phase transitions was found up to 1000 K. The compound shows a strong anisotropy of the thermal expansion. A large negative thermal expansion along the a-axis is observed over a wide temperature range (T = 300–600 K) with αa = −35 M K−1 at T = 500 K with simultaneous expansion along the b- and c-axes with αb = 70 M K−1 and αc = 110 M K−1, respectively. The mechanisms of thermal expansion are explored by structural analysis. The activation energy of the conductivity decreases significantly above 700 K. Electronic transport was found to be a dominant conduction mechanism in the entire temperature range. The correlations between the thermal expansion, electrical resistivity, and effective magnetic moment were revealed and attributed to the evolution of the spin state of Co3+ ions towards the spin crossover and gradual charge-ordering transition.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Instituto de Nanociencia y Materiales de Aragon (INMA), CSIC-Universidad de Zaragoza and Departamento de Fisica de la Materia Condensada, Zaragoza, 50009, Spain
Servicio de Medidas Fisicas, Universidad de Zaragoza, Zaragoza, 50009, Spain
Research and Development Department, Kemerovo State University, Kemerovo, 650000, Russian Federation
Institute of Chemistry and Chemical Technology, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation

Доп.точки доступа:
Kazak, N. V.; Казак, Наталья Валерьевна; Arauzo, A.; Bartolome, J.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Solovyov, L.; Borus, A.; Борус, Андрей Андреевич; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич
}
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Anisotropic thermal expansion in Co3BO5 ludwigite / Yu. S. Gokhfeld, N. V. Kazak, M. S. Molokeev [et al.] // VIII Euro-Asian symposium "Trends in magnetism" (EASTMAG-2022) : Book of abstracts / program com. S. G. Ovchinnikov [et al.]. - 2022. - Vol. 2, Sect. H : Magnetism of strongly correlated electron systems. - Ст. H.P6. - P. 87-88. - Cited References: 3. - Support by RFBR 20-02-00559 and 21-52-12033 ННИО_а is acknowledged . - ISBN 978-5-94469-051-7

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russia
Institute of Chemistry and Chemical Technology, Federal Research Center KSC SB RAS

Доп.точки доступа:
Gokhfeld, Yu. S.; Гохфельд, Ю.С.; Kazak, N. V.; Казак, Наталья Валерьевна; Molokeev, M. S.; Молокеев, Максим Сергеевич; Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Solovyov, L. A.; Соловьев, Леонид Александрович; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Российская академия наук; Физико-технический институт им. Е.К. Завойского ФИЦ Казанского научного центра РАН; Казанский (Приволжский) федеральный университет; Euro-Asian Symposium "Trends in MAGnetism"(8 ; 2022 ; Aug. ; 22-26 ; Kazan); "Trends in MAGnetism", Euro-Asian Symposium(8 ; 2022 ; Aug. ; 22-26 ; Kazan)
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Anomalies of the electronic structure and physical properties of rare-earth cobaltites near spin crossover / V. A. Dudnikov [et al.] // JETP Letters. - 2016. - Vol. 104, Is. 8. - P. 588-600, DOI 10.1134/S002136401620011X. - Cited References: 101. - We are grateful to our colleagues A. Anshits, N. Perov, L. Solov’ev, S. Vereshchagin, S. Gavrilkin, V. Voronov, K. Shaikhutdinov, A. Rogalev, and M.V. Gorev for the fruitful collaboration in the studies of cobaltites for many years. This work was supported by the Council of the President of the Russian Federation for Support of Young Scientists and Leading Scientific Schools (project nos. NSh-7559.2016.2, SP-1844.2016.1, and SP-938.2015.5), by the Foundation for Support of Innovations (program UMNIK), by the Russian Foundation for Basic Research (project nos. 16-02-00507, 16-02-00098, 16-32-60049-mol-a-dk, and 16-32-00206_mol-a), and jointly by the Russian Foundation for Basic Research and the Krasnoyarsk Territorial Science Foundation (project nos. 16-42-240413, 16-43-240505, and 16-42-240470). . - ISSN 0021-3640
Аннотация: The features of the characteristics of LnCoO3 cobaltites, where Ln is a rare-earth element, are discussed. Both experiment and theory demonstrate that their essentials are related to the low-spin ground state of cobalt ions. The thermally induced occupation of the excited high-spin state gives rise to peaks in the magnetic susceptibility, specific heat, and thermal expansion, as well as to a smooth insulator–metal transition. The analysis is based both on the data from the current literature concerning LaCoO3 and in many aspects on our own studies of GdCoO3 and La1?xGdxCoO3 solid solutions. © 2016, Pleiades Publishing, Inc.

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Публикация на русском языке Аномалии электронной структуры и физических свойств редкоземельных кобальтитов в окрестности спинового кроссовера [Текст] / В. А. Дудников [и др.] // Письма в Журн. эксперим. и теор. физ. : Наука, 2016. - Т. 104 Вып. 7-8. - С. 604-616

Держатели документа:
Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences, Krasnoyarsk, Russian Federation
Siberian Federal University, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Orlov, Yu. S.; Орлов, Юрий Сергеевич; Kazak, N. V.; Казак, Наталья Валерьевна; Platunov, M. S.; Платунов, Михаил Сергеевич; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич
}
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Anomalous structural, magnetic, optical and electronic properties of GdCoO3-y / S. G. Ovchinnikov [et al.] // 20th Int. Сonf. on Magnetism (ICM-2015) : book of abstracts. - 2015. - Ст. TH.C

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Доп.точки доступа:
Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Orlov, Yu. S.; Орлов, Юрий Сергеевич; Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Kazak, N. V.; Казак, Наталья Валерьевна; Shaikhutdinov, K. A.; Шайхутдинов, Кирилл Александрович; International Conference on Magnetism(20 ; 2015 ; Jul ; 5-10 ; Barselona, Spain)
}
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Antiferromagnetic ordering in REM cobaltite GdCoO3 / V. A. Dudnikov [и др.] // Phys. Solid State. - 2012. - Vol. 54, Is. 1. - P. 79-83, DOI 10.1134/S106378341201009X. - Cited References: 16. - This study was supported by the program of the Branch of Physical Sciences of the Russian Academy of Sciences "Strong Electron Correlations," the Russian Foundation for Basic Research (project no. 09-02-00171-a), and Federal Agency for Science and Innovations (grant no. MK-5632.2010.2). . - ISSN 1063-7834

РУБ Physics, Condensed Matter
Рубрики:
SPIN-STATE
   RCo3O3 R
   Sm
   Eu
   Nd
Аннотация: Temperature and magnetic-field dependences of the static magnetization of polycrystalline cobaltite GdCoO3 have been measured. The magnetic properties of the GdCoO3 sample have been studied in the paramagnetic and antiferromagnetic states. The magnetic phase diagram has been constructed. The exchange field between the Gd-Gd sublattices and the anisotropy field have been estimated.

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Публикация на русском языке Антиферромагнитное упорядочение в РЗМ-кобальтите GdCoO[3] [Текст] / В. А. Дудников [и др.] // Физ. тверд. тела. - 2012. - Т. 54 Вып. 1. - С. 72-78

Доп.точки доступа:
Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Velikanov, D. A.; Великанов, Дмитрий Анатольевич; Kazak, N. V.; Казак, Наталья Валерьевна; Michel, C. R.; Bartolome, J.; Arauzo, A.; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Patrin, G. S.; Патрин, Геннадий Семёнович
}
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Concentration dependence of the spin gap in solid solutions La1−xGdxCoO3−δ / S. G. Ovchinnikov [et al.] // J. Magn. Magn. Mater. - 2015. - Vol. 383. - P. 162-165, DOI 10.1016/j.jmmm.2014.11.083. - Cited References:20. - This work is supported by Siberian Branch of Russian Academy of Sciences (Projects no. 38), RFBR Grants nos. 13-02-00358, 13-02-00958, 13-02-01395, 14-02-31051, and 14-02-00186, and President of Russia Grant no. NSh-2886.2014.2. . - ISSN 0304

РУБ Materials Science, Multidisciplinary + Physics, Condensed Matter
Рубрики:
STATE TRANSITION
   TEMPERATURE
   LACOO3
   GDCOO3
   COBALTITES
Кл.слова (ненормированные):
Strong correlated electron systems -- Spin crossover systems -- Magnetic -- properties -- Solid solutions
Аннотация: The temperature dependence of the static magnetization of polycrystalline rare-earth cobaltites La1−xGdxCoO3−δ (x=0.2, 0.5, 1) was measured in a wide temperature range up to 900 K. The contribution from Co3+ ions at high temperatures to the magnetic susceptibility was obtained. The Birch–Murnaghan equation and the magnetic date were used to determine the spin gap Δ S as the difference between the energies of high-spin and low-spin states in these compounds.

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Доп.точки доступа:
Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Orlov, Yu. S.; Орлов, Юрий Сергеевич; Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Vereschagin, S. N.; Perov, N. S.; Siberian Branch of Russian Academy of Sciences [38]; Moscow International Symposium on Magnetism(6 ; 2014 ; June-July ; Moscow)
}
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Contribution of Co3+ ions to the high-temperature magnetic and electrical properties of GdCoO3 / V. A. Dudnikov [et al.] // J. Exp. Theor. Phys. - 2012. - Vol. 114, Is. 5. - P. 841-849, DOI 10.1134/S106377611203003X. - Cited References: 28. - This work was supported by the Ural Branch of the Russian Academy of Sciences and Siberian Branch of the Russian Academy of Sciences (project no. 40), the Russian Foundation for Basic Research (project nos. 09-02-00171-a, 10-02-00251), program 2.3 of the Department of Physical Sciences of Russian Academy of Sciences, and Nonprofit Dinastiya Foundation. . - ISSN 1063-7761

РУБ Physics, Multidisciplinary
Рубрики:
SPIN-STATE
   RCOO3 R
   TRANSITIONS
   COBALTITES
   LACOO3
   OXIDES
   SM
   EU
   ND
Аннотация: The temperature dependence of the static magnetization of polycrystalline rare-earth cobaltite GdCoO3 is measured in the temperature range 2-800 K. The magnetic behaviors of GdCoO3 and Gd3+ are found to be different at temperatures above room temperature, which is caused by the appearance of a contribution from Co3+ ions at high temperatures. The temperature dependence of the magnetic susceptibility of GdCoO3 is determined by the magnetization of rare-earth gadolinium ions and the additional paramagnetic contribution induced by the thermally excited magnetic terms of Co3+ ions. The LDA + GTB method is used to calculate the electronic structure of GdCoO3 in the temperature range 0-300 K with allowance for strong electron correlations. The energy spectrum of GdCoO3 is found to have intragap states that decrease the dielectric gap width with increasing temperature.

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Публикация на русском языке Вклад ионов Co3+ в высокотемпературные магнитные и электрические свойства GdCoO3 [Текст] / В. А. Дудников [и др.] // Ж. эксперим. и теор. физ. : Наука, 2012. - Т. 141 Вып. 5. - С. 966-975

Держатели документа:
[Dudnikov, V. A.
Ovchinnikov, S. G.
Orlov, Yu S.
Kazak, N. V.
Patrin, G. S.
Yurkin, G. Yu] Russian Acad Sci, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
[Dudnikov, V. A.] Reshetnev Siberian State Aerosp Univ, Krasnoyarsk 660014, Russia
[Ovchinnikov, S. G.
Patrin, G. S.] Siberian Fed Univ, Krasnoyarsk 660041, Russia
[Michel, C. R.] Univ Guadalajara, Guadalajara 44430, Jalisco, Mexico

Доп.точки доступа:
Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Orlov, Yu.S.; Орлов, Юрий Сергеевич; Kazak, N. V.; Казак, Наталья Валерьевна; Michel, C. R.; Patrin, G. S.; Патрин, Геннадий Семёнович; Yurkin, G.Yu.; Юркин, Глеб Юрьевич
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Contribution of the multiplicity fluctuation in the temperature dependence of phonon spectra of rare-earth cobaltites / Y. S. Orlov, A. E. Sokolov, V. A. Dudnikov [et al.] // Molecules. - 2020. - Vol. 25, Is. 18. - Ст. 4316, DOI 10.3390/molecules25184316. - Cited References: 34. - This work was supported by the Russian Science Foundation grant 18-02-00022. The scanning electron microscopy investigations were conducted in the SFU Joint Scientific Center, supported by the State assignment (#FSRZ-2020-0011) of the Ministry of Science and Higher Education of the Russian Federation. The other research was carried out at the Krasnoyarsk Regional Center of Research Equipment of the Federal Research Center “Krasnoyarsk Science Center SB RAS” . - ISSN 1420-3049
Кл.слова (ненормированные):
Rare-earth cobalt oxides -- Multiplicity fluctuations -- Phonon spectra
Аннотация: We have studied, both experimentally and theoretically, the unusual temperature dependence of the phonon spectra in NdCoO3, SmCoO3 and GdCoO3, where the Co3+ ion is in the low-spin (LS) ground state, and at the finite temperature, the high-spin (HS) term has a nonzero concentration nHS due to multiplicity fluctuations. We measured the absorption spectra in polycrystalline and nanostructured samples in the temperature range 3–550 K and found a quite strong breathing mode softening that cannot be explained by standard lattice anharmonicity. We showed that the anharmonicity in the electron–phonon interaction is responsible for this red shift proportional to the nHS concentration.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Institute of Engineering Physics and Radio Electronics, Siberian Federal University, Krasnoyarsk, 660041, Russian Federation

Доп.точки доступа:
Orlov, Yu. S.; Орлов, Юрий Сергеевич; Sokolov, A. Е.; Соколов, Алексей Эдуардович; Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Shulga, K. V.; Volochaev, M. N.; Волочаев, Михаил Николаевич; Zharkov, S. M.; Жарков, Сергей Михайлович; Shestakov, N. P.; Шестаков, Николай Петрович; Vysotin, M. A.; Высотин, Максим Александрович; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич
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Crystal structure and electronic states of Co and Gd ions in a Gd0.4Sr0.6CoO2.85 single crystal / M. S. Platunov [et al.] // JETP Letters. - 2016. - Vol. 103, Is. 3. - P. 196-200, DOI 10.1134/S0021364016030139. - Cited References:20. - This work was supported in part by the Russian Foundation for Basic Research (project nos. 13-02-00958, 13-02-00358, 14-02-31051, and 16-32-60049), by the Council of the President of the Russian Federation for Support of Young Scientists and Leading Scientific Schools (project no. SP-938.2015.5), and by the program "UMNIK." The X-ray diffraction and thermochemical studies were supported by the Siberian Branch, Russian Academy of Sciences (project no. V.45.3.1). . - ISSN 0021-3640. - ISSN 1090-6487

РУБ Physics, Multidisciplinary
Рубрики:
X-RAY-ABSORPTION
   PROFILE REFINEMENT
   PEROVSKITE
   CHARGE
   SPIN
Аннотация: X-ray diffraction and X-ray absorption near edge structure (XANES) spectra have been measured at the Со K-edge and Gd L3-edge in GdCoO3 and Gd0.4Sr0.6CoO2.85 cobaltites. The effect of Sr substitution on the crystal structure and electronic and magnetic states of Co3+ ions in a Gd0.4Sr0.6CoO2.85 single crystal has been analyzed. The XANES measurements at the Co K-edge have not showed a noticeable shift of the absorption edge with an increase in the concentration of Sr. This indicates that the effective valence of cobalt does not change. An increase in the intensity of absorption at the Gd L3-edge is due to an increase in the degree of hybridization of the Gd(5d) and O(2p) states. The effect of hole doping on the magnetic properties results in the appearance of the ferromagnetic component and in a significant increase in the magnetic moment.

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Публикация на русском языке Кристаллическая структура и электронные состояния ионов Co и Gd в монокристалле Gd0.4Sr0.6CoO2.85 [Текст] / М. С. Платунов [и др.] // Письма в Журн. эксперим. и теор. физ. : Наука, 2016. - Т. 103 Вып. 3-4. - С. 214-219

Держатели документа:
Russian Acad Sci, Kirensky Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia.
Russian Acad Sci, Inst Chem & Chem Technol, Siberian Branch, Krasnoyarsk 660036, Russia.
Natl Res Ctr Kurchatov Inst, Pl Akad Kurchatova 1, Moscow 123182, Russia.
Natl Res Nucl Univ MEPhI, Kashirskoe Sh 31, Moscow 115409, Russia.

Доп.точки доступа:
Platunov, M. S.; Платунов, Михаил Сергеевич; Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Orlov, Yu. S.; Орлов, Юрий Сергеевич; Kazak, N. V.; Казак, Наталья Валерьевна; Solovyov, L. A.; Соловьев, Леонид Александрович; Zubavichus, Y. V.; Veligzhanin, A. A.; Dorovatovskii, P. V.; Vereshchagin, S. N.; Shaykhutdinov, K. A.; Шайхутдинов, Кирилл Александрович; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Russian Foundation for Basic Research [13-02-00958, 13-02-00358, 14-02-31051, 16-32-60049]; Council of the President of the Russian Federation for Support of Young Scientists and Leading Scientific Schools [SP-938.2015.5]; program "UMNIK"; Siberian Branch, Russian Academy of Sciences [V.45.3.1]
}
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10.

Crystal structure and electronic statesof the Co and Gd ions in the single crystal Gd0.4Sr0.6CoO2.85 / V. A. Dudnikov [et al.] // VI Euro-Asian Symposium "Trends in MAGnetism" (EASTMAG-2016) : abstracts / ed.: O. A. Maksimova, R. D. Ivantsov. - Krasnoyarsk : KIP RAS SB, 2016. - Ст. P3.12. - P. 194. - References: 2. - This work was supported by Russian Science Foundation (Project 16-13-00060) . - ISBN 978-5-904603-06-9
Кл.слова (ненормированные):
Gd1-xSrxCoO3-δ perovskites -- X-ray absorption spectroscopy -- valence state -- electronic structure

Доп.точки доступа:
Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Platunov, M. S.; Платунов, Михаил Сергеевич; Orlov, Yu. S.; Орлов, Юрий Сергеевич; Kazak, N. V.; Казак, Наталья Валерьевна; Solov’ev, L. A.; Соловьев, Леонид Александрович; Zubavichus, Y. V.; Veligzhanin, A. A.; Велигжанин А. А.; Dorovatovskii, P. V.; Дороватовский П. В.; Vereshchagin, S. N.; Верещагин, С. Н.; Shaikhutdinov, K. A.; Шайхутдинов, Кирилл Александрович; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Euro-Asian Symposium "Trends in MAGnetism"(6 ; 2016 ; Aug. ; 15-19 ; Krasnoyarsk); "Trends in MAGnetism", Euro-Asian Symposium(6 ; 2016 ; Aug. ; 15-19 ; Krasnoyarsk); Институт физики им. Л.В. Киренского Сибирского отделения РАН

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11.

Crystal structure and thermoelectric properties of mechanically activated LaCoO3 / V. A. Dudnikov, Yu. S. Orlov, L. A. Solovyov [et al.] // J. Taiwan Inst. Chem. Eng. - 2024. - Vol. 162. - Ст. 105560, DOI 10.1016/j.jtice.2024.105560. - Cited References: 88. - This study was supported by the Russian Science Foundation , project no. 24-22-00091 . - ISSN 1876-1070. - ISSN 1876-1089
Кл.слова (ненормированные):
Rare-earth cobalt oxides -- Crystal structure -- Thermoelectric properties -- Mechanical activation
Аннотация: Background: Crystal structure of rare-earth LaCoO3 cobalt oxide subjected to high energy mechanical activation has been studied. In the temperature range of 300–800 K, the electrical conductivity and Seebeck coefficient were measured. Thermal conductivity was measured at 300–480 K. Methods: Comparative analysis of thermoelectric properties of the samples prepared by standard solid-state reaction and using high-energy mechanical activation was carried out. Findings: It was found that the experimental X-ray diffraction patterns are best described within the model that allows the coexistence of two domains in samples with the same crystal symmetry, but different lattice a and c parameters. The percentage ratio of these domains in the samples depends significantly on the size of the initial particles in the solid-state synthesis reaction and the annealing temperature. Mechanical activation and increase of synthesis temperature result in change of Seebeck coefficient sign and significant decrease of electrical resistivity. The Seebeck coefficient of non-activated samples takes positive values over the entire temperature range and decreases monotonically with increasing temperature, in contrast to mechanically activated samples exhibiting ambipolar behavior.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russia
Siberian Federal University, Krasnoyarsk, 660041, Russia
Institute of Chemistry and Chemical Technology, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russia

Доп.точки доступа:
Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Orlov, Yu. S.; Орлов, Юрий Сергеевич; Solovyov, L. A.; Vereshchagin, S. N.; Ustyuzhanin, Yu. N.; Устюжанин, Юрий Николаевич; Zharkov, S. M.; Жарков, Сергей Михайлович; Zeer, G. M.; Borus, A. A.; Борус, Андрей Андреевич; Bondarev, V. S.; Бондарев, Виталий Сергеевич; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич
}
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12.

Effect of A-site cation ordering on the thermoelectric properties of the complex cobalt oxides Gd1-xSrxCoO3-δ (x = 0.8 and 0.9) / V. A. Dudnikov [et al.] // Ceram. Int. - 2018. - Vol. 44, Is. 9. - P. 10299-10305, DOI 10.1016/j.ceramint.2018.03.037. - Cited References: 38. - This work was supported by the Russian Science Foundation , project no. 16-13-00060. . - ISSN 0272-8842
Кл.слова (ненормированные):
Substituted rare earth cobalt oxides -- Thermoelectric oxide materials -- Ordered and disordered states
Аннотация: The effect of substitution of Sr2+ ions for Gd3+ ions on the phase composition, electrical resistivity, thermoelectricity, and thermal conductivity of rare-earth cobalt oxides Gd1-xSrxCoO3-δ (x = 0.8 and 0.9) has been investigated. It has been determined that at the investigated strontium concentrations, the single-phase disordered nonstoichiometric cubic perovskites and superstructures with ordered Sr2+/Gd3+ ions and anion vacancies can be formed. The influence of ordering/disordering of Gd and Sr cations over crystal-lattice A- sites on the thermoelectric figure of merit and sample stability at high temperatures has been studied. The thermoelectric figure of merit of the disordered samples was found to exceed by far the analogous parameter of the ordered samples, which allows us to consider the disordering as a way of improving the thermoelectric parameters. Two contributions to the conductivities are discussed: high-temperature thermoactivation and low-temperatures variable range hopping. The parameters of the Mott electronic structure, including DOS N(εF), hopping energy ε (the energy of hopping conductivity activation), and hopping length Rh, have been estimated.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation
Siberian Federal University, Krasnoyarsk, Russian Federation
Institute of Chemistry and Chemical Technology, Federal Research Center KSC SB RAS, Krasnoyarsk, Russian Federation
Ioffe Physical-Technical Institute, Russian Academy of Sciences, St. Petersburg, Russian Federation
Lebedev Physical Institute, Russian Academy of Sciences, Moscow, Russian Federation

Доп.точки доступа:
Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Orlov, Yu. S.; Орлов, Юрий Сергеевич; Kazak, N. V.; Казак, Наталья Валерьевна; Fedorov, A. S.; Федоров, Александр Семенович; Solov'yov, L. A.; Vereshchagin, S. N.; Burkov, A. T.; Novikov, S. V.; Gavrilkin, S. Yu.; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич
}
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13.

Effect of cation ordering on a-sites on the physical properties of substituted rare-earth cobaltite oxides GD1-XSRXCOO3-Δ / V. A. Dudnikov [et al.] // Moscow International Symposium on Magnetism (MISM-2017) : 1-7 July 2017 : book of abstracts. - 2017. - Ст. 4PO-I-48. - P. 878

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Доп.точки доступа:
Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Orlov, Yu. S.; Орлов, Юрий Сергеевич; Gavrilkin, S. Yu.; Kazak, N. V.; Казак, Наталья Валерьевна; Platunov, M. S.; Платунов, Михаил Сергеевич; Solovyov, L. A.; Соловьев, Леонид Александрович; Vereshchagin, S. N.; Velikanov, D. A.; Великанов, Дмитрий Анатольевич; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Moscow International Symposium on Magnetism(7 ; 2017 ; Jul. ; Moscow); Московский государственный университет им. М.В. Ломоносова; Российский фонд фундаментальных исследований
Нет сведений об экземплярах (Источник в БД не найден)
}
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14.

    Effect of Gd and Sr ordering in a sites of doped Gd0.2Sr0.8CoO3-δ perovskite on its structural, magnetic, and thermodynamic properties / V. A. Dudnikov [et al.] // J. Phys. Chem. C. - 2016. - Vol. 120, Is. 25. - P,. 13443-13449, DOI 10.1021/acs.jpcc.6b04810. - Cited References: 45. - The authors are thankful to the Russian Science Foundation (Project No. 16-13-00060) for financial support. The magnetic measurements were carried out in the Shared Facility Centre of P. N. Lebedev Physical Institute of RAS. . - ISSN 1932-7447
Рубрики:
Ln1-xSrxCoO(3-δ) Ln
   PROFILE REFINEMENT
   CRYSTAL-STRUCTURE
   OXYGEN-CONTENT
   COBALTITES
   OXIDE
   La1-xSrxCoO3-δ
   Dy3+
   SPIN
   Ho3+
Аннотация: Magnetic and thermodynamic properties of perovskite Gd0.2Sr0.8CoO3−δ, with ordered and disordered states of Gd and Sr in the A-sites of the crystal lattice have been studied revealing remarkable differences in the physical properties of the ordered and disordered states. The ordered samples have larger oxygen nonstoichiometry, heat capacity, and thermal expansion anomalies, and abnormal temperature dependence of the magnetization around 350 K.

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Держатели документа:
Kirensky Institute of Physics, Krasnoyarsk, Russian Federation
Siberian Federal University, Krasnoyarsk, Russian Federation
Lebedev Physical Institute, Moscow, Russian Federation
Institute of Chemistry and Chemical Technology, Krasnoyarsk, Russian Federation
Faculty of Physics, Lomonosov Moscow State University, Moscow, Russian Federation

Доп.точки доступа:
Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Orlov, Yu. S.; Орлов, Юрий Сергеевич; Gavrilkin, S. Yu.; Gorev, M. V.; Горев, Михаил Васильевич; Vereshchagin, S. N.; Solovyov, L. A.; Соловьев, Леонид Александрович; Perov, N. S.; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич
}
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15.

Effect of mechanical activation on the thermoelectric properties of Sr1-xSmxTiO3 ceramics / Y. S. Orlov, S. N. Vereshchagin, S. V. Novikov [et al.] // Ceram. Int. - 2021. - Vol. 47, Is. 20. - P. 28992-28999, DOI 10.1016/j.ceramint.2021.07.060. - Cited References: 31. - This study was supported by the Russian Science Foundation, project no. 19-72-00097 . - ISSN 0272-8842. - ISSN 1873-3956

РУБ Materials Science, Ceramics
Рубрики:
SRTIO3
   LA
   MICROSTRUCTURE
   CONDUCTIVITY
   PERFORMANCE
   FIGURE
   MERIT
Кл.слова (ненормированные):
Strontium titanate solid solutions -- Thermoelectric oxide materials -- Mechanochemical activation
Аннотация: The Sr1-xSmxTiO3 (х = 0.025, 0.05, 0.075, 0.1, 0.2) strontium titanate solid solutions were prepared from oxides and carbonates using a conventional ceramic technology based on the mechanochemical activation. The electrical conductivity and Seebeck coefficient of the synthesized compounds were measured in the temperature range from 300 to 800 K. We found that the properties of the samples significantly depend on the preliminary mechanochemical activation. The thermoelectric power factor attains maximum value in the hydrogen reduced samples with concentration of х = 0.05 and 0.075 obtained from nanoparticles: 5.5 μW/(cm · K2) for Sr0.95Sm0.05TiO3 (580 K) and 4.10 μW/(cm · K2) for Sr0.925Sm0.075TiO3 (650 K). An increase in the annealing temperature of mechanically activated samples leads to an even greater increase in electrical conductivity and power factor: 9.2 μW/(cm · K2) for Sr0.925Sm0.075TiO3 (650 K).

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Держатели документа:
Russian Acad Sci, Siberian Branch, Krasnoyarsk Sci Ctr, Kirensky Inst Phys, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Russian Acad Sci, Inst Chem & Chem Technol, Krasnoyarsk Sci Ctr, Siberian Branch, Krasnoyarsk 660036, Russia.
Ioffe Inst, St Petersburg 194021, Russia.

Доп.точки доступа:
Orlov, Yu. S.; Орлов, Юрий Сергеевич; Vereshchagin, S. N.; Novikov, S., V; Burkov, A. T.; Borus, A. A.; Борус, Андрей Андреевич; Sitnikov, M., V; Solovyov, L. A.; Volochaev, M. N.; Волочаев, Михаил Николаевич; Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Russian Science FoundationRussian Science Foundation (RSF) [19-72-00097]
}
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16.

Effect of multiplicity fluctuation in cobalt ions on crystal structure, magnetic and electrical properties of NdCoO3 and SmCoO3 / V. A. Dudnikov, Y. S. Orlov, L. A. Solovyov [et al.] // Molecules. - 2020. - Vol. 25, Is. 6. - Ст. 1301, DOI 10.3390/molecules25061301. - Cited References: 56. - This work is supported by the Russian Science Foundation grant 18-02-00022. . - ISSN 1420-3049

РУБ Biochemistry & Molecular Biology + Chemistry, Multidisciplinary
Рубрики:
SPIN-STATE TRANSITIONS
   CO3+ ION
   CONDUCTIVITY
   TEMPERATURE
   BEHAVIOR
Кл.слова (ненормированные):
rare-earth cobalt oxides -- multiplicity fluctuations -- structural -- magnetic -- electrical -- and dilatation properties
Аннотация: The structural, magnetic, electrical, and dilatation properties of the rare-earth NdCoO3 and SmCoO3 cobaltites were investigated. Their comparative analysis was carried out and the effect of multiplicity fluctuations on physical properties of the studied cobaltites was considered. Correlations between the spin state change of cobalt ions and the temperature dependence anomalies of the lattice parameters, magnetic susceptibility, volume thermal expansion coefficient, and electrical resistance have been revealed. A comparison of the results with well-studied GdCoO3 allows one to single out both the general tendencies inherent in all rare-earth cobaltites taking into account the lanthanide contraction and peculiar properties of the samples containing Nd and Sm.

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Держатели документа:
RAS, Kirensky Inst Phys, Fed Res Ctr KSC, SB, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Inst Engn Phys & Radio Elect, Krasnoyarsk 660041, Russia.
RAS, Fed Res Ctr KSC, Inst Chem & Chem Technol, SB, Krasnoyarsk 660036, Russia.
Russian Acad Sci, Lebedev Phys Inst, Moscow 119991, Russia.
Russian Acad Sci, Ioffe Inst, St Petersburg 194021, Russia.

Доп.точки доступа:
Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Orlov, Yu. S.; Орлов, Юрий Сергеевич; Solovyov, Leonid A.; Vereshchagin, Sergey N.; Gavrilkin, Sergey Yu.; Tsvetkov, Alexey Yu.; Velikanov, D. A.; Великанов, Дмитрий Анатольевич; Gorev, M. V.; Горев, Михаил Васильевич; Novikov, Sergey V.; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Russian Science FoundationRussian Science Foundation (RSF) [18-02-00022]
}
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17.

Effect of oxygen nonstoichiometry on electrical conductivity and thermopower of Gd0.2Sr0.8FeO3-δ ferrite samples / V. Dudnikov [et al.] // Materials. - 2019. - Vol. 12, Is. 1. - Ст. 74, DOI 10.3390/ma12010074. - Cited References: 24 . - ISSN 1996-1944
Кл.слова (ненормированные):
Rare-earth-substituted cobalt oxides -- Stability -- Thermoelectric properties
Аннотация: The behavior of the resistivity and thermopower of the Gd0.2Sr0.8FeO3−δ ferrite samples with a perovskite structure and the sample stability in an inert gas atmosphere in the temperature range of 300–800 K have been examined. It has been established that, in the investigated temperature range, the thermoelectric properties in the heating‒cooling mode are stabilized at δ ≥ 0.21. It is shown that the temperature dependencies of the resistivity obtained at different δ values obey the activation law up to the temperatures corresponding to the intense oxygen removal from a sample. The semiconductor‒semiconductor electronic transitions accompanied by a decrease in the activation energy have been observed with increasing temperature. It is demonstrated that the maximum thermoelectric power factor of 0.1 µW/(cm·K2) corresponds to a temperature of T = 800 K.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center Krasnoyarsk Scientific Center, Russian Academy of Sciences, Siberian Branch, Krasnoyarsk, 660036, Russian Federation
Institute of Engineering Physics and Radio Electronics, Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Institute of Chemistry and Chemical Technology, Federal Research Center Krasnoyarsk Scientific Center, Russian Academy of Sciences, Siberian Branch, Krasnoyarsk, 660036, Russian Federation
Ioffe Institute, St. Petersburg, 194021, Russian Federation

Доп.точки доступа:
Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Orlov, Yu. S.; Орлов, Юрий Сергеевич; Fedorov, A. S.; Федоров, Александр Семенович; Solovyov, L.; Vereshchagin, S.; Burkov, A. T.; Novikov, S.; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич
}
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18.

    Electronic states of the iron ions in the oxygen deficient perovskite Gd0.2Sr0.8FeO3-δ / Yu. V. Knyazev [и др.] // Мёссбауэровская спектроскопия и её применения : сб. материалов XV международной конференции. - Ростов-на-Дону, 2018. - С. 45 . - ISBN 978-5-9275-2831-8
   Перевод заглавия: Электронные состояния ионов железа в перовските Gd0.2Sr0.8FeO3-δ

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Доп.точки доступа:
Knyazev, Yu. V.; Князев, Юрий Владимирович; Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Kazak, N. V.; Казак, Наталья Валерьевна; Platunov, M. S.; Платунов, Михаил Сергеевич; Solovyov, L. A.; Соловьев, Леонид Александрович; Verechschagin, S. N.; Burkov, A. T.; Novikov, S. V.; Мёссбауэровская спектроскопия и её применения, международная конференция(15 ; 2018 ; сент ; 10-16 ; Сочи); Mössbauer Spectroscopy and Applications, International Conference(15 ; 2018 ; Sept. ; 10-16 ; Sochi); Южный федеральный университет; МИРЭА-Российский технологический университет; Российская академия наук; Институт кристаллографии им. А.В. Шубникова РАН; Федеральный научно-исследовательский центр "Кристаллография и фотоника" РАН; Московский государственный университет им. М.В. Ломоносова
}
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19.

Element selective magnetism in Ho0.5Nd0.5Fe3(BO3)4 single crystal probed with hard X-ray magnetic circular dichroism / M. Platunov [et al.] // J. Magn. Magn. Mater. - 2019. - Vol. 479. - P. 312-316, DOI 10.1016/j.jmmm.2019.02.040. - Cited References: 40. - The study was supported in part by the grants of the Russian Foundation for Basic Research (project Nos. 16-32-60049, 17-02-00826, 18-42-243007) and the Foundation for Assistance to Small Innovative Enterprises (FASIE, UMNIK program). The magnetic measurements were carried out in the Shared Facility Centre of P.N. Lebedev Physical Institute of RAS. We are grateful to Dr. Alexey Bosak for providing assistance of the structural experiments on the ID28 beamline. We are also grateful to Dr. Evgeniy Eremin from Kirensky Institute of Physics for providing the results of magnetic measurements and for useful discussions. The authors thank the ID12 beamline staffs for help during the XMCD experiment and also gratefully acknowledge the beamtime provision (proposal HC-1804) by the ESRF. . - ISSN 0304-8853. - ISSN 1873-4766

РУБ Materials Science, Multidisciplinary + Physics, Condensed Matter
Рубрики:
MICROSTRUCTURE
TRANSITIONS
ND
Кл.слова (ненормированные):
X-ray magnetic circular dichroism -- X-ray absorption -- Magnetic properties
Аннотация: We present a study of a Ho0.5Nd0.5Fe3(BO3)4 single crystal aiming at understanding the roles of each magnetic sublattices in magnetic transitions at low temperatures. The crystal structure is determined to have the R32 symmetry in whole studied temperature range but the crystal appears to be racemic. Element selective magnetic properties studied with X-ray magnetic circular dichroism at the L2,3-edges of Ho and Nd, and at the Fe K-edge at T = 3 K under magnetic fields of ±17 T are compared with the results of macroscopic magnetization measurements in pure and substituted crystals. All three magnetic sublattices are shown to be strongly coupled and to undergo a spin-reorientation transition when magnetic field is applied along the trigonal c-axis. On the contrary, when magnetic field is applied in the ab-plane only the holmium atoms exhibit a sizeable magnetization jump. This result allows us to conclude that the spin-flop transitions observed in macroscopic magnetization curves and associated anomalies of electric polarization are due to the Ho3+ magnetic moment reorientation.

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Держатели документа:
RAS, Fed Res Ctr KSC SB, Kirensky Inst Phys, Akademgorodok 50,Bld 38, Krasnoyarsk 660036, Russia.
European Synchrotron, ESRF, 71 Ave Martyrs CS40220, F-38043 Grenoble 9, France.
Swiss Norwegian Beamlines ESRF, 71 Ave Martyrs CS40220, F-38043 Grenoble 9, France.
RAS, PN Lebedev Phys Inst, Moscow 119991, Russia.

Доп.точки доступа:
Platunov, M. S.; Платунов, Михаил Сергеевич; Kazak, N. V.; Казак, Наталья Валерьевна; Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Temerov, V. L.; Темеров, Владислав Леонидович; Gudim, I. A.; Гудим, Ирина Анатольевна; Knyazev, Yu. V.; Князев, Юрий Владимирович; Gavrilkin, S. Yu.; Dyadkin, Vadim; Dovgaliuk, Iurii; Chernyshov, Dmitry; Hen, Amir; Wilhelm, Fabrice; Rogalev, Andrei; Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Russian Foundation for Basic Research [16-32-60049, 17-02-00826, 18-42-243007]; Foundation for Assistance to Small Innovative Enterprises (FASIE, UMNIK program)
}
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20.

Exciton Phase in Strongly Correlated Systems with the Spin Crossover / Yu. S. Orlov, S. V. Nikolaev, V. A. Dudnikov, S. G. Ovchinnikov // International conference "Functional materials" : book of abstracts / ed. V. N. Berzhansky ; org. com. S. G. Ovchinnikov [et al.]. - Simferopol, 2021. - P. 40. - Библиогр.: 3 назв. - The authors thank the Russian Scientific Foundation for the financial support under the grant 18-12-00022.

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Доп.точки доступа:
Berzhansky, V. N. \ed.\; Бержанский, Владимир Наумович; Ovchinnikov, S. G. \org. com.\; Овчинников, Сергей Геннадьевич; Orlov, Yu. S.; Орлов, Юрий Сергеевич; Nikolaev, S. V.; Николаев, Сергей Викторович; Dudnikov, V. A.; Дудников, Вячеслав Анатольевич; Ovchinnikov, S. G.; "Functional materials", International conference(2021 ; Oct. 4-8 ; Alushta, Russia); Крымский федеральный университет имени В.И. Вернадского
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