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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Chistyakov N. S., Tuschkov B. P.
Заглавие : Constituents measurement of complex superhighfrequency susceptibility of magnetic films
Коллективы : Академия наук СССР, Научный совет по комплексной проблеме "Физика твердого тела" АН СССР, Институт физики им. Л.В. Киренского Сибирского отделения РАН, Иркутский государственный педагогический институт, International colloquium on physics of magnetic films, Международный коллоквиум по физике магнитных пленок
Место публикации : International colloquium on physics of magnetic films: [program and abstracts]/ chairman L. V. Kirensky ; vice-chaiman: V. A. Buravikhin, R. V. Telesnin ; progr. and publ. com. N. M. Salansky ; progr. com.: V. A. Ignatchenko, Yu. V. Zakharov [et al]. - Irkutsk, 1968. - Section Ferromagnetic resonance, spin-wave resonance, high-frequency properties. - Ст.6-A.1. - P.59 (Шифр В37/H99-248389966)
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kuzmin E. V., Ovchinnikov S. G., Sandalov I. S.
Заглавие : Paramagnetic-susceptibility and phonon instability of metal with localized and collectivized electron state mixing
Место публикации : Fiz. Tverd. Tela. - 1980. - Vol. 22, Is. 2. - P.424-430. - ISSN 0367-3294
Примечания : Cited References: 22
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : ERUKHIMOV M. S.
Заглавие : MAGNETIC-SUSCEPTIBILITY OF INTERMEDIATE VALENCE COMPOUND FILMS
Место публикации : Fiz. Tverd. Tela: MEZHDUNARODNAYA KNIGA, 1982. - Vol. 24, Is. 11. - P3485-3487. - ISSN 0367-3294
Примечания : Cited References: 4
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : VERSHININ V. V., POLSKII A. I.
Заглавие : MAGNETOSTRICTIVE SUSCEPTIBILITY OF THIN-FILM TRANSFORMERS OF SURFACE ACOUSTIC-WAVES
Место публикации : Zhurnal Tek. Fiz.: MEZHDUNARODNAYA KNIGA, 1982. - Vol. 52, Is. 2. - P356-361. - ISSN 0044-4642
Примечания : Cited References: 4
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : PETRAKOVSKII G. A., FEDOSEEVA N. V., APLESNIN S. S., KOROLEV V. K.
Заглавие : IRREVERSIBLE BEHAVIOR OF SUSCEPTIBILITY AND MAGNETIZATION IN RB2MNXCD1-XCL4
Место публикации : Fiz. Tverd. Tela: MEZHDUNARODNAYA KNIGA, 1987. - Vol. 29, Is. 9. - P2579-2586. - ISSN 0367-3294
Примечания : Cited References: 11
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : AVERIANOV E. M.
Заглавие : LONGITUDINAL SUSCEPTIBILITY OF A UNIAXIAL NEMATIC
Место публикации : Zhurnal Eksperimentalnoi Teor. Fiz.: MEZHDUNARODNAYA KNIGA, 1990. - Vol. 97, Is. 3. - P855-862. - ISSN 0044-4510
Примечания : Cited References: 32
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Averyanov E. M.
Заглавие : Orientation ordering and critical behavior of discoid nematics
Место публикации : Zhurnal Eksperimentalnoi Teor. Fiz.: MEZHDUNARODNAYA KNIGA, 1996. - Vol. 110, Is. 5. - P1820-1840. - ISSN 0044-4510
Примечания : Cited References: 55
Предметные рубрики: LIQUID-CRYSTALS
PHASE-TRANSITION
ISOTROPIC-PHASE
LOCAL FIELD
SMECTIC-A
MOLECULES
SUSCEPTIBILITY
CONFORMATION
PARAMETER
DYNAMICS
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Shalaev V. M., Poliakov E. Y., Markel V. A.
Заглавие : Small-particle composites .2. Nonlinear optical properties
Место публикации : Phys. Rev. B: AMERICAN PHYSICAL SOC, 1996. - Vol. 53, Is. 5. - P2437-2449. - ISSN 0163-1829, DOI 10.1103/PhysRevB.53.2437
Примечания : Cited References: 45
Предметные рубрики: FRACTAL CLUSTERS
RAMAN-SCATTERING
SUSCEPTIBILITY
CONDUCTIVITY
EXCITATIONS
COLLOIDS
LIGHT
Аннотация: Strong fluctuations of local fields may result in very large optical nonlinearities in small-particle composites. Enhancement associated with particle clustering is found for a number of optical processes, including four-wave mixing (FWM), third-harmonic generation (THG), Raman scattering, and nonlinear refraction and absorption in Kerr media. Field fluctuations and optical nonlinear susceptibilities are especially large in fractal clusters. The enhancement of optical processes is expressed in terms of the resonant linear absorption by collective dipolar eigenmodes in a cluster, and quality factors, q, of the modes (q much greater than 1). It is shown that the susceptibility of a composite material consisting of random small-particle clusters is proportional to q(3) for Raman scattering and the Kerr optical nonlinearity, and to q(4) and q(6) for THG and FWM, respectively. For all of these processes, a spectral dependence of the effective susceptibility is found. Broad-scale numerical simulations of the optical response in small-particle composites are performed to complement the theory. The simulations are in reasonable agreement with available experimental data.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Bayukov O. A., Petrakovskii G. A., Savitskii A. F.
Заглавие : Orbital ordering in CuGeO3
Место публикации : Phys. Solid State: AMER INST PHYSICS, 1998. - Vol. 40, Is. 9. - P1534-1539. - ISSN 1063-7834, DOI 10.1134/1.1130602
Примечания : Cited References: 25
Предметные рубрики: SPIN-PEIERLS TRANSITION
COMPOUND CUGEO3
DIMERIZATION
STATE
SUSCEPTIBILITY
(VO)2P2O7
LADDER
Аннотация: The combined effect of the ligand crystal field and the exchange interaction on the Cu2+ cation in CuGeO3 is examined. It is shown that, if the magnitude of the exchange interaction exceeds the splitting of the energy levels of the d(x2-y2) and d(xy) orbitals, then an alternate filling of the d orbitals along a chain (orbital ordering) is possible. This effect creates an antiferromagnetic interaction between Cu2+ pairs in 90 degrees exchange and a doubling of the lattice period. A Jahn-Teller pseudoeffect causes singletization of the ground state of the antiferromagnetic chain of Cu2+ spins. (C) 1998 American Institute of Physics. [S1063-7834(98)02609-4].
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Petrakovskii G. A., Sablina K. A., Velikanov D. A., Vorotynov A. M., Volkov N. V., Bovina A. F.
Заглавие : Weak ferromagnetism in copper metaborate CuB2O4
Место публикации : Phys. Solid State: AMER INST PHYSICS, 1999. - Vol. 41, Is. 7. - P1157-1161. - ISSN 1063-7834, DOI 10.1134/1.1130957
Примечания : Cited References: 10
Предметные рубрики: SUSCEPTIBILITY
Аннотация: CuB2O4 single crystals have been grown and their magnetic and resonance properties have been investigated for the first time. The temperature dependence of the susceptibility was found to contain features at T = 21 and 10 K. The CuB2O4 single crystal transformed at T = 21 K to a weakly ferromagnetic state. The sharp drop in susceptibility at T 10 K is caused by a transition of the magnetic system of CuB2O4 to an antiferromagnetic state. The effective magnetic moment of the Cu2+ ion, determined from the high-temperature part of the magnetic susceptibility, is 1.77 mu(B). The room-temperature g factors are, respectively, 2.170 and 2.133 for magnetic field parallel and perpendicular to the c axis of the crystal. The antiferromagnetic resonance parameters in the weakly ferromagnetic and antiferromagnetic phases were measured. (C) 1999 American Institute of Physics. [S1063-7834(99)02907-X].
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11.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ignatchenko V. A., Man'kov Y. I., Pozdnyakov A. V.
Заглавие : Spin-wave susceptibility of partially randomized ferromagnetic superlattices
Место публикации : J. Exp. Theor. Phys.: MAIK NAUKA/INTERPERIODICA/SPRINGER, 1999. - Vol. 89, Is. 4. - P717-722. - ISSN 1063-7761, DOI 10.1134/1.559033
Примечания : Cited References: 15
Предметные рубрики: SPECTRUM
LOCALIZATION
Аннотация: This paper is a theoretical investigation of the effect of inhomogeneities in the period of a ferromagnetic superlattice on the high-frequency superlattice susceptibility. The calculations are done for a model in which the uniaxial magnetic anisotropy is taken as the physical parameter that characterizes both the ideal superlattice and a partially randomized superlattice. It is found that as the inhomogeneities become more intense, the two resonance peaks corresponding to the splitting of the spectrum at the edge of the Brillouin zone of the superlattice broaden, move closer to each other, and finally merge into one. The height of this peak increases and the peak width decreases as the intensity of the inhomogeneities increases further. The effect of inhomogeneities on the susceptibility differs dramatically in the two limits of short- and long-wave inhomogeneities: in the latter case (in contrast to the former) the dependence of the separation of the susceptibility peaks on the intensity and correlation properties of the inhomogeneities is nonmonotonic. The possibility of observing these effects in spin-wave resonance experiments involving multilayer magnetic films is also discussed. (C) 1999 American Institute of Physics. [S1063-7761(99)01510-3].
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12.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Petrakovskii G. A., Balaev A. D., Vorotynov A. M.
Заглавие : Magnetic susceptibility and magnetic-field behavior of CuB(2)O(4) copper metaborate
Место публикации : Phys. Solid State: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2000. - Vol. 42, Is. 2. - P321-325. - ISSN 1063-7834, DOI 10.1134/1.1131205
Примечания : Cited References: 10
Предметные рубрики: TRANSITION
STATE
Аннотация: An experimental study is reported regarding the temperature dependence of the magnetic susceptibility of a CuB(2)O(4) tetragonal single crystal within the 4.2-200-K range. It has been established that the magnetic susceptibility exhibits anomalies at 21 and 10 K and depends strongly on crystal orientation in the magnetic field. A study has been carried out of the field dependences of the magnetization of CuB(2)O(4) at various temperatures and crystal orientations. It is shown that for T 21 K, the crystal is in a paramagnetic state determined by Cu(2+) copper ions with an effective magnetic moment of 1.77 mu(B). Within the 10-21 K interval, the field dependence of the magnetization is typical of a weak ferromagnet with magnetic moments of the two antiferromagnetically coupled sublattices lying in the tetragonal plane of the crystal. The spontaneous weakly-ferromagnetic moment is 0.56 emu/g at 10 K. The canting angle of the sublattice magnetic moments, determined by the Dzyaloshinski-Moriya interaction, is 0.49 degrees. It is believed that below 10 K, the CuB(2)O(4) crystal retains its easy-plane magnetic structure, but with a zero spontaneous magnetic moment. (C) 2000 MAIK "Nauka/Interperiodica".
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13.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S.
Заглавие : Static and dynamic magnetic properties of coupled spin-1/2 antiferromagnetic chains
Место публикации : J. Phys.: Condens. Matter: IOP PUBLISHING LTD, 2000. - Vol. 12, Is. 37. - P.8191-8207. - ISSN 0953-8984, DOI 10.1088/0953-8984/12/37/316
Примечания : Cited References: 21
Предметные рубрики: ONE-DIMENSIONAL ANTIFERROMAGNETS
SYSTEMS
SUSCEPTIBILITY
EXCITATIONS
SR2CUO3
CA2CUO3
KCUF3
Ключевые слова (''Своб.индексиров.''): computational methods--copper compounds--correlation methods--functions--magnetic field effects--magnetic properties--magnetization--monte carlo methods--quantum theory--specific heat--thermal effects--excitation spectroscopy--interchain coupling--intrachain couplings--mean-field approximation--spin-spin correlation function--spinons--antiferromagnetic materials
Аннотация: Calculations of the thermodynamic quantities, and the spectra of spinons, triplet excitations, and two-particle spin-singlet (Delta S-z = 0, +/- 1) excitations for a weakly coupled antiferromagnetic S = 1/2 spin chain are made using a mean-field approximation for the interchain couplings (J(2)) by the quantum Monte Carlo method. The mass gaps in these excitation spectra are estimated as functions of the interchain coupling. The critical held H-c, and the temperatures at which the spinon and singlet gaps close (T-1 and T-2, respectively) are obtained. Some peculiarities of the staggered magnetization, the specific heat, and the spin-spin correlation function are found at T-1 = 0.9J(2), T-2 = 1.5J(2), H-c = 3.8J(2), as determined by linear function fitting for J(2)/J(1) 0.15 The intrachain and interchain couplings, and the staggered magnetization for KCuF3, Sr2CuO3, and Ca2CuO3 are estimated, and mass gaps are predicted to exist in the spectra of the spinons and the singlet two-particle excitations.
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14.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Belyaev B. A., Izotov A. V., Kiparisov S. Y.
Заглавие : Singularity in high-frequency susceptibility of thin magnetic films with uniaxial anisotropy
Место публикации : JETP Letters. - 2001. - Vol. 74, Is. 4. - P.226-230. - ISSN 0021-3640, DOI 10.1134/1.1413559
Примечания : Cited References: 9
Аннотация: A sharp peak of magnetic susceptibility has been observed in the ferromagnetic resonance spectra of uniaxial magnetic films placed in a planar field directed orthogonal to the easy magnetization axis, along which a pumping high-frequency magnetic field has been oriented. The peak width is considerably narrower than the line width of the uniform ferromagnetic resonance, and its position in a field equal to the film anisotropy field does not depend on the pumping frequency. The nature of the peak is associated with a drastic increase in the static transverse susceptibility of the film in the vicinity of the anisotropy field. It is shown phenomenologically that the peak can be observed only for quality samples with small angular and amplitude dispersion of the uniaxial anisotropy. (C) 2001 MAIK "Nauka/Interperiodica".
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15.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kliava J., Edelman I. S., Potseluyko A. M., Petrakovskaja E. A., Berger R., Bruckental I., Yeshurun Y., Malakhovskii A. V., Zarubina Y. V.
Заглавие : Magnetic and optical properties and electron paramagnetic resonance of gadolinium-containing oxide glasses
Место публикации : J. Phys.: Condens. Matter: IOP PUBLISHING LTD, 2003. - Vol. 15, Is. 40. - P6671-6681. - ISSN 0953-8984, DOI 10.1088/0953-8984/15/40/005
Примечания : Cited References: 30
Предметные рубрики: ABSORPTION-SPECTRA
FARADAY-ROTATION
SPIN-RESONANCE
IONS
GD3+
SPECTROSCOPY
BEHAVIOR
GD-3
Ключевые слова (''Своб.индексиров.''): doping (additives)--electronic structure--glass--lanthanum compounds--light absorption--magnetic susceptibility--oxides--paramagnetic resonance--positive ions--rate constants--substitution reactions--absorption band--gadolinium containing oxide glasses--positive weiss constants--gadolinium compounds
Аннотация: Magnetic susceptibility, electron paramagnetic resonance (EPR) and optical absorption have been studied in a glass system 20La(2)O(3)-22Al(2)O(3)-23B(2)O(3)-35(SiO2 + GeO2) with a part of La2O3 substituted by Gd2O3 in different concentrations. Positive Weiss constants have been found in more heavily doped glasses and ascribed to clustering of Gd3+ ions. Computer simulations of the EPR spectra show that the short-range ordering in the environment of the Gd3+ ions is well preserved. The relative distribution widths of the ligand coordinates are less than 2%. In the more heavily doped glasses the EPR spectra are superpositions of signals arising from isolated ions and ferromagnetic clusters. The increase of Gd3+ concentration is shown to change substantially the strong optical absorption edge while only small changes of f-f absorption band characteristics are observed. This difference is associated with the different effect of the Gd ion clustering on the mechanisms of the strong absorption in the ultraviolet region and the f-f absorption.
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16.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S., Piskunova N. I.
Заглавие : Influence of the four-spin exchange interaction on the magnetic properties of manganites
Место публикации : J. Phys.: Condens. Matter: IOP PUBLISHING LTD, 2005. - Vol. 17, Is. 37. - P.5881-5888. - ISSN 0953-8984, DOI 10.1088/0953-8984/17/37/023
Примечания : Cited References: 18
Предметные рубрики: METAL-INSULATOR-TRANSITION
PHASE
SUSCEPTIBILITY
LA1-XSRXMNO3
FERROMAGNET
TRANSPORT
Ключевые слова (''Своб.индексиров.''): computer simulation--ion exchange--lanthanum compounds--magnetic properties--monte carlo methods--phase diagrams--phase transitions--four-spin exchange interaction--magnetic phase diagram--manganites--metal-dielectric transition--manganese compounds
Аннотация: It is shown that non-Heisenberg exchange interaction should be taken into account to reproduce the magnetic phase diagram of La(1-x)A(x)MnO(3) (A = Ca, Sr) using only effective exchange parameters and spins. The formation of the four-spin exchange arises from carrier hopping and coincides with the critical concentration metal-dielectric transition. The two- and four-spin exchange parameters are determined by Monte Carlo simulations.
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17.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ignatchenko V. A., Mankov Y. I.
Заглавие : Effect of the correlation properties of one- and three-dimensional inhomogeneities on the high-frequency magnetic susceptibility of sinusoidal superlattices
Место публикации : Phys. Solid State: AMER INST PHYSICS, 2005. - Vol. 47, Is. 3. - P587-594. - ISSN 1063-7834, DOI 10.1134/1.1884725
Примечания : Cited References: 29
Предметные рубрики: PERIODIC MULTILAYERS
WAVE SPECTRUM
SPIN-WAVES
LOCALIZATION
SYSTEMS
DISORDER
Аннотация: The effect of one-(1D) and three-dimensional (3D) inhomogeneities on the high-frequency magnetic susceptibility at the boundary of the first Brillouin zone of a ferromagnetic superlattice is studied. The study is performed with an earlier developed method of random spatial modulation (RSM) of the superlattice period. In this method, structural inhomogeneities are described in terms of the random-phase model, in which the phase depends on three coordinates in the general case. The frequency spacing Delta v(m) between two peaks in the imaginary part of the averaged Green's function, which characterizes the gap width in the frequency spectrum at the boundary of the Brillouin zone, is calculated as a function of both the root-mean-square fluctuations gamma(i) and the correlation wavenumbers eta(i) of phase inhomogeneities (i = 1 and 3 for 1D and 3D inhomogeneities, respectively). The function Delta v(m)(gamma(1), eta(1)) for 1D inhomogeneities is shown to be symmetric with respect to inter- changing the variables gamma(1)(2) and eta(1), whereas the function Delta v(m)(gamma(3), eta(3)) for 3D inhomogeneities is strongly asym- metric with respect to interchanging gamma(3)(2) eta(3). This effect is associated with the difference in form between the correlation functions of 1D and 3D inhomogeneities and can be used to determine the dimensionality of inhomogeneities from the results of spectral studies of such superlattices. (c) 2005 Pleiades Publishing, Inc.
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18.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ignatchenko V. A., Mankov Y. I.
Заглавие : Effects of cross correlations between 1D and 3D inhomogeneities on the high-frequency susceptibility of superlattices
Место публикации : J. Exp. Theor. Phys.: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2006. - Vol. 102, Is. 4. - P625-635. - ISSN 1063-7761, DOI 10.1134/S106377610604011X
Примечания : Cited References: 29
Предметные рубрики: ELASTIC MEDIUM THEORY
3-DIMENSIONAL INHOMOGENEITIES
PERIODIC MULTILAYERS
SPIN-WAVES
LOCALIZATION
SPECTRUM
SYSTEMS
MEDIA
DISORDER
Ключевые слова (''Своб.индексиров.''): correlation methods--damping--function evaluation--wave equations--brillouin zone--distribution function--random variables--superlattices
Аннотация: Cross Correlations between components of a mixture of one-dimensional (I D) and three-diniensional (3D) inhomogenetics are described by introducing a distribution function taking into account correlations between absolute values of two random variables in the absence of correlations between the variables themselves. This distribution function is used for derivation and analysis of the superlattice correlation function containing a mixture of cross-correlated 1D and 3D in homogeneitics. The effect of such inhomogeneities on the high-frequency susceptibility at the edge of the first Brillouin zone of the superlattice is investigated. It is shown that positive cross correlations partly suppress the effect of a mixture of 1D and 3D inhomogeneities on the wave spectrum: the gap at the boundary of the Brillouin zone increases, and wave damping decreases as compared to the effect produced by a mixture of 1D and 3D inhomogeneities in the absence of cross correlations. Negative cross correlations lead to the opposite effect: the gap decreases and wave damping increases. Cross correlations also lead to the emergence of new resonance effects: a narrow dip or a narrow peak at the center of the band gap (depending on the sign of the correlation factor).
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19.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ritter C., Balaev A. D., Vorotynov A. M., Petrakovskii G. A., Velikanov D. A., Temerov V. L., Gudim, I. A.
Заглавие : Magnetic structure, magnetic interactions and metamagnetism in terbium iron borate TbFe3(BO3)(4): a neutron diffraction and magnetization study
Разночтения заглавия :авие SCOPUS: Magnetic structure, magnetic interactions and metamagnetism in terbium iron borate TbFe3(BO3)4: Aneutron diffraction and magnetization study
Место публикации : J. Phys.: Condens. Matter: IOP PUBLISHING LTD, 2007. - Vol. 19, Is. 19. - Ст.196227. - ISSN 0953-8984, DOI 10.1088/0953-8984/19/19/196227
Примечания : Cited References: 15
Предметные рубрики: GDFE3(BO3)(4)
Ключевые слова (''Своб.индексиров.''): magnetic structure--magnetic susceptibility--metamagnetism--neutron diffraction--neutron scattering--phase transitions--aneutron diffraction--magnetic interactions--neutron scattering measurements--terbium iron borate--terbium compounds
Аннотация: Magnetization, susceptibility and neutron scattering measurements were performed on the terbium iron borate TbFe3(BO3)(4). Structural and magnetic phase transitions were obtained as a function of external magnetic field and temperature. A metamagnetic transition of the terbium spins and a spin-flop transition of the iron sublattice are obtained at an external magnetic field 35 kOe Ht 60 kOe. The values of the effective exchange HE and the anisotropy HA fields are evaluated. Temperature dependent neutron diffraction studies reveal the magnetic structure of TbFe3(BO3)(4) and the thermal evolution of the two magnetic sublattices. An antiferromagnetic coupling along the helicoidal chains of Fe atoms sets in at 40 K with a propagation vector k
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20.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Popova M. N., Chukalina E. P., Stanislavchuk T. N., Malkin B. Z., Zakirov A. R., Antic-Fidancev E., Popova E. A., Bezmaternykh L. N., Temerov V. L.
Заглавие : Optical spectra, crystal-field parameters, and magnetic susceptibility of multiferroic NdFe3(BO3)(4)
Разночтения заглавия :авие SCOPUS: Optical spectra, crystal-field parameters, and magnetic susceptibility of multiferroic Nd Fe3 (B O3) 4
Место публикации : Phys. Rev. B: AMERICAN PHYSICAL SOC, 2007. - Vol. 75, Is. 22. - Ст.224435. - ISSN 1098-0121, DOI 10.1103/PhysRevB.75.224435
Примечания : Cited References: 22
Предметные рубрики: IRON BORATE GDFE3(BO3)(4)
CRYSTALLIZATION
SPECTROSCOPY
LASER
ND3+
Аннотация: We report high-resolution optical absorption spectra for NdFe3(BO3)(4) trigonal single crystal, which is known to exhibit a giant magnetoelectric effect below the temperature of magnetic ordering T-N=33 K. The analysis of the temperature-dependent polarized spectra reveals the energies and, in some cases, symmetries and exchange splittings of Nd3+ 84 Kramers doublets. We perform crystal-field calculations starting from the exchange-charge model, obtain a set of six real crystal-field parameters, and calculate wave functions and magnetic g factors. In particular, the values g(perpendicular to)=2.385 and g(parallel to)=1.376 were found for the Nd3+ ground-state doublet. We obtain B-loc=7.88 T and parallel to J(FN)parallel to=0.48 K for the values of the local effective magnetic field at liquid-helium temperatures at the Nd3+ site and the Nd-Fe exchange integral, respectively, using the experimentally measured Nd3+ ground-state splitting of 8.8 cm(-1). To check the reliability of our set of crystal-field parameters, we model the magnetic susceptibility data from literature. A dimer containing two nearest-neighbor iron ions in the spiral chain is considered to partly account for quasi-one-dimensional properties of iron borates, and then the mean-field approximation is used. The results of calculations with the exchange parameters for Fe3+ ions J(nn)=-6.25 K (intrachain interactions) and J(nnn)=-1.92 K (interchain interactions) obtained from fitting agree well with the experimental data.
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