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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Peng J. L., Bulcock S., Belobrov P. I., Bursill L. A.
Заглавие : Surface bonding states of nano-crystalline diamond balls
Место публикации : Int. J. Mod. Phys. B: WORLD SCIENTIFIC PUBL CO PTE LTD, 2001. - Vol. 15, Is. 31. - P4071-4085. - ISSN 0217-9792, DOI 10.1142/S0217979201007865
Примечания : Cited References: 20
Предметные рубрики: PLASMON RESPONSE
POWDER
SPECTROSCOPY
MICROSCOPY
SILICON
SI(111)
Ключевые слова (''Своб.индексиров.''): diamond--article--crystal structure--electron--energy transfer--nanoparticle--particulate matter--structure analysis--surface property--transmission electron microscopy
Аннотация: The rough surface of nano-crystalline diamond spheres induces surface electronic states which appear as a broadened pre-peak over approx. 15 eV at the C K-edge energy threshold for carbon in the parallel electron energy loss spectrum (PEELS). This appears to be at least partially due to 1s-pi* transitions, although typically the latter occupy a range of only 4 eV for the sp(2) edge of highly-oriented pyrollytic graphite (HOPG). No pi* electrons appear in the conduction band inside the diamond particles, where all electrons are sp(3) hybridized. PEELS data were also obtained from a chemical vapour deposited diamond film (CVDF) and gem-quality diamond for comparison with the spectra of nano-diamonds. The density of sp(2) and sp(3) states on the surface of diamond nano-crystals is calculated for simple structural models of the diamond balls, including some conjecture about surface structures. The results are used to interpret the sp(2)/sp(3) ratios measured from the PEELS spectra recorded as scans across the particles. Surface roughness at the atomic scale was also examined using high-resolution transmission electron microscopy (HRTEM) and electron nano-diffraction patterns were used to confirm the crystal structures.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Markel V. A., Pustovit V. N., Karpov S. V., Obuschenko A. V., Gerasimov V. S., Isaev I. L.
Заглавие : Electromagnetic density of states and absorption of radiation by aggregates of nanospheres with multipole interactions
Место публикации : Phys. Rev. B: AMER PHYSICAL SOC, 2004. - Vol. 70, Is. 5. - Ст.54202. - ISSN 1098-0121, DOI 10.1103/PhysRevB.70.054202
Примечания : Cited References: 81
Предметные рубрики: DISCRETE-DIPOLE APPROXIMATION
ENHANCED RAMAN-SCATTERING
METAL FRACTAL CLUSTERS
OPTICAL-PROPERTIES
SELECTIVE PHOTOMODIFICATION
DISORDERED CLUSTERS
NUMERICAL-SIMULATION
SPECTRAL DEPENDENCE
PARTICULATE MATTER
LIGHT-SCATTERING
Ключевые слова (''Своб.индексиров.''): carbon--iron--palladium--silver--article--dipole--electromagnetic field--geometry--mathematical analysis--molecular interaction--nanoparticle--radiation absorption
Аннотация: We calculate the quasistatic electromagnetic density of states for aggregates of touching spheres, in particular, linear chains and computer-generated random fractal aggregates. Multipole moments with orders of up to L=64 are taken into account for random aggregates with the number of particles of up to N=100 and up to L=8000 for linear chains. Extensive comparisons with the dipole approximation and geometrical cluster renormalization method are performed. Extinction spectra are calculated for several metals and black carbon. Long wavelength electromagnetic properties of fractal aggregates are considered in details.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Vasilyeva I. G., Dovlitova L. S., Zaikovskii V. I., Malakhov V. V., Edel'man I. S., Stepanov A. S., Aleksandrov K. S.
Заглавие : Actual composition and structure of manganese ferrite nanoparticles dispersed in the borate glass matrix
Место публикации : Doklady Chemistry. - 2005. - Vol. 401, Is. 1-3. - P.47-50. - ISSN 0012-5008, DOI 10.1007/s10631-005-0029-y
Ключевые слова (''Своб.индексиров.''): boric acid--ferrite--glass--manganese derivative--analytic method--article--chemical composition--chemical structure--nanoparticle--stoichiometry--structure analysis--transmission electron microscopy--x ray analysis
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kliava J., Malakhovskii A. V., Edelman I. S., Potseluyko A. M., Petrakovskaja E. A., Melnikova S.V., Zarubina T. V., Petrovskii G., Bruckental Y., Yeshurun Y.
Заглавие : Unusual magnetic transitions and nature of magnetic resonance spectra in oxide glasses containing gadolinium
Место публикации : Phys. Rev. B: AMER PHYSICAL SOC, 2005. - Vol. 71, Is. 10. - Ст.104406. - ISSN 1098-0121, DOI 10.1103/PhysRevB.71.104406
Примечания : Cited References: 40
Предметные рубрики: ELECTRON-PARAMAGNETIC-RESONANCE
BORATE GLASSES
IONS
BEHAVIOR
GD3+
SPECTROSCOPY
SYSTEMS
GD-3+
FIELD
SHAPE
Ключевые слова (''Своб.индексиров.''): gadolinium--glass--lanthanide--oxide--anisotropy--article--chemical structure--concentration response--electron spin resonance--energy--magnetism--molecular physics--nanoparticle--phase transition--refraction index--temperature sensitivity
Аннотация: Magnetic susceptibility, electron paramagnetic resonance (EPR), and optical properties have been studied in a glass system {20La(2)O(3)-22Al(2)O(3)-23B(2)O(3)-35(SiO2+GeO2)} with a part of La2O3 substituted by Gd2O3 in different concentrations. Positive Weiss constants have been found in the more heavily doped glasses and ascribed to clustering of Gd3+ ions. Two magnetic phase transitions at 55 and 12 K were detected and ascribed, respectively, to ferromagnetic and antiferromagnetic clusters containing Gd ions. The overall shape of the EPR spectra shows the presence of clustering at the higher Gd contents. At low temperatures the cluster-related resonance signal is altered in shape, indicating an onset of magnetic anisotropy field. This signal is convincingly fitted to superparamagnetic resonance arising from ferromagnetic nanoparticles. The clustering, depending on the Gd concentration, correlates with a significant shift to lower energies of the strong optical absorption band edge, ascribed to a charge transfer transition between Gd ions. A nonmonotonous change of refractive index with the increase of the Gd content indicates changes in the glass matrix and in Gd cluster structure.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Gavrilyuk A. P., Karpov S. V.
Заглавие : The model of resonant domain of metal nanoparticle aggregates in pulsed laser fields
Коллективы : ICONO 2007: Novel Photonics Materials; Optics and Optical Diagnostics of Nanostructures
Место публикации : Proceedings of SPIE - The International Society for Optical Engineering/ sponsors: SPIE Russia Chapter, National Academy of Sciences, Belarus, Russian Academy of Sciences, Belarus Foundation for Basic Research, Russian Physical Society ; ICONO 2007: Novel Photonics Materials; Optics and Optical Diagnostics of Nanostructures (2007 ; 28.05 - 01.06 ; Минск): S P I E - International Society for Optical Engineering, 2007. - 6728. - С. 67281T. - ISBN 0819468851, DOI 10.1117/12.752386 (Шифр 15048789)
ГРНТИ : 31.15
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gavrilyuk A.P., Karpov S.V.
Заглавие : Processes in Resonant Domains of Metal Nanoparticle Aggregates and Optical Nonlinearity of Aggregates in Pulsed Laser Fields
Место публикации : arXiv: Cornell University, 2008. - Ст.0808.2355
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gavrilyuk A. P., Karpov S. V.
Заглавие : Processes in resonant domains of metal nanoparticle aggregates and optical nonlinearity of aggregates in pulsed laser fields
Место публикации : Appl. Phys. B-Lasers Opt. - NEW YORK: SPRINGER, 2009. - Vol. 97, Is. 1. - С. 163-173. - SEP. - ISSN 0946-2171, DOI 10.1007/s00340-009-3592-y
Примечания : Cited Reference Count: 43. - Гранты: Authors are thankful to Prof. V. A. Markel ( University of Pennsylvania) for computation of multipole polarizability of silver nanoparticle bispheres, for the attention to this paper, fruitful discussions and great support. This research was supported by grants: 27.1 of the Presidium of RAS, 9.1 DPS RAS, 5 SB RAS, 3818.2008.3 and 6612.2006.3 of the President of RF ( SS RAS), DSP 2.1.1.1814, 05- 03- 32642 RFBR.Финансирующая организация: [27.1 of the Presidium of RAS]; [9.1 DPS RAS]; [5 SB RAS]; [3818.2008.3]; [6612.2006.3]
Предметные рубрики: SMALL-PARTICLE COMPOSITES
FRACTAL CLUSTERS
SELECTIVE PHOTOMODIFICATION
ABSORPTION-COEFFICIENTS
REFRACTIVE-INDEXES
SILVER
ENHANCEMENT
RESPONSES
GOLD
Ключевые слова (''Своб.индексиров.''): metal nanoparticles--nanosecond pulsed laser--nonlinear refractive index--optical nonlinearity--physical effects--pulsed-laser field--resonant domain--silver nanoparticles--simple physical models--aggregates--laser excitation--nanoparticles--nonlinear optics--organic polymers--pulsed laser applications--refractive index--silver
Аннотация: Optical nonlinearities in aggregates of nanoparticles formed in silver hydrosols (SHs) are studied under pico- and nanosecond pulsed laser excitation. The dependence of the nonlinear refractive index n (2) on the degree of hydrosol aggregation is studied experimentally at the wavelength lambda=1.064 mu m. It is found that n (2) changes sign when the degree of hydrosol aggregation is increased. Various physical effects occurring in resonant domains of the aggregates are analyzed using a simple physical model of two bound silver nanoparticles. The theory takes into account thermal, elastic, electrostatic, and light-induced effects. Experimental results are discussed in the context of this theory.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Gavrilyuk A.P., Karpov. S.V.
Заглавие : Dynamic changes of optical characteristics of resonant domains in metal nanoparticle aggregates under pulsed laser fields
Коллективы : International Conference on Coherent and Nonlinear Optics, International Conference on Lasers, Applications, and Technologies
Место публикации : Technical digest International conference ICONO/LAT 2010. - Казань, 2010. - Ст.ITuQ39
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gavrilyuk A.P., Karpov S.V.
Заглавие : Dynamic Changes of Optical Characteristics of Resonant Domains in Metal Nanoparticle Aggregates under Pulsed Laser Fields
Место публикации : Applied Physics B: Lasers and Optics. - 2010. - Vol. 101. - С. 512
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10.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Edelman. I., Ivanova O., Ivantsov R., Velikanov D., Zubavichus Y., Veligzhanin A., Curely J.
Заглавие : Magnetic properties and morphology of ferrite nanoparticle dispersed in glass
Коллективы : Moscow International Symposium on Magnetism
Место публикации : Moscow Int. Symp. on Magnet. (MISM-2011): Book of abstracts. - 2011. - Ст.23OR-B-9. - P.281-282
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11.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Edelman I. S., Ivanova O. S., Ivantsov R. D., Petrakovskaja E. A., Zabluda V. N., Hennet L., Thiaudiere D., Saboungi M. -L., Stepanov S., Artemenko A., Kliava J.
Заглавие : Nanoparticle-containing oxide glasses: transparent magnets
Коллективы : International Conference on the Chemistry of Glasses and Glass-Forming Melts, Society of Glass Techology
Место публикации : Int. Conf. on the Chem. of Glas. and Glass-Form. Melts: In celebration of the 300th Annuversary of the birth of Mikhail Vasilievich Lomonosov, 4-8 Sept., 2011 : abstracts. - 2011. - P.13
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12.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Edelman I. S., Ivanova O. S., Ivantsov R. D.
Заглавие : Magnetooptical Studies of Nanoparticle-Containing Borate Glasses
Коллективы : Euro-Asian Symposium "Trends in MAGnetism", "Trends in MAGnetism", Euro-Asian Symposium
Место публикации : Solid State Phenomena. - 2011. - Vol. 168-169. - P.525-528. - ISBN 1012-0394, DOI 10.4028/www.scientific.net/SSP.168-169.525
Примечания : Cited Reference Count: 9
Предметные рубрики: Materials Science, Multidisciplinary
Physics, Condensed Matter
Ключевые слова (''Своб.индексиров.''): magnetic nanoparticles--oxide glasses--faraday rotation--magnetic circular dichroism
Аннотация: Faraday rotation (FR) and magnetic circular dichroism (MCD) of nanocomposite structures based on potassium-aluminum-germanium-boron glasses co-doped with Fe and rare earth (RE) or Y+Bi oxides have been studied. Formation of magnetic nanoparticles as a result of the glass heat treatment ensures them magnetic and magneto-optical properties typical of magnetically ordered substances. At the same time, glasses keep transparence in visual spectral range owing to low paramagnetic oxides concentration. FR and MCD spectra of the heat treated glasses are shown to be very close to those of gamma-Fe(2)O(3) and practically independent of the RE element nature for the light wave energies lower than 22000 cm(-1). For higher energies, the MCD spectrum shape depends strongly an RE what evidences the different origin of magneto-optical effects in two spectral ranges.
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13.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Buktiyarova G.A., Shuvaeva М.А., Bayukov O. A., Yakushkin S.S., Martyanov O.N.
Заглавие : Facile synthesis of nanosized е-РегОз particles on the silica support
Место публикации : J. Nanopart. Res. - 2011. - Vol. 13, Is. 10. - Ст.5527-5534. - DOI 10.1007/sl 1051-011-0542-5
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14.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kliava J., Edelman I., Ivanova O., Ivantsov R., Petrakovskaja E. A., Hennet L., Thiaudire D., Saboungi M. L.
Заглавие : Electron magnetic resonance and magnetooptical studies of nanoparticle-containing borate glasses
Место публикации : Journal of Magnetism and Magnetic Materials. - 2011. - Vol. 323, Is. 5. - P.451-460. - ISSN 0304-8853, DOI 10.1016/j.jmmm.2010.09.045
Примечания : Cited Reference Count: 40. - RFBRRussian Foundation for Basic Research (RFBR) [07-02-92174]; CNRSCentre National de la Recherche Scientifique (CNRS)European Commission [07-02-92174]; Russian Federal Program [FCP NK-209P/GK P1227], This work was supported in part by RFBR-CNRS joint project, Grant no. 07-02-92174 and by the Russian Federal Program, project FCP NK-209P/GK P1227. It is a pleasure to thank I. Bruckental and Y. Yeshurun for the magnetization measurements.
ГРНТИ : 29.19
Ключевые слова (''Своб.индексиров.''): borate glasses--electron magnetic resonance--magnetic nanoparticles--magnetooptics
Аннотация: We report electron magnetic resonance (EMR) and magnetooptical studies of borate glasses of molar composition 22.5K2O22.5Al2O 355B2O3 co-doped with low concentrations of Fe2O3
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15.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Mankov Yu.I., Khlebopros R. G.
Заглавие : Effect of the shape of an antiferromagnetic nanoparticle on its magnetization
Место публикации : Tech. Phys.: MAIK Nauka-Interperiodica / Springer, 2012. - Vol. 57, Is. 5. - P.733-734. - ISSN 1063-7842, DOI 10.1134/S1063784212050209
Примечания : Cited References: 21
Предметные рубрики: DES GRAINS FINS
Аннотация: The dependence of the magnetization of an antiferromagnetic nanoparticle on its shape is studied in terms of a core-shell model. The magnetizations of a nanodisk, nanowire, and spherical particle are shown to differ several fold.
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16.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ershov A. E., Isaev I. L., Semina P. N., Markel V. A., Karpov S. V.
Заглавие : Effects of size polydispersity on the extinction spectra of colloidal nanoparticle aggregates
Место публикации : Phys. Rev. B: American Physical Society, 2012. - Vol. 85, Is. 4. - Ст.045421. - P. - ISSN 1098-0121, DOI 10.1103/PhysRevB.85.045421
Примечания : Cited References: 41. - This work was supported by grants from the following foundations of the Russian Federation: Presidium of RAS, OFN RAS, and SB RAS.
Предметные рубрики: METAL FRACTAL CLUSTERS
OPTICAL-PROPERTIES
ABSORPTION
NONLINEARITIES
COMPOSITES
SCATTERING
PARTICLES
SPHERES
GRAINS
Аннотация: We investigate the effect of particle polydispersity on the optical extinction spectra of colloidal aggregates of spherical metallic (silver) nanoparticles, taking into account the realistic interparticle gaps caused by layers of stabilizing polymer adsorbed on the metal surface (adlayers). The spectra of computer-generated aggregates are computed using two different methods. The coupled-multipole method is used in the quasistatic approximation and the coupled-dipole method beyond the quasistatics. The latter approach is applicable if the interparticle gaps are sufficiently wide relative to the particle radii. Simulations are performed for two different particle size distribution functions (bimodal and Gaussian), varying the number of particles per aggregate, and different distribution functions of the interparticle gap width. The strong influence of the latter factor on the spectra is demonstrated and investigated in detail.
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17.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Edelman I. S., Ivanova O., Ivantsov R. D., Petrakovskaja E. A., Velikanov D. A., Zabluda V. N., Hennet L., Thiaudiere D., Saboungi M. L., Zubavichus Y., Stepanov S., Zaikovskii V. I., Artemenko A., Kliava J.
Заглавие : Nanoparticle-containing glasses co-doped with transition and rare earth elements: comparative studies of transparent magnets
Коллективы : International Conference on the Chemistry of Glasses and Glass-Forming Melts (2011 ; Sept.; Oxford, England)
Место публикации : Phys. Chem. Glasses - Eur. J. Glass Sci. Technol. Part B: Society of Glass Technology, 2012. - Vol. 53, Is. 2. - P.37-44. - ISSN 1753-3562
Примечания : Cited References: 22
Предметные рубрики: ANISOTROPY
RESONANCE
FERRITE
Аннотация: A comparative multitechnique study (including transmission electron microscopy, synchrotron radiation, static magnetisation, magnetic circular dichroism and electron magnetic resonance) has been carried out of nanoparticle-containing borate glasses of two different types: (i) with iron and manganese oxide additives and (ii) with iron and rare earth oxide additives. Due to the presence of magnetic nanoparticles, these glasses have a nonlinear magnetic field dependence of magnetization with hysteresis and saturation while remaining transparent in the visible and near-infrared spectral ranges. The nature of the nanoparticles has been identified as manganese ferrite for type (i) glasses and maghemite for type (ii) glasses. The synchrotron radiation studies as well as the computer-assisted electron magnetic resonance provide an insight into the morphological characteristics of the magnetic nanoparticles in the glass.
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18.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Churilov G. N., Osipova I. V., Vnukova N. G., Glushchenko G. A., Petrakovskaya E. A., Kolonenko A. L., Chiganov A. S., Tomashevich Y. V., Zhyzhaev A. M.
Заглавие : Processing of detonation diamonds with metal-containing high-frequency arc plasma and their properties
Место публикации : Fuller. Nanotub. Carbon Nanostruct.: Taylor & Francis, 2012. - Vol. 20, Is. 4/7 SI. - P.611-615. - ISSN 1536-383X, DOI 10.1080/1536383X.2012.657014
Примечания : Cited References: 5. - The work was partially supported by RFBR foundation (project 09-03-00383).
Ключевые слова (''Своб.индексиров.''): nanodiamond--nanoparticle--metal-containing plasma
Аннотация: This paper describes coating of diamond powder with metal by plasma. Arc plasma was generated in double jet high-frequency argon-operated plasmatron with atomized metal inserts. The diamond powder was added to the plasma in a flow of helium. Copper and nickel coated particles of detonation and industrial diamonds were studied by XRD, XPS, SEM methods and electron magnetic resonance. Results of these studies are presented.
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19.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Lyubutin I. S., Starchikov S. S., Lin Chun-Rong, Lu Shin-Zong, Shaikh M. O., Funtov K. O., Dmitrieva T. V., Ovchinnikov S. G., Edelman I. S., Ivantsov R. D.
Заглавие : Magnetic, structural, and electronic properties of iron sulfide Fe3S4 nanoparticles synthesized by the polyol mediated process
Место публикации : J. Nanopart. Res.: Springer, 2013. - Vol. 15. - P.1397. - DOI 10.1007/s11051-012-1397-0
Аннотация: Iron sulfide nanoparticles Fe3S4 with the spinel-type crystal structure were synthesized by the polyol mediated process. The particle size depends on preparation conditions and varies from 9 to 20 nm. Mössbauer data have revealed that the dominating fraction of iron ions in the 9-nm sample is in the high-spin ferric state. This implies an occurrence of the cation vacancies in nonstoichiometric greigite. The stoichiometric phase of greigite Fe3S4 dominates in the 18-nm-size nanoparticles. Magnetic measurements have shown a ferrimagnetic behavior of all samples at temperatures between 78 and 300 K. The estimated value of magnetic moment of the stoichiometric greigite nanoparticles is about 3.5 μB per Fe3S4 unit. The Mössbauer spectra indicate a superparamagnetic behavior of small particles, and some fraction of superparamagnetic phase is observed in all samples synthesized which may be caused by the particle size distribution. The blocking temperatures of T B ≈ 230 and 250 K are estimated for the 9 and 14 nm particles, respectively. The Mössbauer parameters indicate a great degree of covalency in the Fe–S bonds and support the fast electron Fe3+ ⇆ Fe2+ exchange in the B-sites of greigite. An absence of the Verwey transition at temperatures between 90 and 295 K is established supporting a semimetal type of conductivity. The temperature and magnetic field dependences of the magnetic circular dichroism (MCD) of optical spectra were measured in Fe3S4 for the first time. The spectra differ substantially from that of the isostructural oxide Fe3O4. It is supposed that the MCD spectra of greigite nanoparticles result from the collective electron excitations in a wide band with superimposed peaks of the d–d transitions in Fe ions.
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20.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Stolyar S. V., Bayukov O. A., Ladygina V. P., Ischenko L. A., Iskhakov R. S.
Заглавие : Structure and magnetic properties of biogenic ferrihydrite nanoparticles doped with gadolinium
Место публикации : J. Sib. Fed. Univ. Math. Phys. - 2013. - Vol. 6, Is. 3. - P.358-365. - ISSN 1997-1397; Журн. СФУ. Сер. "Математика и физика"
Ключевые слова (''Своб.индексиров.''): ferrihydrite nanoparticle--bacterial culture klebsiela oxytoca--mössbauer spectroscopy--gadolinium doping
Аннотация: Bacterial culture Klebsiella oxytoca was grown in a Lovley medium at various concentrations of gadolinium salt. Biogenic magnetic nanoparticles of ferrihydrite were investigated by Mossbauer spectroscopy and magnetization curves were obtained. The results of structural studies showed that iron Fe(5) takes new position when cultivating is carried out in medium with high concentrations of gadolinium. It was found that gadolinium is fit into the crystal structure of ferrihydrite. These results are consistent with the analysis of the magnetization curves.
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