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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Orlov Yu. S., Nikolaev S. V., Ovchinnikov S. G., Nesterov A. I.
Заглавие : Ultrafast Quantum Relaxation Dynamics of Magnetically Ordered Systems with Spin Crossover in an Excited State under a Sudden Perturbation
Место публикации : JETP Letters. - 2020. - Vol. 112, Is. 4. - P.250-256. - ISSN 0021-3640, DOI 10.1134/S0021364020160109. - ISSN 1090-6487(eISSN)
Примечания : Cited References: 27. - This work was supported by the Russian Science Foundation (project no. 18-12-00022)
Аннотация: A theoretical model based on the relaxation equation for the density matrix has been proposed to describe the ultrafast time dynamics of magnetically ordered systems with spin crossover in an excited state under a sudden perturbation. Oscillations of the magnetization, the population of the high-spin state, and the generation of local vibrons at a transition of the system from the light-excited Franck-Condon low-spin state to the highspin ground state.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Orlov Yu. S., Nikolaev S. V., Nesterov A. I., Ovchinnikov S. G.
Заглавие : Light-induced ultrafast dynamics of spin crossovers under high pressure
Место публикации : J. Exp. Theor. Phys. - 2021. - Vol. 132, Is. 3. - P.399-415. - ISSN 10637761 (ISSN), DOI 10.1134/S1063776121030079
Примечания : Cited References: 71. - The authors thank the Russian Scientific Foundation for the financial support under the grant 18-12-00022
Аннотация: Within the multielectron model of magnetic insulator with two different spin terms at each cation and spin crossover under high pressure we have studied dynamics of a sudden excited non equilibrium spin state. We obtain the different relaxation of the magnetization, high spin/low spin occupation numbers, and the metal-oxygen bond length for different values of the external pressure. For each pressure-temperature values stationary state agrees to the mean field phase diagrams. We found the long living oscillations of magnetization for the high spin ground state at small pressure. Close to crossover pressure the smooth relaxation is accompanied with a set of sharp strongly non linear oscillations of magnetization and HS/LS occupation numbers that are accompanied by the Franck–Condon resonances.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Mikhaylovskiy, R., V, Huisman T. J., Gavrichkov V. A., Polukeev S. I., Ovchinnikov S. G., Afanasiev D., Pisarev, R., V, Rasing, T.h., Kimel, A., V
Заглавие : Resonant Pumping of d-d Crystal Field Electronic Transitions as a Mechanism of Ultrafast Optical Control of the Exchange Interactions in Iron Oxides
Место публикации : Phys. Rev. Lett. - 2020. - Vol. 125, Is. 15. - Ст.157201. - ISSN 0031-9007, DOI 10.1103/PhysRevLett.125.157201. - ISSN 1079-7114(eISSN)
Примечания : Cited References: 46. - We thank A. Toonen and S. Semin for technical assistance. The work at Radboud University was supported by de Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO) and the European Research Council ERC Grant Agreement No. 339813 (Exchange). R. V. M. thanks ERC, Grant Agreement No. 852050 (MAGSHAKE). V. A. G., S. I. P., and S. G. O. are thankful to the Russian Science Foundation for the financial support under the Grant No. 18-12-00022. The theoretical part of this research was performed by V. A. G., S. I. P., and S. G. O. under the RSF Grant No. 18-12-00022. The contribution of R. V. P. into the experimental part was supported by the RSF Grant No. 16-12-10456
Предметные рубрики: BORATE
Аннотация: The microscopic origin of ultrafast modification of the ratio between the symmetric (J) and antisymmetric (D) exchange interaction in antiferromagnetic iron oxides is revealed, using femtosecond laser excitation as a pump and terahertz emission spectroscopy as a probe. By tuning the photon energy of the laser pump pulse we show that the effect of light on the D/J ratio in two archetypical iron oxides FeBO3 and ErFeO3 is maximized when the photon energy is in resonance with a spin and parity forbidden d-d transition between the crystal-field split states of Fe3+ ions. The experimental findings are supported by a multielectron model, which accounts for the resonant absorption of photons by Fe3+ ions. Our results reveal the importance of the parity and spin-change forbidden, and therefore often underestimated, d-d transitions in ultrafast optical control of magnetism.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ekholm V., Chiuzbaian G. S., Sathe C., Nicolaou A., Guarise M., Simon M., Jaouen N., Luning J., Hague C. F., Gel'mukhanov F., Odelius M., Bjorneholm O., Rubensson, J-E
Заглавие : Core-hole localization and ultra-fast dissociation in SF6
Коллективы : Swedish Research Council (VR)Swedish Research Council; Russian Science FoundationRussian Science Foundation (RSF) [16-12-10109]
Место публикации : J. Phys. B. - 2020. - Vol. 53, Is. 18. - Ст.185101. - ISSN 0953-4075, DOI 10.1088/1361-6455/aba204. - ISSN 1361-6455(eISSN)
Примечания : Cited References: 36. - This work was supported by the Swedish Research Council (VR). The calculations were performed on resources provided by the Swedish National Infrastructure for Computing (SNIC). FG acknowledges support within the Russian Science Foundation (Project No. 16-12-10109)
Предметные рубрики: X-RAY-EMISSION
SYMMETRY-BREAKING
AB-INITIO
SPECTROSCOPY
SPECTRA
Аннотация: Resonant inelastic x-ray scattering spectra excited at the fluorine K resonances of SF6 have been recorded. While a small but significant propensity for electronically parity-allowed transitions is found, the observation of parity-forbidden electronic transitions is attributed to vibronic coupling that breaks the global inversion symmetry of the electronic wavefunction and localizes the core hole. The dependence of the scattering cross section on the polarization of the incident radiation and the scattering angle is interpreted in terms of local π/σ symmetry around the S–F bond. This symmetry selectivity prevails during the dissociation that occurs during the scattering process.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Liu, Yan Rong, Wu, Yong, Wang, Jian Guo, Vendrell, Oriol, Kimberg V., Zhang, Song Bin
Заглавие : Electron-rotation coupling in diatomics under strong-field excitation
Место публикации : Phys. Rev. A. - 2020. - Vol. 102, Is. 3. - Ст.033114. - ISSN 2469-9926, DOI 10.1103/PhysRevA.102.033114. - ISSN 2469-9934(eISSN)
Примечания : Cited References: 78. - S.B.Z. thanks H. D. Meyer for his helpful instructions of Wigner-DVR in MCTDH. Grants from the National Basic Research Program of China (2017YFA0403200), NSFC (No. 11604197, No. 11974230, and No. 11934004), the Science Challenge Program of China (TZ2018005 and TZ2016005) are acknowledged. V.K. acknowledges financial support from Swedish Research Council (VR) and the Ministry of Science and High Education of Russian Federation, Project No. FSRZ2020-0008.
Предметные рубрики: REAL-TIME OBSERVATION
DYNAMICS
LASER
ULTRAFAST
MOLECULES
Аннотация: he photoexcitation and photodissociation of diatomic molecules by intense pulse lasers has been the subject of extensive investigations over the past decades. However, the usually employed theoretical framework neglects the coupling between the molecular rotational angular momentum (R) and the angular momentum of the electrons projected onto the molecular axis Ω=Λ+Σ, which results in the known Λ-doubling phenomenon in high-resolution electronic spectra of diatomic molecules. While neglecting this coupling is an excellent approximation in the weak-field or perturbative regime owing to the large mass difference between the rotating atoms and the electrons, the approximation breaks down for intense laser pulses because of the repeated Rabi cycling of the electronic transitions, which can have a significant effect on the rotational degrees of freedom of the molecule. By correcting the transition dipole matrix elements and introducing angular basis sets based on Wigner D functions, the conventional theoretical treatment is generalized to a universal description valid for both the weak- and strong-field regimes. The theoretical treatment developed here is applied to the ∣1Σ› to ∣1Π› transitions in diatomic systems. Our results reveal that, for field intensities resulting in about one Rabi cycling for extreme ultraviolet or x-ray transitions, the theoretical predictions by the conventional theoretical frame need to be corrected when considering observables such as the molecular alignment and the angular distribution of the photofragments.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aleksandrovsky A.S., Vyunishev A.M., Zaitsev A.I., Slabko V.V.
Заглавие : Random quasi-phase-matched conversion of broadband radiation in a nonlinear photonic crystal
Место публикации : Phys. Rev. A. - 2010. - Vol. 82, Is. 5. - ISSN 1050-2947, DOI 10.1103/PhysRevA.82.055806
Примечания : Cited Reference Count: 22. - Гранты: The work was supported by the Ministry of Education and Science of the Russian Federation (Contract 16.740.11.0150), Grant of the President of the Russian Federation for the support of leading scientific schools No. SS-4645.2010.2, Grant No. RNP.2.1.1.3455, Projects 2.5.2 and 3.9.1 of PSB RAS, and Projects No. 27.1 and No. 5 of SB RAS. A. M. Vyunishev is grateful for the support from Krasnoyarsk Regional Fund of Science and Technical Activity Support.Финансирующая организация: Ministry of Education and Science of the Russian Federation [16.740.11.0150]; Russian Federation for the support of leading scientific schools [SS-4645.2010.2, RNP.2.1.1.3455]; PSB RAS [2.5.2, 3.9.1]; SB RAS [27.1, 5]; Krasnoyarsk Regional Fund of Science and Technical Activity
Ключевые слова (''Своб.индексиров.''): broad spectrum--broadband radiation--femtosecond laser pulse--fundamental wave--nonlinear generation--nonlinear photonic crystals--quasi-phase-matched--quasi-phase-matched frequency doubling--red shift--shorter wavelength--tetraborate--tuning ranges--vacuum ultraviolets--band structure--crystal structure--strontium--ultrafast lasers--ultrashort pulses--photonic crystals
Аннотация: Radiation in the range 187.5-215 nm was generated via random quasi-phase-matched frequency doubling of femtosecond laser pulses in nonlinear photonic crystals of strontium tetraborate. Abroad spectrum of fundamental radiation favors the probing of the nonlinear photonic crystal band structure. The red shift of the band structure upon the fundamental wave-vector rotation was observed. No principal limitations of the tuning range at its shorter wavelength boundary from the nonlinear photonic crystal (NPC) material are found. Calculation shows that the NPC structure enables enhancement of nonlinear generation in the vacuum ultraviolet.
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Orlov Yu. S., Nikolaev S. V., Ovchinnikov S. G.
Заглавие : Light-induced ultrafast quantum relaxation dynamics of magnetically ordered spin crossover systems
Коллективы : Российская академия наук, Физико-технический институт им. Е.К. Завойского ФИЦ Казанского научного центра РАН, Казанский (Приволжский) федеральный университет, Euro-Asian Symposium "Trends in MAGnetism", "Trends in MAGnetism", Euro-Asian Symposium
Место публикации : VIII Euro-Asian symposium "Trends in magnetism" (EASTMAG-2022): Book of abstracts/ program com. S. G. Ovchinnikov [et al.]. - 2022. - Vol. 2, Sect. H: Magnetism of strongly correlated electron systems. - Ст.H.P16. - P.106. - ISBN 978-5-94469-051-7
Примечания : Cited References: 1. - The study was supported by the Russian Scientiʅc Foundation, the Krasnoyarsk Regional Fund of Science, grant No. 22-22-20007
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Orlov Yu. S., Nikolaev S. V., Ovchinnikov S. G.
Заглавие : Light-Induced Ultrafast Quantum Relaxation Dynamics of Magnetically Ordered Spin Crossover Systems under High Pressure
Коллективы : "Functional materials", International conference, Крымский федеральный университет имени В.И. Вернадского
Место публикации : Ovchinnikov S. G. International conference "Functional materials": book of abstracts/ ed. V. N. Berzhansky ; org. com. S. G. Ovchinnikov [et al.]. - Simferopol, 2021. - P.46
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Liu, Ji-Cai, Savchenko, Viktoriia, Kimberg V., Gel'mukhanov F., Odelius, Michael
Заглавие : High-resolution x-ray spectra of carbon monoxide reveal ultrafast dynamics induced by long UV pulse
Коллективы : RFBRRussian Foundation for Basic Research (RFBR) [19-29-12015]; National Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [11974108, 11574082]; Fundamental Research Funds for the Central UniversitiesFundamental Research Funds for the Central Universities [2021MS046]; European UnionEuropean Commission [860553]; Carl Tryggers Foundation [CTS18:285]; Helmholtz Virtual Institute [VI419]; Swedish Research CouncilSwedish Research CouncilEuropean Commission [VR 2019-03470, 2018-05973]
Место публикации : New J. Phys. - 2021. - Vol. 23, Is. 6. - Ст.063030. - ISSN 1367-2630, DOI 10.1088/1367-2630/ac0198
Примечания : Cited References: 47. - The reported study was funded by RFBR, project number 19-29-12015. J-CL thanks the support by the National Science Foundation of China under Grant Nos. 11974108, 11574082, and the Fundamental Research Funds for the Central Universities (No. 2021MS046). MO acknowledges funding from the European Union's Horizon 2020 research and innovation programme under the Marie Skodowska-Curie Grant Agreement No. 860553 and the Carl Tryggers Foundation (contract CTS18:285). FG acknowledges also the support from the Helmholtz Virtual Institute VI419 'Dynamic Pathways in Multidimensional Landscapes'. VK acknowledges the Swedish Research Council (VR 2019-03470). The calculations were partially enabled by resources provided by the Swedish National Infrastructure for Computing (SNIC) partially funded by the Swedish Research Council through Grant Agreement No. 2018-05973
Предметные рубрики: VIBRATIONAL STRUCTURE
SCATTERING
RAMAN
CO
COLLAPSE
PROBE
Аннотация: In theoretical simulations of a UV + x-ray pump-probe (UVX-PP) setup, we show that frequency detuning of the pump UV pulse acts as a camera shutter by regulating the duration of the UVX-PP process. This two-photon absorption with long overlapping UV and x-ray pulses, allowing for high spectral resolution, thereby provides information about ultrafast dynamics of the nuclear wave packet without the requirement of ultrashort pulses and controlled delay times. In a case study of carbon monoxide, the calculated UVX-PP spectra of the O1s−12π1 and C1s−12π1 core-excited states show different vibrational profiles. The interference of intermediate vibrational states reveals details of nuclear dynamics in the UVX-PP process related to a variable duration time controlled by the UV detuning. Both O1s−12π1 and C1s−12π1 pump-probe channels display a splitting of the spectral profile, which however is associated with different physical mechanisms. At the O1s−12π1 resonance, the observed dispersive and non-dispersive spectral bands intersect and result in destructive interference.
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zhou G., Ren Q., Molokeev M. S., Zhou Y., Zhang J., Zhang X. -M.
Заглавие : Unraveling the ultrafast self-assembly and photoluminescence in zero-dimensional Mn2+-based halides with narrow-band green emissions
Место публикации : ACS Appl. Electron. Mater. - 2021. - Vol. 3, Is. 9. - P.4144-4150. - ISSN 26376113 (ISSN), DOI 10.1021/acsaelm.1c00606
Примечания : Cited References: 37. - This work is supported by the Natural Science Foundation of China (no. 21871167) and the 1331 project of Shanxi Province and funded by RFBR according to the research project no. 19-52-80003
Аннотация: The discovery of narrow-band luminescent materials remains an immense challenge to optimize the performance of white light-emitting diodes (LEDs). So far, the zero-dimensional (0D) Mn2+-based halides with near-unity narrow-band emissions have emerged as a class of promising phosphors in solid-state displays, but the related large-scale synthesis strategies have not been proposed and evaluated. Herein, we report an in situ synthetic process of 0D Mn2+-based halides and utilize (C20H20P)2MnBr4 as a case to investigate the photoluminescence characteristics and the structural essence of ultrafast self-assembly. The bright green emission peak at 523 nm with a full width at half maximum of 48 nm for (C20H20P)2MnBr4 is attributed to the d–d transition (4T1–6A1) of tetrahedrally coordinated [MnBr4]2– centers, and the fabricated white LED device shows a wide color gamut of 103.7% National Television System Committee (NTSC) standard. Remarkably, the experimental and theoretical results indicate that there are hydrogen bonding of C–H···Br and weak van der Waals interactions between [C20H20P]+ and [MnBr4]2–, resulting in the root for the realization of ultrafast self-assembly in 0D Mn2+-based halides. This work reveals a feasible and general synthesis method for preparing 0D Mn2+-based halides, thereby providing a possibility for their industrial application in solid-state displays.
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