Библиотека института физики им. Л.В. Киренского СО РАН

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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Platunov M. S., Dudnikov V. A., Orlov Yu. S., Kazak N. V., Solovyov L. A., Zubavichus Y. V., Veligzhanin A. A., Dorovatovskii P. V., Vereshchagin S. N., Shaykhutdinov K. A., Ovchinnikov S. G.
Заглавие : Crystal structure and electronic states of Co and Gd ions in a Gd0.4Sr0.6CoO2.85 single crystal
Коллективы : Russian Foundation for Basic Research [13-02-00958, 13-02-00358, 14-02-31051, 16-32-60049]; Council of the President of the Russian Federation for Support of Young Scientists and Leading Scientific Schools [SP-938.2015.5]; program "UMNIK"; Siberian Branch, Russian Academy of Sciences [V.45.3.1]
Место публикации : JETP Letters. - 2016. - Vol. 103, Is. 3. - P.196-200. - ISSN 0021-3640, DOI 10.1134/S0021364016030139. - ISSN 1090-6487(eISSN)
Примечания : Cited References:20. - This work was supported in part by the Russian Foundation for Basic Research (project nos. 13-02-00958, 13-02-00358, 14-02-31051, and 16-32-60049), by the Council of the President of the Russian Federation for Support of Young Scientists and Leading Scientific Schools (project no. SP-938.2015.5), and by the program "UMNIK." The X-ray diffraction and thermochemical studies were supported by the Siberian Branch, Russian Academy of Sciences (project no. V.45.3.1).
Предметные рубрики: X-RAY-ABSORPTION
PROFILE REFINEMENT
PEROVSKITE
CHARGE
SPIN
Аннотация: X-ray diffraction and X-ray absorption near edge structure (XANES) spectra have been measured at the Со K-edge and Gd L3-edge in GdCoO3 and Gd0.4Sr0.6CoO2.85 cobaltites. The effect of Sr substitution on the crystal structure and electronic and magnetic states of Co3+ ions in a Gd0.4Sr0.6CoO2.85 single crystal has been analyzed. The XANES measurements at the Co K-edge have not showed a noticeable shift of the absorption edge with an increase in the concentration of Sr. This indicates that the effective valence of cobalt does not change. An increase in the intensity of absorption at the Gd L3-edge is due to an increase in the degree of hybridization of the Gd(5d) and O(2p) states. The effect of hole doping on the magnetic properties results in the appearance of the ferromagnetic component and in a significant increase in the magnetic moment.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Dzebisashvili D. M., Klyuchantsev, Andrey B.
Заглавие : London Penetration Depth as a Test of Order Parameter Symmetry in Sodium Cobaltate Superconductors
Коллективы : Russian Foundation for Basic Research (RFBR) [18-02-00837]; Presidium of the Russian Academy of Sciences [12]
Место публикации : Symmetry-Basel. - 2019. - Vol. 11, Is. 5. - Ст.633. - ISSN 2073-8994, DOI 10.3390/sym11050633
Примечания : Cited References: 43. - The work was financially supported by the Russian Foundation for Basic Research (RFBR) (project no. 18-02-00837) and by the program of the Presidium of the Russian Academy of Sciences No. 12 "Fundamental problems of high-temperature superconductivity".
Предметные рубрики: SPIN
DEPENDENCE
POWDER
CHARGE
PHASE
GAP
Аннотация: Temperature dependence of the magnetic field penetration depth λ was calculated for water intercalated sodium cobaltate superconductor NaxCoO2⋅yH2O. Assuming that the system is in the chiral d+id–wave superconducting state, it was shown that the shifting of the excitation spectrum nodal points off the normal phase Fermi surface due to variation of the sodium content x changes the functional form of the temperature dependence of λ−2 from exponential to linear in the low temperatures region. It is argued that this change in the functional form of T–dependence of the λ−2 can serve as a proof for the chiral symmetry of the superconducting order parameter in the sodium cobaltate.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ovchinnikov S. G., Orlov Y. S., Nekrasov I. A., Pchelkina Z. V.
Заглавие : Electronic structure, magnetic properties, and mechanism of the insulator-metal transition in LaCoO3 taking into account strong electron correlations
Разночтения заглавия :авие SCOPUS: Electronic structure, magnetic properties, and mechanism of the insulator-metal transition in LaCoO 3 taking into account strong electron correlations
Место публикации : J. Exp. Theor. Phys.: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2011. - Vol. 112, Is. 1. - P140-151. - ISSN 1063-7761, DOI 10.1134/S1063776110061159
Примечания : Cited References: 36. - This study was supported financially by the Siberian and Ural Branches of the Russian Academy of Sciences (Integration Project no. 40), Department of Physics of the Russian Academy of Sciences (Program 2.3), Russian Foundation for Basic Research (Project nos. 09-02-00171-a and 10-02-00251), and Noncommercial "Dynasty" Foundation.
Предметные рубрики: SPIN-STATE TRANSITION
CHARGE
Ключевые слова (''Своб.индексиров.''): energy spectra--excited energy level--finite temperatures--gap state--gap widths--high temperature--high-temperature anomalies--insulator metal transition--pauli contribution--spin crossovers--strong electron correlations--temperature dependence--total magnetization--cobalt compounds--density functional theory--electron correlations--electron density measurement--electronic properties--electronic structure--magnetic susceptibility--semiconductor insulator boundaries--spectroscopy--metal insulator transition
Аннотация: The electronic structure of LaCoO3 at finite temperatures is calculated using the LDA+GTB method taking into account strong electron correlations and possible spin crossover upon an increase in temperature. Gap states revealed in the energy spectrum of LaCoO3 reduce the dielectric gap width upon heating; this allowed us to describe the insulator-metal transition observed in this compound at T = 500-600 K. The temperature dependence of the magnetic susceptibility with a peak at T a parts per thousand 100 K is explained by the Curie contribution from thermally excited energy levels of the Co3+ ion. At high temperatures, the Pauli contribution from a band electron is added and the total magnetization of LaCoO3 is considered as the sum M (tot) = M (loc) + M (band). The second term describes the band contribution appearing as a result of the insulator-metal transition and facilitating the emergence of a high-temperature anomaly in the magnetic susceptibility of LaCoO3.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Orlov Y. S., Ovchinnikov S. G.
Заглавие : Construction of a Multielectron Basis for Mott Insulators with Strong Electron Correlations, Spin-Orbit Interaction, and Covalence
Место публикации : J. Exp. Theor. Phys. - 2009. - Vol. 109, Is. 2. - P.322-338. - ISSN 1063-7761, DOI 10.1134/S1063776109080196
Примечания : Cited References: 35
Предметные рубрики: NARROW ENERGY BANDS
MAGNETIC ANISOTROPY ENERGY
ORIGIN
TRANSITION
PHYSICS
MANGANITES
OXIDES
CHARGE
Аннотация: We propose that the apparatus of quantum mechanics of a free atom (in particular, the theory of nj symbols and Rakah-Wigner genealogic coefficients generalized to the case of point groups and widely used in crystal field theory) be used for constructing multielectron bases with allowance for covalence and spin-orbit interaction. This allows us to take into account the electron-electron interaction for 3d ions the most comprehensively. The basis constructed in this way can be used in the generalized strong coupling method for the multiband p-d model in describing the structure of the quasiparticle energy spectrum and physical properties of systems with strong electron correlations. The procedure of construction and computation is demonstrated for the (5)T(2g) term in the d(6) configuration of the transition metal atom in an octahedral field. The mechanism for the emergence of magnetic anisotropy in S ions (Fe(3+) and Mn(2+)) due to covalent mixing of d(6) (L) under bar configurations with a nonzero orbital angular momentum ((L) under bar is a hole in ligands) is demonstrated
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ovchinnikov S. G., Orlov Yu.S., Dudnikov V. A.
Заглавие : Temperature and field dependent electronic structure and magnetic properties of LaCoO3 and GdCoO3
Коллективы : Moscow International Symposium on Magnetism
Место публикации : J. Magn. Magn. Mater./ Moscow international symposium on magnetism (5 ; 2011 ; 21–25 aug. ; Moscow): Elsevier Science BV, 2012. - Vol. 324, Is. 21. - P.3584-3587. - ISSN 0304-8853, DOI 10.1016/j.jmmm.2012.02.096
Примечания : Cited References: 25. - We acknowledge discussions with G.A. Sawatzky, M.W. Haverkort, S.V. Nikolaev and V.A. Gavrichkov. This work is supported by the Siberia-Urals integration project no. 44, SBRAS project no. 38, Presidium RAS Program 20, RFBR Grant no. 10-02-00251.
Предметные рубрики: SPIN-STATE TRANSITION
CHARGE
Ключевые слова (''Своб.индексиров.''): electronic structure--spin crossover--insulator-metal transition
Аннотация: The transformation of the band structure of LaCoO3 in the applied magnetic field has been theoretically studied. If the field is below its critical value B-C approximate to 65 T, the dielectric band gap decreases with the field, thus giving rise to negative magnetoresistance that is highest at T approximate to 300 divided by 500 K. The critical field is related to the crossover between the low- and high-spin terms of Co3+ ions. The spin crossover results in an insulator-metal transition induced by an increase in the magnetic field. Similar calculations have been done for GdCoO3 which is characterized by large spin gap similar to 2000K. (C) 2012 Elsevier B.V. All rights reserved.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Val'kov V. V., Golovnya A. A., Korovushkin M. M.
Заглавие : Kinematic mechanism of the modulation of the spectral intensity in the spatially uniform system of Hubbard fermions
Место публикации : JETP Letters. - 2011. - Vol. 94, Is. 3. - P.197-201. - ISSN 0021-3640, DOI 10.1134/S0021364011150148
Примечания : Cited References: 21. - We are grateful to R.O. Zaitsev and N.M. Plakida for the constructive criticism and helpful discussions. This work was supported by the Presidium of the Russian Academy of Sciences (program "Quantum Physics of Condensed Matter"), the Russian Foundation for Basic Research (project no. 09-02-00127), the Ministry of Education and Science of the Russian Federation (federal program "Scientific and Pedagogical Personnel of Innovative Russia" for 2009-2013), and the Siberian Branch, the Russian Academy of Sciences (integration project no. 53). The work of A.A.G. and M.M.K. was also supported by the Council of the President of the Russian Federation for Support of Young Scientists and Leading Scientific Schools (grant no. MK-1300-2011.2) and by the Siberian Branch, Russian Academy of Sciences (Lavrent'ev Competition).
Предметные рубрики: SPIN SUSCEPTIBILITY
ANTIFERROMAGNETS
DYNAMICS
CHARGE
MODEL
Аннотация: Using the exact representation of the Green's function constructed in terms of the Hubbard operators, it has been shown that the kinematic interaction that induces the spin-fluctuation processes in the spatially uniform system of Hubbard fermions leads to significant variations in the spectral intensity A(k, omega) in the Brillouin zone. As a result, the modulation of A(k, omega) appears in the Fermi contour. The sign of the hopping integral within the first coordination sphere is determined by the contour section, where A(k, omega) decreases according to the angle-resolved photoemission spectroscopy data.
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