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Zhandun, V. S.
The arising of ferromagnetism in Al-doped Mn2(Ga1−xAlx)C MAX phases / V. S. Zhandun, N. G. Zamkova, O. N. Draganyuk // J. Magn. Magn. Mater. - 2024. - Vol. 601. - Ст. 172193, DOI 10.1016/j.jmmm.2024.172193. - Cited References: 30. - The study was funded by a grant from the Russian Science Foundation # 23-22-10020 https://rscf.ru/project/23-22-10020/, Krasnoyarsk Regional Fund of Science. The calculations were performed with the computer resources of "Complex modeling and data processing research installations of mega-class" SRC "Kurchatovsky Institute" (http://ckp.urcki.ru). The ternary phase diagrams for the calculation of formation enthalpies were taken from Materials Project (https://materialsproject.org) and OQMD (https://oqmd.org/) databases . - ISSN 0304-8853. - ISSN 1873-4766
Кл.слова (ненормированные):
MAX phases -- First-principle calculations -- Doping -- Magnetic properties -- Ferromagnetism -- Exchange constants
Аннотация: The magnetic properties of ordered MAX phases Mn2(AlxGa1−x)C (x = 0.125, 0.25, 0.5, 0.75 and 0.875) have been studied within the DFT-GGA. We have found that increase of Al atom at A-site leads to the formation of the ferromagnetic phase with large magnetization of about 3.6 μB/f.u. The investigation of the phase stability is performed by comparing the total energy of the MAX phases with that of a set of competitive phases for calculation of the phase formation enthalpy. Up to a concentration of Al atoms x = 0.7 the compound remains thermodynamically stable. The exchange constants analysis shows the crucial role of exchange interactions between manganese atoms along the c-axis in forming of ferromagnetism. The magnetic transition temperature of Mn2(AlxGa1−x)C alloys increases with increase of the aluminum concentration.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk 660036, Russia
Professor L.F. Voino-Yasenetsky Krasnoyarsk State Medical University, Krasnoyarsk, 660022 Russia

Доп.точки доступа:
Zamkova, N. G.; Замкова, Наталья Геннадьевна; Draganyuk, O. N.; Драганюк, Оксана Николаевна; Жандун, Вячеслав Сергеевич
}
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    Modulation of Bi3+ luminescence from broadband green to broadband deep red in Lu2WO6 by Gd3+ doping and its applications in high color rendering index white LED and near-infrared LED / X. Wang, X. Feng, M. S. Molokeev [и др.] // Dalton Trans. - 2023. - Vol. 52, Is. 9. - P. 2619-2630, DOI 10.1039/D2DT03751C. - Cited References: 4. - This work is supported in part by the Project of Education Department of Liaoning Province (Grant No. LQ2019014) and he Natural Science Foundation of Liaoning Province (Grant No. 2020-MS-286). The authors are thankful for the support for the 4B9A Beamline from the Beijing Synchrotron Radiation Facility (BSRF) (Project No. 2021-BEPC-PT-005290). The authors would like to thank Siqi Liu from Shiyanjia Lab ( . - ISSN 1477-9226. - ISSN 1477-9234
   Перевод заглавия: Модуляция люминесценции Bi3+ от широкополосного зеленого до широкополосного темно-красного в Lu2WO6 с помощью легирования Gd3+ и его применение в белых светодиодах с высоким индексом цветопередачи и светодиодах ближнего инфракрасного диапазона
Аннотация: Phosphors that exhibit tunable broadband emissions are highly desired in multi-functional LEDs, including pc-WLEDs and pc-NIR LEDs. In this work, broadband emissions were obtained and modulated in the unexpectedly wide spectral range of 517–609 nm for (Lu0.99−xGdxBi0.01)2WO6 phosphors by tuning the Gd3+ content (x = 0–0.99). The effects of Gd3+ doping on phase constituents, particle morphology, crystal structure, and photoluminescence were systematically investigated. Broadband green emission was obtained from Gd3+-free (Lu0.99Bi0.01)2WO6 phosphors (x = 0), whose emission intensity was enhanced by 50% with 5 at% Gd3+ (x = 0.05). The phase transition happened when x 0.50 and the broadband red-NIR emission was obtained when x = 0.75–0.99. Three luminescence centers were proved to be responsible for the broadband green emissions via crystal structure, spectral fitting and fluorescence decay analysis. A pc-WLED with a high color rendering index (Ra = 91.3), a stable emission color, and a low color temperature (3951 K) was fabricated from the (Lu0.94Gd0.05Bi0.01)2WO6 broadband green phosphor, and an LED device that simultaneously emits high color rendering index white light and NIR light was obtained with the (Gd0.99Bi0.01)2WO6 broadband red-NIR phosphor. Night vision and noninvasive imaging were also demonstrated using the latter LED device.

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Держатели документа:
College of Chemistry and Materials Engineering, Bohai University, Jinzhou, Liaoning 121007, China
Research Center for Functional Materials, National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan
Laboratory of Crystal Physics, Kirensky Institute of Physics, FRC KSC SB RAS, Krasnoyarsk 660036, Russia
Research and Development Department, Kemerovo State University, Kemerovo 650000, Russia
Siberian Federal University, Krasnoyarsk 660041, Russia
Jilin Engineering Laboratory for Quantum Information Technology, Institute for Interdisciplinary Quantum Information Technology, Jilin Engineering Normal University, Changchun 130052, China

Доп.точки доступа:
Wang, Xuejiao; Feng, Xiaowen; Molokeev, M. S.; Молокеев, Максим Сергеевич; Zheng, Huiling; Wang, Qiushi; Xu, Chunyan; Li, Ji-Guang
}
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Zhandun, V. S.
Doping-induced changes in the electronic and magnetic properties of Mn- and Cr-based MAX phases / V. S. Zhandun, O. N. Draganyuk, N. G. Zamkova // V International Baltic Conference on Magnetism. IBCM : Book of abstracts. - 2023. - P. 17. - Cited References: 2. - РНФ № 23-22-10020

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS
Siberian Federal University

Доп.точки доступа:
Draganyuk, O. N.; Драганюк, Оксана Николаевна; Zamkova, N. G.; Замкова, Наталья Геннадьевна; Жандун, Вячеслав Сергеевич; International Baltic Conference on Magnetism(5 ; 2023 ; Aug. 20-24 ; Svetlogorsk, Russia); Балтийский федеральный университет им. И. Канта
}
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Temperature and doping dependent short range antifferomagnetic order and pseudogap formation in hole-doped cuprates / S. G. Ovchinnikov, V. I. Kuzmin, S. V. Nikolaev, M. A. Visotin // 8th International conference on supercondactivity and magnetism (ICSM2023) : abstract book. - 2023. - Ст. 159. - P. 248. - Cited References: 1

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Держатели документа:
Kirensky Institute of Physics, FRC KSC SB RAS

Доп.точки доступа:
Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Kuzmin, V. I.; Кузьмин, Валерий Ипполитович; Nikolaev, S. V.; Visotin, M. A.; Высотин, Максим Александрович; International Conference on Supercondactivity and Magnetism(8 ; 2023 ; May 4-11 ; Ölüdeniz-Fethiye, Turkey)
}
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    Structural and magnetic alteration of Cu2GaBO5 forced by Mn3+ doping / E. Moshkina, E. Eremin, D. Velikanov [et al.] // J. Alloy. Compd. - 2022. - Vol. 902. - Ст. 163822, DOI 10.1016/j.jallcom.2022.163822. - Cited References: 43. - The study was supported by the Russian Science Foundation (Grant No. 21-72-00130) . The specific heat measurements were supported by the subsidy allocated to Kazan Federal University for the state assignment in the sphere of scientific activities (Project No.Journal of Alloys and Compounds 902 (2022) 163822 0671-2020-0 050) . The magnetic measurements, powder X-ray and EDX data were obtained using the analytical equipment of Krasnoyarsk Regional Center of Research Equipment of Federal Research Center "Krasnoyarsk Science Center SB RAS". The X-ray single-crystal experiment was done using the equipment of the Research and Education Centre "Molecular Design and Environmentally Safe Technologies" at NSU. The authors acknowl-edge Prof. Rushana Eremina and Dr. Tatyana Gavrilova for the valu-able discussion of the obtained results . - ISSN 0925-8388. - ISSN 1873-4669
   Перевод заглавия: Структурная и магнитная перестройка Cu2GaBO5, вызванная допированием Mn3+

РУБ Chemistry, Physical + Materials Science, Multidisciplinary + Metallurgy & Metallurgical
Рубрики:
CRYSTAL-STRUCTURE
SUSCEPTIBILITY
Кл.слова (ненормированные):
Ludwigites -- Flux growth -- Magnetic susceptibility -- Spin glass state
Аннотация: To study the gradual change of the structure and the magnetic state of the ludwigite Cu2GaBO5 upon Mn3+ doping, single crystals of Cu2Ga1−xMnxBO5 (x = 0.55, 0.7, 0.8) with the size up to 3 × 3 × 10 mm3 were grown using the flux technique. The phase homogeneity and crystal structure of the obtained compounds were investigated by the powder and single crystal X-ray diffraction. All the samples possessed the monoclinic-distorted ludwigite structure with the P21/c space group. The study of the actual Cu/Ga/Mn composition by the EDX (energy-dispersive X-ray spectroscopy) technique revealed the lower Mn content in all the samples and the refined formulas were Cu2Ga0.47Mn0.53BO5, Cu1.92Ga0.5Mn0.58BO5 and Cu2Ga0.32Mn0.68BO5, respectively. Despite the high manganese content, the concentration transition (from Cu2GaBO5 to Cu2MnBO5) and change of the monoclinic angle did not occur, but strong Me-O octahedra distortions exceeding those both in the parent ludwigites Cu2GaBO5 and Cu2MnBO5 were found. The study of the thermodynamic and magnetic properties revealed the low-temperature magnetic phase transition inherited from the parent Cu2GaBO5 in all the samples. However, the nature and ordering type for the compounds with different Mn content were different: there was a complex transformation of the magnetic state from the partially ordered AFM (antiferromagnetically) in Cu2Ga0.47Mn0.53BO5, through the spin glass state, to the combined spin glass/ordered state in Cu2Ga0.32Mn0.68BO5 with the appearance of magnetic anisotropy. The evident dependence of Tc (phase transition temperature) on the magnetic field was found as well as its decrease at the nonzero magnetic field in the samples with x = 0.53 and 0.68.

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Держатели документа:
Kirensky Inst Phys, Krasnoyarsk 660036, Russia.
Siberian State Univ Sci & Technol, Krasnoyarsk 660037, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Far Eastern State Transport Univ, Dept Phys, Khabarovsk 680021, Russia.
Novosibirsk State Univ, Novosibirsk 630090, Russia.
Inst Geol & Mineral, Novosibirsk 630090, Russia.
Kazan Fed Univ, Inst Phys, Kazan 420008, Russia.
Russian Acad Sci, Fed Res Ctr, Krasnoyarsk Sci Ctr, Siberian Branch, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Moshkina, E. M.; Мошкина, Евгения Михайловна; Eremin, E. V.; Еремин, Евгений Владимирович; Velikanov, D. A.; Великанов, Дмитрий Анатольевич; Bovina, A. F.; Бовина, Ася Федоровна; Molokeev, M. S.; Молокеев, Максим Сергеевич; Seryotkin, Y.; Cherosov, M.; Batulin, R.; Nemtsev, I. V.; Немцев, Иван Васильевич; Bezmaternykh, L. N.; Безматерных, Леонард Николаевич; Russian Science FoundationRussian Science Foundation (RSF) [21-72-00130]; Kazan Federal University [0671-2020-0 050]
}
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    Анализ распределения меди в кристаллах LiNBO3:Cu с поверхностным легированием / Р. И. Анисимов, А. А. Колмаков, А. С. Темерева [и др.] // XI Международная конференция по фотонике и информационной оптике : сборник научных трудов. - Москва, 2022. - С. 451-452. - Библиогр.: . - ISBN 978-5-7262-2842-6
   Перевод заглавия: Analysis of copper distribution in LiNBO3:Cu crystals with surface doping
Рубрики:

Аннотация: Представлены результаты исследований распределения примеси по глубине в структурах, сформированных термической диффузией меди в пластинах X-среза ниобата лития.

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Держатели документа:
Томский государственный университет систем управления и радиоэлектроники
Институт физики им. Л.В. Киренского СО РАН
Сибирский федеральный университет

Доп.точки доступа:
Анисимов, Р. И.; Колмаков, А. А.; Темерева, А. С.; Шараева, А. Е.; Шандаров, С. М.; Тимофеев, Иван Владимирович; Timofeev, I. V.; Пятнов, Максим Владимирович; Pyatnov, M. V.; Международная конференция по фотонике и информационной оптике(11 ; 2022 ; 26-28 янв. ; Москва); Российская академия наук; Национальный исследовательский ядерный университет "МИФИ"
}
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    Influence of Jahn-Teller Cu2+ doping on the structural and magnetic properties of quasi-two-dimensional oxyborate (Ni,Cu)2MnBO5 / A. Kartashev, E. Eremin, E. Moshkina [et al.] // J. Magn. Magn. Mater. - 2022. - Vol. 545. - Ст. 168747, DOI 10.1016/j.jmmm.2021.168747. - Cited References: 23. - This study was carried out on the equipment of the Krasnoyarsk Regional Center for Collective Use, Krasnoyarsk Science Center, Siberian Branch of the Russian Academy of Sciences. This work was supported by the Russian Foundation for Basic Research, Government of the Krasnoyarsk Region, and Krasnoyarsk Regional Foundation for Support of Scientific and R&D Activities, project no. 20-42-240011 . - ISSN 0304-8853
   Перевод заглавия: Влияние ян-теллеровского легирования Cu2+ на структурные и магнитные свойства квазидвумерного оксибората (Ni,Cu)2MnBO5
Кл.слова (ненормированные):
Ferrimagnet -- Frustrated materials -- Low-dimensional system -- Ludwigites
Аннотация: Using the flux technique single crystals of (Ni,Cu)2MnBO5 were grown. The crystal structure of this compound belongs to the space group Pbam(55). There are no monoclinic distortions of the crystal structure. The analysis of the structural data shows that the content of copper ions in the crystal is lower than 10 percent. The magnetic ordering into the ferrimagnetic phase occurs at 75 K. The assessment of the exchange interactions shows that changes in the exchange interactions lead to increasing frustrations in the system which could result in a decrease in the temperature of magnetic ordering.

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Держатели документа:
Kirensky Institute of Physics, Krasnoyarsk Scientific Center, Siberian Branch, Russian Academy of Sciences, Krasnoyarsk, 660036, Russian Federation
Reshetnev Siberian State University of Science and Technology, Krasnoyarsk, 660037, Russian Federation

Доп.точки доступа:
Kartashev, A. V.; Карташев, Андрей Васильевич; Eremin, E. V.; Еремин, Евгений Владимирович; Moshkina, E. M.; Мошкина, Евгения Михайловна; Molokeev, M. S.; Молокеев, Максим Сергеевич; Sofronova, S. N.; Софронова, Светлана Николаевна
}
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    Coordination units of Mn2+ modulation toward tunable emission in zero-dimensional bromides for white light-emitting diodes / G. J. Zhou, J. L. Ding, X. X. Jiang [et al.] // J. Mater. Chem. C. - 2022. - Vol. 10, Is. 6. - P. 2095-2102, DOI 10.1039/d1tc05680h. - Cited References: 57. - The present work was supported by the Natural Science Foundation of China (21871167), the 1331 Project of Shanxi Province and the Postgraduate Innovation Project of Shanxi Normal University (2019XBY018), the Beijing Natural Science Foundation (No. 2214068) and funded by RFBR according to the research project no. 19-52-80003 . - ISSN 2050-7526. - ISSN 2050-7534
   Перевод заглавия: Модуляция координационных блоков с Mn2+ для управляемой люминесценции в нульмерных бромидах для белых светодиодов

РУБ Materials Science, Multidisciplinary + Physics, Applied
Рубрики:
HALIDE PEROVSKITE NANOCRYSTALS
RECENT PROGRESS
DOPING MN2+
Аннотация: Organic–inorganic metal halides have become a multifunctional platform for manipulating photoluminescence due to highly efficient and tunable emissions, especially for lead-free Mn2+-based halides. Herein, the zero-dimensional (0D) bromides of (C5H14N3)2MnBr4 and (CH6N3)2MnBr4 with different coordination environments were designed and synthesized by a solvent evaporation method. They exhibit green and red broadband emission peaks at 528 nm and 627 nm with high photoluminescence quantum yields of 86.83% and 61.91%, respectively, which are attributed to the d–d transition (4T1(G) → 6A1(S)) of [MnBr4]2− tetrahedral and [Mn3Br12]6− octahedral units. The cases emphasize the effect of organic ligands on the intrinsic emissions of Mn2+ ions, thereby revealing the luminescence mechanism of Mn2+ ions in 0D isolated structures through the Tanabe–Sugano (TS) energy diagram. Thanks to their bright and stable emissions, the fabricated white light-emitting diode (LED) based on (C5H14N3)2MnBr4 and (CH6N3)2MnBr4 provides an outstanding color rendering index (Ra) of 90.8 at a correlated color temperature (CCT) of 3709 K, along with the CIE chromaticity coordinates of (0.3985, 0.3979) and a luminous efficacy of 51.2 lm W−1. This work aims at clarifying the relationship between the coordination units of Mn2+ and tunable emissions, and in particular, proposes a new strategy to explore phosphors excited by blue light for white LEDs.

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Держатели документа:
Shanxi Normal Univ, Sch Chem & Mat Sci, Key Lab Magnet Mol & Magnet Informat Mat, Minist Educ, Taiyuan 030006, Peoples R China.
Chinese Acad Sci, China Tech Inst Phys & Chem, Beijing 100190, Peoples R China.
Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Lab Crystal Phys, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Dept Engn Phys & Radioelect, Krasnoyarsk 660041, Russia.
Kemerovo State Univ, Res & Dev Dept, Kemerovo 650000, Russia.
Beijng Technol & Business Univ, Dept Phys, Beijing 100048, Peoples R China.
Taiyuan Univ Technol, Coll Chem & Chem Engn, Key Lab Interface Sci & Engn Adv Mat, Minist Educ, Taiyuan 030024, Shanxi, Peoples R China.

Доп.точки доступа:
Zhou, Guojun; Ding, Jialiang; Jiang, Xingxing; Zhang, Jian; Molokeev, M. S.; Молокеев, Максим Сергеевич; Ren, Qiqiong; Zhou, Jun; Li, Shili; Zhang, Xian-Ming
}
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    Broad luminescence tuning in Mn2+-doped Rb2Zn3(P2O7)2 via doping level control based on multiple synergies / Q. Liu, P. Dang, G. Zhang [et al.] // CrystEngComm. - 2022. - Vol. 24, Is. 31. - P. 5622-5629, DOI 10.1039/d2ce00719c. - Cited References: 31. - We acknowledge the financial support from the National Natural Science Foundation of China (NSFC No. 51932009, 51720105015, 51929201, 52072349, and 52172166), Projects for the Science and Technology Development Plan of Jilin Province (20210402046GH), and the Natural Science Foundation of Zhejiang Province (LR22E020004) . - ISSN 1466-8033
   Перевод заглавия: Широкая перестройка люминесценции в Rb2Zn3(P2O7)2, легированном Mn2+, посредством управления уровнем легирования на основе множественного синергизма
Кл.слова (ненормированные):
Binary alloys -- Color -- Energy transfer -- High temperature applications -- Light emission -- Solid state reactions -- Centrosymmetric structures -- Crystallographic sites -- Doping levels -- Emission color -- Energy-transfer -- High temperature solid-state reaction -- Luminescence tuning -- Multi band -- Non-centrosymmetric -- Orange-red -- Phosphors
Аннотация: Here we constructed a series of novel non-centrosymmetric structure phosphors [Rb2Zn3(P2O7)2:Mn2+] by a high-temperature solid-state reaction. The multiband emission can be designed by Mn2+ preferentially occupying three types of crystallographic sites in Rb2Zn3(P2O7)2:Mn2+. The emission color could be continuously tuned from yellow-green to orange-red via multiple synergies among crystallographic site engineering, energy transfer, and Mn-Mn dimmers alone through the dopant concentration. These color-tunable phosphors have good thermal stability (I150 °C/I25 °C = 91%). The as-prepared pc-WLED has a low corresponding color temperature (CCT = 4820 K) and a high color rendering index (Ra = 90.4) with CIE color coordinates of (0.351, 0.358). These results show that emission-tunable Rb2Zn3(P2O7)2:xMn2+ phosphors are potential candidates for application in n-UV-based pc-WLED devices. This study offers a new insight for wide-range tuning of PL properties by using crystallographic site engineering through changing the doping level in Mn-activated phosphors.

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Держатели документа:
State Key Laboratory of Rare Earth Resource Utilization, Changchun Institute of Applied Chemistry, Chinese Academy of Science, Changchun, 130022, China
School of Applied Chemistry and Engineering, University of Science and Technology of China, Hefei, 230026, China
Faculty of Materials Science and Chemistry, China University of Geoscience, Wuhan, 430074, China
Zhejiang Institute, China University of Geosciences, Hangzhou, 311305, China
Laboratory of Crystal Physics, Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Department of Engineering Physics and Radioelectronics, Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Department of Physics, Far Eastern State Transport University, Khabarovsk, 680021, Russian Federation

Доп.точки доступа:
Liu, Q.; Dang, P.; Zhang, G.; Lian, H.; Li, G.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Cheng, Z.; Lin, J.
}
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10.

Draganyuk, O. N.
Effect of substitution of Mn and Ga atoms by Fe atom in the Mn2GaC MAX phase / O. N. Draganyuk, N. G. Zamkova, V. S. Zhandun // J. Magn. Magn. Mater. - 2022. - Vol. 563. - Ст. 169860, DOI 10.1016/j.jmmm.2022.169860. - Cited References: 40. - The reported study was funded by Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science to the research project № 20-42-240004: “The effect of the composition, pressure, and dimension on the magnetic, electronic, optical, and elastic properties of the magnetic M n+1 AX n (M = Cr, Mn; Fe, A = Al, Ga, Si, Ge, P, In; X = C, N; n = 1-3) MAX-phases”. The calculations were performed with the computer resources of “Complex modeling and data processing research installations of mega-class” SRC “Kurchatovsky Institute” ( http://ckp.urcki.ru ). The ternary phase diagrams for the calculation of formation enthalpies were taken from Materials Project ( https://materialsproject.org ) and OQMD ( https://oqmd.org/ ) databases . - ISSN 0304-8853
Кл.слова (ненормированные):
MAX phases -- First-principle calculations -- Doping -- Magnetic properties -- Ferromagnetism -- Monte-Carlo simulations
Аннотация: The magnetic properties of ordered and disordered MAX-phase Mn2-xFe2xGaC and Mn2Ga1-xFexC (x = 12.5, 25, and 50 at.%) have been studied within DFT-GGA. The investigation of phase stability of M2AX phases is performed by comparing the total energy of MAX phases to that of the set of competitive phases for calculation of the phase formation enthalpy. At the small concentration of Fe atoms (x = 12.5 %) compound remains stable. We have found that introducing Fe atom at A-site leads to the forming of ferromagnetic phase with large magnetic moments on magnetic atoms and magnetization. Through detailed group-theoretical analysis we have obtained that only ferromagnetic ordering is possible when Fe atom ordering over Ga sites. The study of exchange constants shows that the out-of-plane Fe-Mn exchange gives the main contribution in appearance of ferromagnetic phase. The temperature dependences of magnetization reveal the increase of Curie temperature in Mn2GaC with Fe atom incorporated into Ga-site.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Siberian Federal Univercity, Krasnoyarsk, Russian Federation

Доп.точки доступа:
Zamkova, N. G.; Замкова, Наталья Геннадьевна; Zhandun, V. S.; Жандун, Вячеслав Сергеевич; Драганюк, Оксана Николаевна
}
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11.

Magnetic ion substitution and peak effect in YBCO: the strange case of Y1–xGd xBa2Cu3O7–δ / D. M. Gokhfeld, S. V. Semenov, I. V. Nemtsev [et al.] // J. Supercond. Novel Magn. - 2022. - Vol. 35, Is. 10. - P. 2679-2687, DOI 10.1007/s10948-022-06317-2. - Cited References: 50. - This work was supported by the Russian Foundation for Basic Research and the Government of the Krasnoyarsk Territory, Krasnoyarsk Territorial Foundation for Support of Scientific and R&D Activities, project “Superconducting properties of YBCO incorporated by paramagnetic rare-earth elements” No. 20-42-240008 . - ISSN 1557-1939
Кл.слова (ненормированные):
Peak effect -- Bulk superconductors -- Critical current -- Pinning -- X-ray diffraction -- YBCO -- Doping -- Paramagnetic magnetization
Аннотация: We present the results of a study of the superconducting and paramagnetic properties of polycrystalline Y1–xGdxBa2Cu3O7–δ samples. The critical current density and critical temperature of YBCO were weakly decreased by the Gd doping. A peak effect, which is a nonmonotonic dependence of the critical current density on magnetic field, was detected for all samples. The peak position shifted to higher magnetic fields with increasing Gd content. This behavior is opposite to the shift of the peak effect observed for other YBCO compounds doped by magnetic ions. This unusual behavior is apparently related to the realized granular structure instead of the type of doping ion. A correlation between the peak position and the granule size was found in the investigated samples and other polycrystalline YBCO compounds.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Federal Research Center “Krasnoyarsk Science Center of the Siberian Branch of the Russian Academy of Sciences”, Krasnoyarsk, 660036, Russian Federation

Доп.точки доступа:
Gokhfeld, D. M.; Гохфельд, Денис Михайлович; Semenov, S. V.; Семёнов, Сергей Васильевич; Nemtsev, I. V.; Немцев, Иван Васильевич; Yakimov, I. S.; Balaev, D. A.; Балаев, Дмитрий Александрович
}
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12.

Triplet-triplet energy transfer from Bi3+to Sb3+in zero-dimensional indium hybrids via a B-site co-doping strategy toward white-light emission / Q. Ren, J. Zhang, M. S. Molokeev [et al.] // Inorg. Chem. Front. - 2022. - Vol. 9, Is. 22. - P. 5960-5968, DOI 10.1039/d2qi01631a. - Cited References: 60. - This work was supported by the Natural Science Foundation of Shanxi Province (No. 20210302124054), the National Natural Science Foundation of China (No. 21871167), the Science and Technology Innovation Project of Colleges and Universities in Shanxi Province (No. 2021L262), the 1331 Project of Shanxi Province and the Postgraduate Innovation Project of Shanxi Normal University (No. 2021XSY040), and funded by RFBR according to the research project No. 19-52-80003 . - ISSN 2052-1553
Кл.слова (ненормированные):
Co-doping -- Doping strategies -- Lightemitting diode -- Lone pair -- Low dimensional -- Photoluminescence properties -- Triplet-triplet energy transfer -- White light emission -- Widely tunable -- Zero-dimensional -- Metal halides
Аннотация: Low-dimensional metal halides have emerged as promising platforms for the development of new-generation phosphor-converted light emitting diodes (pc-LEDs), in which zero-dimensional (0D) hybrids with lone-pair ns2 states, in particular, show unprecedented competitiveness owing to their fascinating photoluminescence (PL) properties. Herein, we designed a novel 0D indium hybrid, (C20H20P)2InCl5, and proposed a co-doping strategy to incorporate Bi3+ (6s2) and Sb3+ (5s2) ions into this indium hybrid. Widely tunable emissions from blue to red are achieved, which are assigned to the triplet self-trapped excitons (STEs) (3P1 → 1S0) of Bi3+ (476 nm) and Sb3+ (658 nm), respectively. Importantly, an uncommon triplet–triplet energy transfer from Bi3+ to Sb3+ contributes to tunable dual emissions, and enables a single-phase cool white-light emission under ultraviolet (UV) excitation. Moreover, the energy transfer mechanism is discussed clearly by fluorescence photon dynamic analysis and DFT calculations. This work provides a deeper insight into triplet–triplet energy transfer, as well as presents a new model system for tuning the PL behaviours of ns2 configuration dopants.

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Держатели документа:
Key Laboratory of Magnetic Molecules and Magnetic Information Materials (Ministry of Education), School of Chemistry and Material Science, Shanxi Normal University, Taiyuan, 030031, China
Laboratory of Crystal Physics, Kirensky Institute of Physics, Federal Research Center Ksc Sb Ras, Krasnoyarsk, 660036, Russian Federation
Research and Development Department, Kemerovo State University, Kemerovo, 650000, Russian Federation
Department of Physics, Far Eastern State Transport University, Khabarovsk, 680021, Russian Federation
College of Chemistry & Chemical Engineering, Key Laboratory of Interface Science and Engineering in Advanced Material, Ministry of Education, Taiyuan University of Technology, Shanxi, Taiyuan, 030024, China

Доп.точки доступа:
Ren, Q.; Zhang, J.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Zhou, G.; Zhang, X. -M.
}
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13.

Interplay of magnetic and superconducting subsystems in Ho-doped YBCO / D. M. Gokhfeld, S. V. Semenov, K. Y. Terentyev [et al.] // J. Supercond. Nov. Magn. - 2021. - Vol. 34. Is. 10. - P. 2537-2543, DOI 10.1007/s10948-021-05954-3. - Cited References: 26. - This work was supported by the Russian Foundation for Basic Research and the Government of the Krasnoyarsk Territory, Krasnoyarsk Territorial Foundation for Support of Scientific and R&D Activities, project "Superconducting properties of YBCO incorporated by paramagnetic rare-earth elements" No. 20-42-240008 . - ISSN 1557-1939. - ISSN 1557-1947

РУБ Physics, Applied + Physics, Condensed Matter
Рубрики:
TEMPERATURE
   TRANSPORT
   PEAK
   DY
   SUSCEPTIBILITY
   TRANSITION
   BEHAVIOR
Кл.слова (ненормированные):
Peak effect -- Bulk superconductors -- Critical current -- Pinning -- X-ray diffraction -- YBCO -- Doping -- Paramagnetic magnetization
Аннотация: Superconducting and paramagnetic contributions to the magnetization of polycrystalline Y1−xHoxBa2Cu3O7−δ samples were investigated. The superconductivity is responsible for a partial screening of magnetic ions from an external magnetic field and for a possible sinking of antiferromagnetic correlations between these ions. Magnetic moments of Ho ions influence on a peak effect induced by the order–disorder transition of the Abrikosov vortex lattice. The critical current density and the critical temperature of YBCO are not changed by the Ho doping.

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Держатели документа:
Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.

Доп.точки доступа:
Gokhfeld, D. M.; Гохфельд, Денис Михайлович; Semenov, S. V.; Семёнов, Сергей Васильевич; Terentyev, K. Yu.; Терентьев, Константин Юрьевич; Yakimov, I. S.; Balaev, D. A.; Балаев, Дмитрий Александрович; Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR); Government of the Krasnoyarsk Territory, Krasnoyarsk Territorial Foundation for Support of Scientific and R&D Activities, project "Superconducting properties of YBCO incorporated by paramagnetic rare-earth elements" [20-42-240008]
}
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14.

Structural, optical, and electronic properties of Cu-doped TiNxOy grown by ammonothermal atomic layer deposition / F. A. Baron, Y. L. Mikhlin, M. S. Molokeev [et al.] // ACS Appl. Mater. Interfaces. - 2021. - Vol. 13, Is. 27. - P. 32531-32541, DOI 10.1021/acsami.1c08036. - Cited References: 69. - This research was funded by the RFBR, Krasnoyarsk Territory and Krasnoyarsk Regional Fund of Science (project code 20-42-240013) and by the grant of the Government of the Russian Federation for Creation of World Tier Laboratories (contract no. 075-15-2019-1886) . - ISSN 1944-8244. - ISSN 1944-8252

РУБ Nanoscience & Nanotechnology + Materials Science, Multidisciplinary
Рубрики:
OXYNITRIDE THIN-FILMS
TITANIUM-NITRIDE
CONFORMAL TIN
Кл.слова (ненормированные):
atomic layer deposition -- titanium oxynitride -- copper doping -- surface segregation -- thin film
Аннотация: Copper-doped titanium oxynitride (TiNxOy) thin films were grown by atomic layer deposition (ALD) using the TiCl4 precursor, NH3, and O2 at 420 °C. Forming gas was used to reduce the background oxygen concentration and to transfer the copper atoms in an ALD chamber prior to the growth initiation of Cu-doped TiNxOy. Such forming gas-mediated Cu-doping of TiNxOy films had a pronounced effect on their resistivity, which dropped from 484 ± 8 to 202 ± 4 μΩ cm, and also on the resistance temperature coefficient (TCR), which decreased from 1000 to 150 ppm °C–1. We explored physical mechanisms causing this reduction by performing comparative analysis of atomic force microscopy, X-ray photoemission spectroscopy, X-ray diffraction, optical spectra, low-temperature transport, and Hall measurement data for the samples grown with and without forming gas doping. The difference in the oxygen concentration between the films did not exceed 6%. Copper segregated to the TiNxOy surface where its concentration reached 0.72%, but its penetration depth was less than 10 nm. Pronounced effects of the copper doping by forming gas included the TiNxOy film crystallite average size decrease from 57–59 to 32–34 nm, considerably finer surface granularity, electron concentration increase from 2.2(3) × 1022 to 3.5(1) × 1022 cm–3, and the electron mobility improvement from 0.56(4) to 0.92(2) cm2 V–1 s–1. The DC resistivity versus temperature R(T) measurements from 4.2 to 300 K showed a Cu-induced phase transition from a disordered to semimetallic state. The resistivity of Cu-doped TiNxOy films decreased with the temperature increase at low temperatures and reached the minimum near T = 50 K revealing signatures of the quantum interference effects similar to 2D Cu thin films, and then, semimetallic behavior was observed at higher temperatures. In TiNxOy films grown without forming gas, the resistivity decreased with the temperature increase as R(T) = – 1.88T0.6 + 604 μΩ cm with no semimetallic behavior observed. The medium range resistivity and low TCR of Cu-doped TiNxOy make this material an attractive choice for improved matching resistors in RF analog circuits and Si complementary metal–oxide–semiconductor integrated circuits.

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Держатели документа:
KSC SB RAS, Inst Chem & Chem Technol, Fed Res Ctr, Krasnoyarsk 660036, Russia.
KSC SB RAS, Kirensky Inst Phys, Fed Res Ctr, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Reshetnev Siberian State Univ Sci & Technol, Krasnoyarsk 660037, Russia.

Доп.точки доступа:
Baron, F. A.; Барон, Филипп Алексеевич; Mikhlin, Yurii L.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Rautskiy, M. V.; Рауцкий, Михаил Владимирович; Tarasov, I. A.; Тарасов, Иван Анатольевич; Volochaev, M. N.; Волочаев, Михаил Николаевич; Shanidze, L. V.; Шанидзе, Лев Викторович; Lukyanenko, A. V.; Лукьяненко, Анна Витальевна; Smolyarova, T. E.; Смолярова, Татьяна Евгеньевна; Konovalov, Stepan O.; Zelenov, Fyodor, V; Tarasov, A. S.; Тарасов, Антон Сергеевич; Volkov, N. V.; Волков, Никита Валентинович; RFBR, Krasnoyarsk Territory and Krasnoyarsk Regional Fund of Science [20-42-240013]; Government of the Russian Federation for Creation of World Tier Laboratories [075-15-2019-1886]
}
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15.

    Li/Na substitution and Yb3+ co-doping enabling tunable near-infrared emission in LiIn2SbO6:Cr3+ phosphors for light-emitting diodes / G. Liu, T. Hu, M. S. Molokeev, Z. Xia // iScience. - 2021. - Vol. 24, Is. 4. - Ст. 102250, DOI 10.1016/j.isci.2021.102250. - Cited References: 45. - The present work was supported by the National Natural Science Foundation of China of China (Grant Nos. 51972118 and 51961145101), the Fundamental Research Funds for the Central Universities (D2190980), the Guangzhou Science & Technology Project (202007020005), the Local Innovative and Research Teams Project of Guangdong Pearl River Talents Pro-gram (2017BT01X137), and RFBR according to the research project No. 19-52-80003 . - ISSN 2589-0042
   Перевод заглавия: Замещение Li/Na и содопирование Yb3+, позволяющее настраивать излучение в ближней инфракрасной области в люминофорах LiIn2SbO6: Cr3+ для светоизлучающих диодов
Кл.слова (ненормированные):
Inorganic Chemistry -- Optical Materials -- Photonics
Аннотация: Near-infrared (NIR) phosphor-converted light-emitting diode (pc-LED) has great potential in non-invasive detection, while the discovery of tunable broadband NIR phosphor still remains a challenge. Here, we report that Cr3+-activated LiIn2SbO6 exhibits a broad emission band ranging from 780 to 1400 nm with a full width at half maximum (FWHM) of 225 nm upon 492 nm excitation. The emission peaks are tuned from 970 to 1020 nm together with considerable broadening of FWHM (∼285 nm) via Li/Na substitution. Depending on Yb3+ co-doping, a stronger NIR fluorescence peak of Yb3+ appears with improved thermal resistance, which is ascribed to efficient energy transfer from Cr3+ to Yb3+. An NIR pc-LED package has been finally designed and demonstrated a remarkable ability to penetrate pork tissues (∼2 cm) so that the insertion depth of a needle can be observed, indicating that the phosphor can be applied in non-destructive monitoring.

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Держатели документа:
State Key Laboratory of Luminescent Materials and Devices, Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques, Guangdong Engineering Technology Research and Development Center of Special Optical Fiber Materials and Devices, School of Materials Science and Engineering, South China University of Technology, Guangzhou, 510641, China
Laboratory of Crystal Physics, Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Research and Development Department, Kemerovo State University, Kemerovo, 650000, Russian Federation

Доп.точки доступа:
Liu, G.; Hu, T.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Xia, Z.
}
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16.

    Photoluminescence tuning in Ba3ScB3O9:Eu2+ phosphor by crystal-site engineering / S. Lai, T. Hu, M. S. Molokeev, Z. Xia // Phys. Open. - 2021. - Vol. 8. - Ст. 100077, DOI 10.1016/j.physo.2021.100077. - Cited References: 31. - The present work was supported by the National Natural Science Foundation of China (Grant Nos. 51972118 and 51961145101), International Cooperation Project of National Key Research and Development Program of China (2021YFE0105700), the Guangzhou Science & Technology Project (202007020005), and the Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program (2017BT01X137). This work is also funded by RFBR according to the research project No. 19-52-80003 . - ISSN 2666-0326
   Перевод заглавия: Управление люминесценцией в люминофоре Ba3ScB3O9: Eu2+ методом кристаллической инженерии
Кл.слова (ненормированные):
Phosphor -- Photoluminescence tuning -- Crystal-site engineering -- Doping
Аннотация: Controlled photoluminescence tuning is essential for optimizing and accelerating the application of phosphor materials. Here, we adopt the crystal-site engineering method to tailor the photoluminescence properties in Ba3ScB3O9:Eu2+. Ba3ScB3O9 host contains multiple cationic sites which help to finely regulate Eu2+ site occupancies and thus the emission color. The relationship between Eu2+ emission and the local environments has been analyzed, and we demonstrate that the emission colors of the phosphors can be widely tuned from NIR to yellow by chemically driving the Eu2+ from octahedrally-coordinated Sc3+ sites to nine-fold coordinated Ba2+ sites. Our study will initiate and guide more explorations on discovering new phosphors through crystal-site engineering.

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Держатели документа:
State Key Laboratory of Luminescent Materials and Devices and Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques, South China University of Technology, Guangzhou, 510641, China
Laboratory of Crystal Physics, Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Department of Physics, Far Eastern State Transport University, Khabarovsk, 680021, Russian Federation

Доп.точки доступа:
Lai, S.; Hu, T.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Xia, Z.
}
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17.

Magnetotransport effects and electronic phase separation in manganese sulfides with electron-hole doping / O. B. Romanova, S. S. Aplesnin, M. N. Sitnikov, L. V. Udod // J. Exp. Theor. Phys. - 2021. - Vol. 132, Is. 5. - P. 831-842, DOI 10.1134/S106377612103016X. - Cited References: 38. - This study was supported by the Russian Foundation for Basic Research and the Belarussian Republic Foundation for Basic Research (project no. 20-52-00005) . - ISSN 1063-7761. - ISSN 1090-6509

РУБ Physics, Multidisciplinary
Рубрики:
MAGNETIC-PROPERTIES
TRANSITION
MAGNETORESISTANCE
Аннотация: We analyze the effect of electron and hole doping with a low substituent concentration (x = 0.01) on the magnetic and electron subsystems in disordered semiconductors MexMn1-xS (Me = Ag and Tm) in a wide range of temperatures (77–1000 K) and magnetic fields up to 12 kOe. Using magnetic measurements, we have established the domains of ferron (polaron) formation in the vicinity of the magnetic phase transition. We have detected the magnetoimpedance and magnetoresistance, the magnitude and sign of which depend on the electric field, temperature, and the type of the substituent element. We have determined the temperatures of thermopower peaks associated with deformation of the crystalline structure. We have established the phonon and magnon contributions to charge carrier relaxation using the method of impedance spectroscopy and the Jahn–Teller mode of oscillations from the IR spectra for the system containing silver. We have determined the diffusion contribution to the conductivity from the impedance hodograph in TmxMn1-xS semiconductors. The experimental results are described using the models of supermagnetic clusters, ferroelectric domains, and the Debye model.

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Публикация на русском языке Магнитотранспортные эффекты и электронное фазовое расслоение в сульфидах марганца с электронно-дырочным допированием [Текст] / О. Б. Романова, С. С. Аплеснин, М. Н. Ситников, Л. В. Удод // Журн. эксперим. и теор. физ. - 2021. - Т. 159 Вып. 5. - С. 938-951

Держатели документа:
Russian Acad Sci, Siberian Branch, Kirensky Inst Phys, Krasnoyarsk 660036, Russia.
Reshetnev Siberian State Univ Sci & Technol, Krasnoyarsk 660037, Russia.

Доп.точки доступа:
Romanova, O. B.; Романова, Оксана Борисовна; Aplesnin, S. S.; Аплеснин, Сергей Степанович; Sitnikov, M. N.; Udod, L. V.; Удод, Любовь Викторовна; Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR); Belarussian Republic Foundation for Basic Research [20-52-00005]
}
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18.

    Liu, Ying.
    Lattice doping of lanthanide ions in Cs2AgInCl6 nanocrystals enabling tunable photoluminescence / Y. Liu, M. S. Molokeev, Zh. Xia // Energy Mater. Adv. - 2021. - Vol. 2021. - Ст. 2585274, DOI 10.34133/2021/2585274. - Cited References: 42. - This work was supported by the National Natural Science Foundation of China (grant numbers 51961145101 and 51972118), the Fundamental Research Funds for the Central Universities (grant number FRFTP-18-002C1), the Guangzhou Science & Technology Project (202007020005), and the Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program (grant number 2017BT01X137). This work was also funded by RFBR according to the research project no. 19-52-80003 . - ISSN 2692-7640
   Перевод заглавия: Решеточное легирование ионами лантаноидов в нанокристаллах Cs2AgInCl6, обеспечивающее перестраиваемую фотолюминесценцию
Аннотация: Lead-free halide double perovskite Cs2AgInCl6 has become the research hotspot in the optoelectronic fields. It is a challenge to utilize the lattice doping by different lanthanide ions with rich and unique photoluminescence (PL) emissions for emerging photonic applications. Here, we successfully incorporated Dy3+, Sm3+, and Tb3+ ions into Cs2AgInCl6 nanocrystals (NCs) by the hot-injection method, bringing diverse PL emissions of yellowish, orange, and green light in Cs2AgInCl6:Ln3+ (Ln3+ = Dy3+, Sm3+, Tb3+). Moreover, benefiting from the energy transfer process, Sm3+ and Tb3+ ion-codoped Cs2AgInCl6 NCs achieved tunable emission from green to yellow orange and a fluorescent pattern from the as-prepared NC-hexane inks by spray coating was made to show its potential application in fluorescent signs and anticounterfeiting technology. This work indicates that lanthanide ions could endow Cs2AgInCl6 NCs the unique and tunable PL properties and stimulate the development of lead-free halide perovskite materials for new optoelectronic applications.

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The Beijing Municipal Key Laboratory of New Energy Materials and Technologies, School of Materials Science and Engineering, University of Science and Technology, Beijing, China
Laboratory of Crystal Physics, Kirensky Institute of Physics, Federal Research Center KSC SB RASs, Russia
Department of Engineering Physics and Radioelectronics, Siberian Federal University, Russia
Department of Physics, Far Eastern State Transport University, Russia
The State Key Laboratory of Luminescent Materials and Devices, Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques, School of Materials Science and Engineering, South China University of Technology, China

Доп.точки доступа:
Molokeev, M. S.; Молокеев, Максим Сергеевич; Xia, Zhiguo
}
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19.

Romanova, O. B.
Effect of electron and hole doping on the transport characteristics of chalcogenide systems / O. B. Romanova, S. S. Aplesnin, L. V. Udod // Phys. Solid State. - 2021. - Vol. 63, Is. 5. - P. 754-757, DOI 10.1134/S1063783421050152. - Cited References: 21. - This study was supported by the Russian Foundation for Basic Research and the Belarusian Republican Foundation for Basic Research, project no. 20-52-00005 . - ISSN 1063-7834. - ISSN 1090-6460

РУБ Physics, Condensed Matter
Рубрики:
MAGNETIC-PROPERTIES
TRANSITION
Кл.слова (ненормированные):
semiconductors -- conductivity -- Hall constant -- mobility
Аннотация: The electrical properties of the Ag0.01Mn0.99S and Tm0.01Mn0.99S semiconductor compounds and the Hall effect in them have been investigated in the temperature range of 80-400 K in a magnetic field of 12 kOe. Using the I-V characteristics, the conductivity mechanism depending on the doping type and concentration has been established. Upon substitution of silver for manganese, the Mott-type conductivity has been found, while substitution of thulium causes the ohmic conductivity. The mobility and type of carriers have been determined from the Hall constant data.

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Публикация на русском языке Романова, Оксана Борисовна. Влияние электронного и дырочного допирования на транспортные характеристики халькогенидных систем [Текст] / О. Б. Романова, С. С. Аплеснин, Л. В. Удод // Физ. тверд. тела. - 2021. - Т. 63 Вып. 5. - С. 606-609

Держатели документа:
Russian Acad Sci, Krasnoyarsk Sci Ctr, Kirensky Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia.
Siberian State Univ Sci & Technol, Krasnoyarsk 660014, Russia.

Доп.точки доступа:
Aplesnin, S. S.; Аплеснин, Сергей Степанович; Udod, L. V.; Удод, Любовь Викторовна; Романова, Оксана Борисовна; Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR); Belarusian Republican Foundation for Basic Research [20-52-00005]
}
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20.

    Eu2+Doping concentration-induced site-selective occupation and photoluminescence tuning in KSrScSi2O7:Eu2+ phosphor / S. Lai, M. Zhao, Y. Zhao [et al.] // ACS. Mater. Au. - 2021. - Vol. 2, Is. 3. - P. 374-380, DOI 10.1021/acsmaterialsau.1c00081. - Cited References: 43. - This work was supported by the International Cooperation Project of National Key Research and Development Program of China (2021YFE0105700), the National Natural Science Foundations of China (Grant Nos. 51972118 and 51961145101), the Guangzhou Science & Technology Project (202007020005), the Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program (2017BT01X137), and the China Postdoctoral Science Foundation (2021M700298). This work was also funded by RFBR according to research project No. 19-52-80003 . - ISSN 2694-2461
   Перевод заглавия: Сайт-селективное заселение и настройка фотолюминесценции в люминофоре KSrScSi2O7:Eu2+, индуцированное Eu2+ допированием
Кл.слова (ненормированные):
photoluminescence -- silicates -- crystal-site engineering -- doping -- light-emitting diodes
Аннотация: Regulation of Eu2+ dopants in different cation sites of solid-state materials is of great significance for designing multicolor phosphors for light-emitting diodes (LEDs). Herein, we report the selective occupation of Eu2+ for multiple cationic sites in KSrScSi2O7, and the tunable photoluminescence from blue to cyan is realized through Eu2+ doping concentration-dependent crystal-site engineering. Eu2+ preferably occupies the K and Sr sites in KSrScSi2O7 at a low doping concentration, resulting in a 440 nm blue emission. As the Eu2+ concentration increases, a new Eu2+ substitution pathway is triggered, that is, Eu2+ enters the Sc site, leading to the red-shifted emission spectra from 440 to 485 nm. The doping mechanism and photoluminescence properties are corroborated by structural analysis, optical spectroscopy study, and density functional theory calculations. The optical properties of the as-fabricated white LEDs are studied, which demonstrates that these phosphors can be applied to full-spectrum phosphor-converted LEDs. This study provides a new design strategy to guide the development of multicolor Eu2+-doped oxide phosphors for lighting applications.

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State Key Laboratory of Luminescent Materials and Devices, Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques, School of Materials Science and Engineering, South China University of Technology, Guangzhou, 510641, China
Institute of Information Photonics Technology, Faculty of Science, Beijing University of Technology, Beijing, 100124, China
Department of Chemistry, City University of Hong Kong, Hong Kong, Kowloon, 999077, Hong Kong
Laboratory of Crystal Physics, Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Research and Development Department, Kemerovo State University, Kemerovo, 650000, Russian Federation
Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Department of Physics, Far Eastern State Transport University, Khabarovsk, 680021, Russian Federation

Доп.точки доступа:
Lai, S.; Zhao, M.; Zhao, Y.; Molokeev, M. S.; Молокеев, Максим Сергеевич; Xia, Z.
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