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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Petrakovskii G. A., Ryabinkina L. I., Kiselev N. I., Velikanov D. A., Bovina A. F., Abramova G. M.
Заглавие : Colossal magnetoresistance of FexMn1-xS magnetic semiconductors
Место публикации : JETP Letters. - 1999. - Vol. 69, Is. 12. - P.949-953. - ISSN 0021-3640, DOI 10.1134/1.568118
Примечания : Cited References: 8
Предметные рубрики: MANGANITES
Аннотация: The magnetic, electric, magnetoresistive, and structural properties are investigated in the sulfide solid solutions FexMn1-xS, which are based on the antiferromagnetic semiconductor alpha-MnS (the fcc NaCl lattice). Colossal negative magnetoresistance (delta(H)similar to-83% at 160 K for x similar to 0.29), comparable to that observed in La-Ca-Mn-O polycrystals and films (delta(H)similar to-90% at 100 K and 40 kOe), is observed in compounds with intermediate concentrations 0.26 x 0.4, corresponding to the region of incipient ferromagnetism. (C) 1999 American Institute of Physics. [S0021-3640(99)01212-8].
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Volkov N. V., Petrakovskii G. A., Vasil'ev V. N., Sablina K. A.
Заглавие : Two-phase paramagnetic-ferromagnetic state of La0.7Pb0.3MnO3 single-crystal lanthanum manganite
Место публикации : Phys. Solid State: AMER INST PHYSICS, 2002. - Vol. 44, Is. 7. - P1350-1354. - ISSN 1063-7834, DOI 10.1134/1.1494635
Примечания : Cited References: 17
Предметные рубрики: COLOSSAL MAGNETORESISTANCE
MAGNETIC-RESONANCE
DOPED MANGANITES
LA1-XCAXMNO3
SEPARATION
TRANSITION
RELAXATION
EPR
Аннотация: Two phases, paramagnetic and ferromagnetic, were shown by the magnetic resonance method to coexist below the temperature T-C in La0.7Pb0.3MnO3 single crystals exhibiting colossal magnetoresistance. The magnetic resonance spectra were studied in the frequency range 10-78 GHz. The specific features in the behavior of the spectral parameters were observed to be the strongest at the temperatures corresponding to the maximum magnetoresistance in the crystals. The concentration ratios of the paramagnetic and ferromagnetic phases in the samples were found to be sensitive to variations in temperature and external magnetic field. This behavior suggests realization of the electronic phase separation mechanism in the system under study. (C) 2002 MAIK "Nauka/Interperiodica".
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Volkov N. V., Petrakovskii G. A., Vasiliev V. N., Velikanov D. A., Sablina K. A., Patrin K. G.
Заглавие : Observation of mixed two-phase state in Eu0.7Pb0.3MnO3 single crystal by magnetic resonance method
Место публикации : Physica B. - 2002. - Vol. 324, Is. 1-4. - P.254-260. - ISSN 0921-4526, DOI 10.1016/S0921-4526(02)01397-2
Примечания : Cited References: 19
Предметные рубрики: OPTIMALLY DOPED MANGANITES
COLOSSAL MAGNETORESISTANCE
PARAMAGNETIC ANOMALIES
CURIE-TEMPERATURE
LA1-XCAXMNO3
RELAXATION
SEPARATION
Ключевые слова (''Своб.индексиров.''): manganites--cmr--magnetic resonance--phase separation--cmr--magnetic resonance--manganites--phase separation--europium compounds--ferromagnetic materials--paramagnetic resonance--phase separation--phase transitions--manganites--single crystals
Аннотация: The magnetic resonance measurements show that the mixed two-phase state takes place in the Eu0.7Pb0.3MnO3 single crystal. The coexistence of the magnetic phases is observed in vicinity of the magnetic phase transition, where the sample exhibits the effect of the CMR. The frequency-field dependencies of the spectra allow to conclude that these phases are paramagnetic and ferromagnetic ones. Moreover, the study of the frequency dependencies shows the sensitivity of the mixed-phase state to the external magnetic field. This suggests that the scenario of the phase separation is realized in this case and the mixed two-phase state is not related to simple chemical inhomogeneity. (C) 2002 Elsevier Science B.V. All rights reserved.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S.
Заглавие : Anomalies in transport properties in a magnetically ordered region on a Kondo lattice
Место публикации : JETP Letters. - 2005. - Vol. 81, Is. 2. - P.66-71. - ISSN 0021-3640, DOI 10.1134/1.1887917
Примечания : Cited References: 33
Предметные рубрики: DOUBLE EXCHANGE MODEL
PHASE-SEPARATION
MANGANITES
LA1-XSRXMNO3
SYSTEMS
SHIFT
EDGE
Аннотация: The temperature dependences of resistivity and thermal emf on a Kondo lattice are calculated using the spinpolaron approximation. The peaks and sign reversal points of thermal emf as a function of temperature and concentration below the temperature of the transition to the paramagnetic state are determined. The concentration region containing the metal-insulator transition below the Curie temperature and the shift of the upper spin-polaron band are calculated. (c) 2005 Pleiades Publishing, Inc.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S., Piskunova N. I.
Заглавие : Influence of the four-spin exchange interaction on the magnetic properties of manganites
Место публикации : J. Phys.: Condens. Matter: IOP PUBLISHING LTD, 2005. - Vol. 17, Is. 37. - P.5881-5888. - ISSN 0953-8984, DOI 10.1088/0953-8984/17/37/023
Примечания : Cited References: 18
Предметные рубрики: METAL-INSULATOR-TRANSITION
PHASE
SUSCEPTIBILITY
LA1-XSRXMNO3
FERROMAGNET
TRANSPORT
Ключевые слова (''Своб.индексиров.''): computer simulation--ion exchange--lanthanum compounds--magnetic properties--monte carlo methods--phase diagrams--phase transitions--four-spin exchange interaction--magnetic phase diagram--manganites--metal-dielectric transition--manganese compounds
Аннотация: It is shown that non-Heisenberg exchange interaction should be taken into account to reproduce the magnetic phase diagram of La(1-x)A(x)MnO(3) (A = Ca, Sr) using only effective exchange parameters and spins. The formation of the four-spin exchange arises from carrier hopping and coincides with the critical concentration metal-dielectric transition. The two- and four-spin exchange parameters are determined by Monte Carlo simulations.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S., Ryabinkina L. I., Abramova G. M., Romanova O. B., Vorotynov A. M., Velikanov D. A., Kiselev N. I., Balaev A. D.
Заглавие : Conductivity, weak ferromagnetism, and charge instability in an alpha-MnS single crystal
Разночтения заглавия :авие SCOPUS: Conductivity, weak ferromagnetism, and charge instability in an α-MnS single crystal; авие SCOPUS: Conductivity, weak ferromagnetism, and charge instability in an ?-MnS single crystal
Место публикации : Phys. Rev. B: AMERICAN PHYSICAL SOC, 2005. - Vol. 71, Is. 12. - Ст.125204. - ISSN 1098-0121, DOI 10.1103/PhysRevB.71.125204; Phys. Rev. B Condens. Matter Mater. Phys. - 2005. - Vol. 71, Is. 12. - Ст.125204. - Вариант Sopus
Примечания : Cited References: 11
Предметные рубрики: MANGANITES
Ключевые слова (''Своб.индексиров.''): ferromagnetic material--manganese derivative--absorption spectroscopy--article--calculation--conductance--crystal--electron spin resonance--hybridization--magnetic field--magnetism--measurement--molecular interaction--temperature dependence--temperature measurement--ferromagnetic material--manganese derivative--absorption spectroscopy--article--calculation--conductance--crystal--electron spin resonance--hybridization--magnetic field--magnetism--measurement--molecular interaction--temperature dependence--temperature measurement
Аннотация: The temperature dependence of resistivity, magnetization, and electron-spin resonance of the α-MnS single crystal were measured in temperature range of 5 K T 550 K. Magnetization hysteresis in an applied magnetic field up to 0.7 T at T
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Volkov N. V., Petrakovskii G. A., Patrin K. G., Sablina K. A., Eremin E. V., Vasiliev V., Vasiliev A., Molokeev M. S., Boni P., Clementyev E.
Заглавие : Intrinsic inhomogeneity in a (La0.4Eu0.6)(0.7)Pb0.3MnO3 single crystal: Magnetization, transport, and electron magnetic resonance studies
Разночтения заглавия :авие SCOPUS: Intrinsic inhomogeneity in a (La0.4 Eu0.6) 0.7 Pb0.3 MnO3 single crystal: Magnetization, transport, and electron magnetic resonance studies
Место публикации : Phys. Rev. B: AMERICAN PHYSICAL SOC, 2006. - Vol. 73, Is. 10. - Ст.104401. - ISSN 1098-0121, DOI 10.1103/PhysRevB.73.104401
Примечания : Cited References: 29
Предметные рубрики: INSULATOR-METAL TRANSITION
PHASE-SEPARATION
MAGNETORESISTANCE
MANGANITES
EXCHANGE
STATE
Аннотация: Conventional magnetic and transport measurements of the melt-grown mixed-valence manganite (La0.4Eu0.6)(0.7)Pb0.3MnO3 have been supplemented by a magnetic resonance study. The experimental data support the model of two magnetic phases coexisting in the crystal volume. At a temperature T-*, which is well above Curie temperature T-C, ferromagnetic clusters appear in the sample. These ferromagnetic regions possess a higher conductivity in comparison with the paramagnetic background (majority phase). On cooling through T-C, the magnetization of the spatially confined ferromagnetic clusters of the minority phase freezes in random directions with respect to the magnetization of the ferromagnetic majority phase due to the difference of the exchange interactions at the phase boundaries from the intraphase interactions in sign and value. Such a mixed state is responsible for the observed magnetic glassylike behavior of the system that is characteristic of inhomogeneous magnets. The fluctuations of the magnetic coupling value and sign in the sample volume are related to strong competition between the ferromagnetic and antiferromagnetic exchange interactions, which, in turn, results from the quenched disorder caused by the random chemical replacement of the perovskite A site of the manganite. A phase-separation state comprised of two different ferromagnetic phases has been used to account for the colossal magnetoresistance phenomenon and the magnetic-field-driven nonlinear conduction found in the crystal.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S., Piskunova N. I.
Заглавие : Anomalies in magnetoresistance and in the bulk modulus for ferromagnetics with four-spin exchange interaction on the Kondo lattice
Место публикации : J. Phys.: Condens. Matter: IOP PUBLISHING LTD, 2006. - Vol. 18, Is. 29. - P.6859-6868. - ISSN 0953-8984, DOI 10.1088/0953-8984/18/29/023
Примечания : Cited References: 29
Предметные рубрики: MIXED-VALENCE MANGANITES
PHASE-SEPARATION
LA1-XSRXMNO3
BEHAVIOR
PECULIARITIES
TRANSITION
Ключевые слова (''Своб.индексиров.''): elastic moduli--electric resistance--ferromagnetism--function evaluation--paramagnetism--transceivers--adiabatic approximation--kondo lattice--paramagnetic state--ring exchange--magnetoresistance
Аннотация: The temperature dependence of resistivity and the bulk modulus are calculated on the Kondo lattice, with ring exchange between localized spins, using the spin-polaron and adiabatic approximation. Peak and zero values of the bulk modulus as functions of temperature and concentration are determined below the temperature of the transition to the paramagnetic state. The effects of the nearest order between transverse spin components and a value of the ring exchange between localized spins on magnetoresistivity are estimated.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Martyanov O., Yudanov V., Lee R., Volkov N. V., Sablina K. A.
Заглавие : A tool to investigate the spatial magnetic phase separation phenomena in manganites
Место публикации : Physics of the Solid State. - 2006. - P.1–3
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Gavrichkov V. A., Ovchinnikov S. G., Yakimov L. E.
Заглавие : The role of orbital ordering in the formation of electron structure in undoped LaMnO3 manganites in the regime of strong electron correlations
Место публикации : J. Exp. Theor. Phys.: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2006. - Vol. 102, Is. 6. - P972-985. - ISSN 1063-7761, DOI 10.1134/S1063776106060112
Примечания : Cited References: 25
Предметные рубрики: COLOSSAL MAGNETORESISTIVE OXIDES
DOUBLE EXCHANGE
BAND
MODEL
Ключевые слова (''Своб.индексиров.''): computational methods--correlation methods--doping (additives)--electrons--ferromagnetic materials--lanthanum compounds--paramagnetic materials--intraatomic electron correlations--mott hubbard correlation gap--orbital ordering--paramagnetic phases--electronic structure
Аннотация: The electron structure of undoped LaMnO3 and slightly doped La1-xSrxMnO3 manganites has been calculated within the framework of a generalized tight binding method with explicit allowance for strong intra-atomic electron correlations. According to the results of these calculations, the ground state in orbitally disordered undoped LaMnO3 ferromagnets would be metallic despite the Mott-Hubbard correlation gap in the spectrum of quasiparticles. Owing to the orbital ordering, the insulating state is stabilized in both antiferromagnetic and paramagnetic phases. In-gap states of a polaron nature with a spectral weight proportional to the dopant concentration have been found near the top of the valence band in La1-xSrxMnO3. As the doping level increases, a metal state appears in the ferromagnetic phase, which has a metallic character for one spin subband and an insulating character for the other subband (representing the so-called half-metallic state).
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11.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aplesnin S. S.
Заглавие : Effect of bond fluctuations on the transport properties of manganites and nickelates
Место публикации : J. Exp. Theor. Phys.: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2007. - Vol. 104, Is. 5. - P766-774. - ISSN 1063-7761, DOI 10.1134/S1063776107050111
Примечания : Cited References: 26
Предметные рубрики: NEUTRON-DIFFRACTION
CHARGE DISPROPORTIONATION
ELECTRONIC-STRUCTURE
MAGNETIC ORDER
TRANSITIONS
PEROVSKITES
PRNIO3
GAP
Ключевые слова (''Своб.индексиров.''): crystal structure--manganites--optimization--thermal conductivity--thermal effects--bond fluctuations--nickelates--orthorhombic crystal structure--nickel compounds
Аннотация: For the manganites RMnO(3) (R = La, Pr, Nd), a mechanism is proposed to explain the anomalous temperature dependences of the kinetic coefficients, resistivity, and thermoelectric power during the transition from the pseudocubic O to the orthorhombic O' crystal structure. The contributions of the bending and stretching modes of the octahedron to the formation of thermal-conductivity maxima and to the deviation from the linear dependence of ln(rho/T) on 1/T at low temperatures have been estimated. In nickelates, the metal-insulator transition is caused by lattice-polaron pinning by the stretching mode of the octahedron, and the low-temperature anomaly of the thermal conductivity is related to electron scattering by the bending mode of the octahedron.
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12.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zinenko V. I., Pavlovskii M. S.
Заглавие : Lattice dynamics and the phase transition from the cubic phase to the tetragonal phase in the LaMnO3 crystal within the polarizable-ion model
Место публикации : Phys. Solid State: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2007. - Vol. 49, Is. 9. - P1749-1758. - ISSN 1063-7834, DOI 10.1134/S1063783407090235
Примечания : Cited References: 23
Предметные рубрики: NEUTRON-DIFFRACTION
PEROVSKITES
MANGANITES
PHONONS
Аннотация: The paper reports on the results of ab initio calculations of the static and dynamic properties of the LaMnO3 crystal with a perovskite structure in the cubic, rhombohedral, and orthorhombic phases. The calculations are performed within the ionic crystal model, which takes into account the deformability and polarizability of the ions. It is revealed that the spectrum of lattice vibrations in the cubic phase contains unstable vibrational modes, which occupy the phase space in the entire Brillouin zone. The eigenvectors of the softest mode at the boundary point R of the Brillouin zone are associated with the displacements of the oxygen ions and correspond to the "rotation" of the MnO6 octahedron. The condensation of one, two, and three components of this mode leads to the tetragonal, orthorhombic, and rhombohedral distortions of the structure. The structural phase transition is described in terms of the local mode approximation with the use of the double perovskite unit cell, in which the MnO6 octahedron is explicitly separated. The parameters of the model Hamiltonian are determined. The static properties are investigated by the Monte Carlo method. The calculated temperature of the phase transition from the cubic phase (9800 K) is considerably higher than the melting temperature of the crystal under investigation. The calculated frequencies of long-wavelength lattice vibrations in the experimentally observed orthorhombic and rhombohedral phases are in reasonable agreement with experimental data.
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14.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Val'kov V. V.
Заглавие : Double exchange model in the problem of the colossal magnetoresistance manganites
Коллективы : "New Layered 3d-Materials for Spintronics", Workshop INTAS - Siberian Branch of the Russian Academy of Sciences Scientific Cooperation on the Research Project
Место публикации : Workshop INTAS - Sib. Branch of the RAS Sci. Cooperation on the Res. Project “New Layered 3d-Materials for Spintronics”/ chairman G. A. Petrakovskii. - 2007. - P.8
Аннотация: INTAS (The International Association for the Promotion of Cooperation with Scientists from the New Independent States of the Former Soviet Union) — международная ассоциация по содействию сотрудничеству с учёными новых независимых государств бывшего Советского Союза. Некоммерческая организация, финансировалась главным образом из бюджета Европейского Союза. Являлась крупнейшим фондом, поддерживающим научное сотрудничество между учёными стран бывшего СССР и Европейского Союза с 1993 г. Программы INTAS охватывали широкий круг научно-исследовательских проблем. 22 сентября 2006 года было принято решение о прекращении осуществления программы на основании рекомендации Европейской Комиссии. С 1 апреля 2007 года прекратилось распределение новых грантов.
Материалы семинара,
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15.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Volkov N. V., Eremin E. V., Shaykhutdinov K. A., Tsikalov V. S., Petrov M. I., Balaev D. A., Semenov S. V.
Заглавие : The magnetic-field-driven effect of microwave detection in a manganite granular system
Место публикации : J. Phys. D. - 2008. - Vol. 41, Is. 1. - Ст.15004. - ISSN 0022-3727, DOI 10.1088/0022-3727/41/1/015004
Примечания : Cited References: 24
Предметные рубрики: IDENTICAL METALS
TUNNEL-JUNCTIONS
MAGNETORESISTANCE
RECTIFICATION
SPINTRONICS
TEMPERATURE
PEROVSKITES
Ключевые слова (''Своб.индексиров.''): bias currents--curie temperature--electric power generation--granular materials--magnetic field effects--microwave irradiation--voltage measurement--direct current voltage--magnetic tunnel junctions--metal insulator metal junctions--nonmagnetic metals--manganites
Аннотация: We demonstrate the microwave detection effect in a granular La0.7Ca0.3MnO3 sample. Dc voltage generated by the sample in response to microwave irradiation below the Curie temperature is found to be dependent on the applied magnetic field. The magnetic field dependence of the dc voltage has a broad peak resembling an absorption line. The detection effect depends substantially on the magnetic history of the sample; however, identical measurement conditions provide reproducibility of the experimental results. The detected dc voltage increases linearly with microwave power and strongly depends on a bias current through the sample. According to the results of systematic measurements, there exist two contributions to a value of the detected output signal. The first is magneto-independent; it can be explained in the framework of a mechanism used traditionally for description of the rectification effect in metal-insulator-metal junctions with nonmagnetic metals. The other is magneto-dependent; it originates from the interplay between the spin-dependent current through magnetic tunnel junctions and spin dynamics of the grains, which form these junctions in the sample.
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16.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Kartashev A. V., Flerov I. N., Volkov N. V., Sablina K. A.
Заглавие : Heat capacity and magnetocaloric effect in manganites (La1-yEuy)0.7Pb0.3MnO3 (y = 0.2; 0.6)
Коллективы : Moscow International Symposium on Magnetism, Московский государственный университет им. М.В. Ломоносова, Российский фонд фундаментальных исследований
Место публикации : Moscow Int. Symp. on Magnet. (MISM-2008): June 20-25, 2008, Moscow : book of abstract. - 2008. - Ст.24PO-7-25. - p.639-640
Примечания : Библиогр.: 1. - Support by the Council of Grants from the President of the Russian Federation for Support of Leading Scientific Schools (project no. NSh -1011.2008.2) is acknowledged
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17.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Gavrichkov V. A., Ovchinnikov S. G.
Заглавие : Polaron in-gap states in CMR manganites
Коллективы : Moscow International Symposium on Magnetism, Московский государственный университет им. М.В. Ломоносова, Российский фонд фундаментальных исследований
Место публикации : Moscow Int. Symp. on Magnet. (MISM-2008): 2008, June 20-25 : book of abstracts. - 2008. - Ст.24PO-7-15. - P.630
Примечания : Библиогр.: 1
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18.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kartashev A. V., Flerov I. N., Volkov N. V., Sablina K. A.
Заглавие : Adiabatic calorimetric study of the intense magnetocaloric effect and the heat capacity of (La(0.4)Eu(0.6))(0.7)Pb(0.3)MnO(3)
Коллективы :
Разночтения заглавия :авие SCOPUS: Adiabatic calorimetric study of the intense magnetocaloric effect and the heat capacity of (La0.4Eu0.6)0.7Pb 0.3MnO3
Место публикации : Phys. Solid State: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2008. - Vol. 50, Is. 11. - P2115-2120. - ISSN 1063-7834, DOI 10.1134/S1063783408110188
Примечания : Cited References: 15. - This study was supported by the Council on Grants from the President of the Russian Federation for the Support of Leading Scientific Schools of the Russian Federation (NSh-1011.2008.2) and the Siberian Branch of the Russian Academy of Sciences ( Lavrent'ev Competition of Young Scientists Projects, grant no. 51) within the framework of the Integration Project no. 3.7 of the Siberian Branch of the Russian Academy of Sciences.
Предметные рубрики: LA0.7CA0.3MNO3
MANGANITES
Ключевые слова (''Своб.индексиров.''): 75--30--sg--75--40--cx
Аннотация: The temperature dependences of the intense magnetocaloric effect T (AD)(T, H) and the heat capacity C (p) (T) of the (La(0.4)Eu(0.6))(0.7)Pb(0.3)MnO(3) manganite are directly measured using adiabatic calorimetry. The experimental dependences T (AD)(T) are in satisfactory agreement with those calculated from the data on the behavior of the magnetization. The factors responsible for the absence of an anomaly in the experimental temperature dependence of the heat capacity C (p) (T) in the range of the magnetic phase transition are discussed.
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19.

Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Kartashev A.V., Flerov I.N., Volkov N.V., Sablina K.A.
Заглавие : Intensive and extensive magnetocaloric effect in manganites (La1-yEuy)0.7Pb0.3MnO3
Коллективы : International Conference on Magnetism
Место публикации : 18th International Conference on Magnetism (ICM-2009). - 2009. - Ст.Mo-A-5.1-03
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20.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Orlov Y. S., Ovchinnikov S. G.
Заглавие : Construction of a Multielectron Basis for Mott Insulators with Strong Electron Correlations, Spin-Orbit Interaction, and Covalence
Место публикации : J. Exp. Theor. Phys. - 2009. - Vol. 109, Is. 2. - P.322-338. - ISSN 1063-7761, DOI 10.1134/S1063776109080196
Примечания : Cited References: 35
Предметные рубрики: NARROW ENERGY BANDS
MAGNETIC ANISOTROPY ENERGY
ORIGIN
TRANSITION
PHYSICS
MANGANITES
OXIDES
CHARGE
Аннотация: We propose that the apparatus of quantum mechanics of a free atom (in particular, the theory of nj symbols and Rakah-Wigner genealogic coefficients generalized to the case of point groups and widely used in crystal field theory) be used for constructing multielectron bases with allowance for covalence and spin-orbit interaction. This allows us to take into account the electron-electron interaction for 3d ions the most comprehensively. The basis constructed in this way can be used in the generalized strong coupling method for the multiband p-d model in describing the structure of the quasiparticle energy spectrum and physical properties of systems with strong electron correlations. The procedure of construction and computation is demonstrated for the (5)T(2g) term in the d(6) configuration of the transition metal atom in an octahedral field. The mechanism for the emergence of magnetic anisotropy in S ions (Fe(3+) and Mn(2+)) due to covalent mixing of d(6) (L) under bar configurations with a nonzero orbital angular momentum ((L) under bar is a hole in ligands) is demonstrated
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