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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zobov V. E., Ivanov Y. N., Popov M. A., Livshits A. I.
Заглавие : Orientational dependence of the tails of dipole-broadened NMR spectra in crystals
Место публикации : J. Exp. Theor. Phys.: AMER INST PHYSICS, 1999. - Vol. 88, Is. 1. - P157-167. - ISSN 1063-7761, DOI 10.1134/1.558778
Примечания : Cited References: 36
Предметные рубрики: NUCLEAR-DOUBLE-RESONANCE
FLUCTUATION SPECTRUM
CROSS-RELAXATION
SOLIDS
DIFFUSION
MEMORY
SHAPE
Аннотация: This paper describes experimental and theoretical studies of the tails of the dipole-broadened nuclear magnetic resonance (NMR) absorption spectra of F-19 in isomorphic single crystals of BaF2 and CaF2 with the magnetic field directed along three crystallographic axes. The results obtained by directly measuring the derivative of the tail of the NMR absorption spectrum and the falloffs of the Engelsberg-Lowe free precession after Fourier transformation qualitatively agree. It is shown that the shape of the tail is well described by an exponential function in which the orientational dependence of the exponent does not reduce to variation of the second moment. The observed shape of the tail and the orientational dependence of its parameters are explained on the basis of a self-consistent fluctuating-local-field theory. Nonlinear integral equations are derived for the correlation functions, taking into account the changes of the actual number of nearest neighbors caused by the anisotropy of the dipole-dipole interaction and the contribution of lattice sums with loops. The equations are solved numerically. Good agreement is obtained for the computed dropoffs of the free precession, the NMR spectra, and the cross-polarization rates with the experimental results. (C) 1999 American Institute of Physics. [S1063-7761(99)02401-4].
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zobov V. E., Popov M. A.
Заглавие : A Monte Carlo study of the dependence of the growth parameter for trees on the lattice dimension in the Eden model
Место публикации : Theor. Math. Phys. - 2001. - Vol. 126, Is. 2. - P.270-279. - ISSN 0040-5779, DOI 10.1023/A:1005260114182
Примечания : Cited References: 17
Предметные рубрики: DIFFUSION-LIMITED AGGREGATION
BRANCHED POLYMERS
HIGH-TEMPERATURES
EXPANSION
TIME
Аннотация: We use the Monte Carlo method to compute the number of trees with n edges in the Eden model on d-dimensional simple cubic lattices for d = 2, 3, 4, 6, 8, 10. We compare these numbers with the exact data derived by the enumeration method up to n = 12 on the square lattice and up to n = 10 on the cubic lattice. We find that for d greater than or equal to 3, the computed values of the growth parameter for trees agree with the values that we derived earlier by the expansion in inverse powers of 2d - 1.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kaptsov O. V., Verevkin I. V.
Заглавие : Differential constraints and exact solutions of nonlinear diffusion equations
Место публикации : J. Phys. A. - 2003. - Vol. 36, Is. 5. - P.1401-1414. - ISSN 0305-4470, DOI 10.1088/0305-4470/36/5/315
Примечания : Cited References: 29
Предметные рубрики: REDUCTION
Аннотация: The differential constraints are applied to obtain explicit solutions of nonlinear diffusion equations. Certain linear determining equations with parameters are used to find such differential constraints. They generalize the determining equations used in the search for classical Lie symmetries.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Markel V. A., Shalaev V. M., Poliakov E. Y., George T. F.
Заглавие : Numerical studies of second- and fourth-order correlation functions in cluster-cluster aggregates in application to optical scattering
Место публикации : Phys. Rev. E: AMERICAN PHYSICAL SOC, 1997. - Vol. 55, Is. 6. - P7313-7333. - ISSN 1063-651X, DOI 10.1103/PhysRevE.55.7313
Примечания : Cited References: 21
Предметные рубрики: DIFFUSION-LIMITED AGGREGATION
COLLOIDAL AGGREGATION
FRACTAL CLUSTERS
ANTICORRELATION
SIMULATIONS
Аннотация: Two- and four-point density correlation functions p(2)(r) and p(4)(r) are studied numerically and theoretically in computer-generated three-dimensional lattice cluster-cluster aggregates (CCA) with the number of particles N up to 20 000 in application to the light scattering problem. The ''pure'' aggregation algorithm is used, where subclusters of all possible sizes are allowed to collide. We find that large CCA clusters demonstrate pronounced multiscaling. In particular, the fractal dimension determined from the slope of p(2)(r) at small distances differs from that found from the dependence of the radius of gyration on the number of monomers (according to our data, 1.80 and 1.94, respectively). We also consider different functional forms for p(2) and their general properties and applicability. We find that the best fit to the numerical data is provided by the generalized exponential cutoff function with coefficients depending on N. The latter dependence is a manifestation of multiscaling. We propose some theoretical approaches for calculating p(4)(r), assuming p(2)(r) is known. In particular, we find the small-r asymptote for the p(4)(r) and verify it numerically. In addition, we find that p(4)(r) cannot be represented by a scaling dependence with a cutoff function, like p(2)(r) Instead, p(4)(r) is given by an expansion in terms of integer powers of r(2D-3), where D is the fractal dimension (approximate to 1.8 for CCA clusters).
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Fedorov A. S., Sadreev A. F.
Заглавие : Thermoactivated transport of molecules H-2 in narrow single-wall carbon nanotubes
Коллективы : RFBR [0602-16132]
Разночтения заглавия :авие SCOPUS: Thermoactivated transport of molecules H 2 in narrow single-wall carbon nanotubes
Место публикации : Eur. Phys. J. B: SPRINGER, 2009. - Vol. 69, Is. 3. - P363-368. - ISSN 1434-6028, DOI 10.1140/epjb/e2009-00152-1
Примечания : Cited References: 40. - We are grateful to S. G. Ovchinnikov for discussions. This work has been supported by RFBR grant 0602-16132.
Предметные рубрики: DIFFUSION
NANOPORES
ENERGY
MOTION
FLUIDS
Ключевые слова (''Своб.индексиров.''): hydrogen molecule--inner potential--lennard-jones potential--periodic potentials--plane wave--potential surfaces--single-wall carbon nanotubes--thermal fluctuations--tube walls--carbon nanotubes--hydrogen--molecules--single-walled carbon nanotubes (swcn)
Аннотация: By use both of the plane wave DFT and the empirical exp-6 Lennard-Jones potential methods we calculate the inner potential in narrow single-wall carbon nanotubes (SWCNT) (6, 0), (7, 0) and (3, 3) which affects the hydrogen molecules. The inner potential forms a goffered potential surface and can be approximated as V(z,r,phi)a parts per thousand V(0)sin (2 pi z/a)+V(r). We show that in these SWCNTs transport of molecules is given mainly by thermoactivated hoppings between minima of the periodic potential along the tube axis. The rate hoppings is substantially depends on temperature because of thermal fluctuations of tube wall.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Myagkov V. G., Mikhlin Y. N., Bykova L. E., Mal'tsev V. K., Bondarenko G. N.
Заглавие : Long-Range Chemical Interaction in Solid-State Synthesis: The Formation of a CuAu Alloy in Au/beta-Co(001)/Cu(001) Epitaxial Film Structures
Коллективы : Russian Foundation for Basic Research [07-03-00190]; Ministry of Education and Science of the Russian Federation
Разночтения заглавия :авие SCOPUS: Long-range chemical interaction in solid-state synthesis: The formation of a CuAu alloy in Au/β-Co(001)/Cu(001) epitaxial film structures
Место публикации : JETP Letters. - 2009. - Vol. 90, Is. 2. - P.111-115. - ISSN 0021-3640, DOI 10.1134/S0021364009140069
Примечания : Cited References: 25. - This work was supported by Russian Foundation for Basic Research ( project no. 07-03-00190) and the Ministry of Education and Science of the Russian Federation ( program "Development of the Scientific Potential of Higher Education").
Предметные рубрики: THIN-FILMS
PHASE-TRANSITION
DIFFUSION
MICROSTRUCTURE
INTERLAYER
INTERFACE
COSI2
AU
Аннотация: The effect of an inert Co layer (0, 210, 480 nm) on the chemical interaction between Cu and Au in Au/beta-Co(001)/Cu(001) epitaxial films has been investigated by X-ray diffraction, nuclear magnetic resonance, photoelectron spectroscopy, and magnetic structure measurements. Mixing at interfaces in Cu/beta-Co(001) and Au/beta-Co(001) bilayer films has not been revealed up to a temperature of 600 C. The solid-state synthesis of ordered CuAu| and CuAu|| phases occurs through the Co inert buffer layer in Au/beta-Co(001)/Cu(001) trilayer film systems with an increase in the annealing temperature. The initiation temperatures of the CuAu| and CuAu|| phases increase only slightly with the thickness of the Co buffer layer. The assumption of the long range of the chemical interaction between Cu and Au through the chemically inert Co layer is justified using the performed investigations.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Fedorov A. S., Sadreev A. F.
Заглавие : Ab-initio investigation of thermoactivated directional transport of hydrogen molecules inside narrow carbon nanotubes
Место публикации : Phys. Status Solidi B. - 2009. - Vol. 246: 23rd Winterschool on Electronic Properties of Novel Materials (MAR 14, 2009, Kirchberg, GERMANY), Is. 11. - P.2598-2601. - ISSN 0370-1972, DOI 10.1002/pssb.200982285
Примечания : Cited References: 21. - A.S.Fedorov thanks the Institute of Computer Modeling (Krasnoyarsk, Russia) and the Joint Supercomputer Center (Moscow) for an assistence in quantum chemical calculations.
Предметные рубрики: DIFFUSION
ENERGY
Аннотация: Using the pseudopotential DFT and the empirical potential methods we calculate the potential acting to the hydrogen molecules in narrow single-wall carbon nanotubes (SWCNT) (6,0),(7,0) and (3,3). The potential forms a goffered potential surface and can be approximated as V(z, r, phi) approximate to V(0) sin(2 pi z/a) + V(r). We show that in these SWCNTs transport of molecules is given mainly by thermoactivated hoppings between minima of the periodic potential along the tube axis. Taking into account that hydrogen density distribution inside nanotube is stationary and assuming the temperature is changed linearly along the SWCNT length we show that the H(2) density is sufficiently variated, especially for the case of (6,0)SWCNT where the density on both SWCNT ends are different at similar to 30 times when the temperature is changed along the SWCNT from 300K to 1200K. Suppose that H2 molecules can penetrate in the both open SWCNT ends, the molecules would move in the direction of the temperature decreasing. This effect may be used potentially to build up a molecular pump driven by the temperature gradient along narrow nanotube. (C) 2009 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Myagkov V. G., Bykova L. E., Bondarenko G. N., Bondarenko G. V.
Заглавие : Long-range chemical interaction in solid-state synthesis: The Kirkendall effect and solid-state reactions in Cu/beta-CuZn and Cu/Fe/beta-CuZn film systems
Коллективы :
Разночтения заглавия :авие SCOPUS: Long-range chemical interaction in solid-state synthesis: The Kirkendall effect and solid-state reactions in Cu/β-CuZn and Cu/Fe/β-CuZn film systems
Место публикации : JETP Letters. - 2010. - Vol. 91, Is. 12. - P.665-669. - ISSN 0021-3640, DOI 10.1134/S0021364010120106
Примечания : Cited References: 26. - We are grateful to Yu. L. Mikhlin for the measurements of the X-ray photoelectron spectra and for stimulating discussions. This work was supported by the Ministry of Education and Science of the Russian Federation (project no. 2.1.1/4399, program "Development of the Scientific Potential of Higher Education in 2009-2010").
Предметные рубрики: PHASE-FORMATION
DIFFUSION
Аннотация: The results of the experimental investigations of the solid-state reaction of Cu with beta brass, which is associated with the Kirkendall, in Cu/beta-CuZn and Cu/Fe/beta-CuZn film systems are reported. It has been shown that the initiation temperature of the solid-state synthesis of alpha brass at the Cu/beta-CuZn interface is about 200A degrees C. The chemically inert Fe barrier layers 420 and 850 nm in thickness between the Cu and beta-CuZn films do not suppress the solid-state synthesis of the alpha brass, but increase the initiation temperature to about 250A degrees C. This behavior indicates that the chemical interaction between the Cu and Zn atoms through the chemically inert Fe layer is long-range. The X-ray photoelectron investigations reveal the migration of Zn atoms from the beta-CuZn layer through the Fe barrier to the Cu layer. The results are interpreted under the assumption that the migration of Zn atoms in the Kirkendall is initiated by the strong chemical interaction between the Cu and Zn atoms in the Cu and beta-CuZn layers, which is due to the synthesis of alpha brass, rather than by the diffusion random walk, as is commonly accepted at present.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Divin A., Markidis S., Lapenta G., Semenov V. S., Erkaev N. V., Biernat H. K.
Заглавие : Model of electron pressure anisotropy in the electron diffusion region of collisionless magnetic reconnection
Коллективы :
Место публикации : Phys. Plasmas: AMER INST PHYSICS, 2010. - Vol. 17, Is. 12. - Ст.122102. - ISSN 1070-664X, DOI 10.1063/1.3521576
Примечания : Cited References: 42. - The present work is supported partially by the Onderzoekfonds KU Leuven (Research Fund KU Leuven) and by the European Commission's Seventh Framework Programme (FP7/2007-2013) under grant Agreement No. 218816 (SOTERIA project, www.soteria- space.eu). Additional support is provided by RFBR (Grant No. 09-05-91000-ANF-a). V.S.S. thanks ISSI for hospitality and financial support. The simulations were conducted on the resources of the Vlaams Supercomputer Centrum (VSC) at the Katholieke Universiteit Leuven.
Предметные рубрики: CURRENT SHEETS
X-LINE
PLASMA
DISSIPATION
FIELD
SIMULATIONS
ACCELERATION
TRANSPORT
Ключевые слова (''Своб.индексиров.''): analytical results--antiparallel configuration--collisionless--electron diffusion--electron population--electron pressures--magnetic reconnections--neutral line--new model--particle-in-cell simulations--two particles--anisotropy--astrophysics--collisionless plasmas--computer simulation--diffusion--geophysics--magnetic fields--magnetic properties--plasma simulation--electrons
Аннотация: A new model of the electron pressure anisotropy in the electron diffusion region in collisionless magnetic reconnection is presented for the case of antiparallel configuration of magnetic fields. The plasma anisotropy is investigated as source of collisionless dissipation. By separating electrons in the vicinity of the neutral line into two broad classes of inflowing and accelerating populations, it is possible to derive a simple closure for the off-diagonal electron pressure component. The appearance of these two electron populations near the neutral line is responsible for the anisotropy and collisionless dissipation in the magnetic reconnection. Particle-in-cell simulations verify the proposed model, confirming first the presence of two particle populations and second the analytical results for the off-diagonal electron pressure component. Furthermore, test-particle calculations are performed to compare our approach with the model of electron pressure anisotropy in the inner electron diffusion region by Fujimoto and Sydora [Phys. Plasmas 16, 112309 (2009)]. (C) 2010 American Institute of Physics. [doi:10.1063/1.3521576]
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Bouznik V. M., Morozov E. V., Avilova I. A., Volkov V. I.
Заглавие : NMR applications for polymer composite materials moisture uptake investigation
Место публикации : Appl. Magn. Reson.: Springer, 2016. - Vol. 47, Is. 3. - P.321-334. - ISSN 09379347 (ISSN), DOI 10.1007/s00723-015-0748-2
Примечания : Cited References: 41. - This research was performed with the financial support of Russian Foundation for Basic Research (project no. 14-29-10178 ofi_m).
Предметные рубрики: FIELD GRADIENT NMR
REINFORCED EPOXY COMPOSITES
WATER SELF-DIFFUSION
TRANSPORT
GLASS
SYSTEM
SPECTROSCOPY
TEMPERATURE
ABSORPTION
ADHESIVE
Аннотация: The 1H nuclear magnetic resonance (NMR) spectroscopy, NMR imaging, and pulsed field gradient NMR (PFG NMR) were applied for comparative study of moisture–polymer composite materials (PCM) interaction. The water uptake in PCM reinforced by aramid and carbon fibers was measured by NMR spectroscopy techniques. The aramid fiber-reinforced PCM absorbs water more intensively compared with PCM reinforced by carbon fiber, but both of them are retaining water inside of pores without formation of chemical bonds. Using NMR imaging the spatial distribution of water absorbed was visualized; preferable water pathways and influence of surface treatment on water-resistant properties were revealed. It was found that the surface rough treatment sufficiently improves the water absorption, but penetration of water molecules is still occurring only through the surfaces and it happens within a thin layer. PFG NMR technique revealed influence of pore structure on moisture–PCM interaction; it was found that additionally to strong hydrophobic properties of carbon fiber, the smaller total volume of pores sufficiently decrease the water uptake. Results achieved in this work demonstrate efficiency of NMR methods applied all together for investigation of PCM, and information obtained is practically important when designing advanced PCM with required properties. © 2016, Springer-Verlag Wien.
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