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Zobov, V. E.
Second moment of multiple-quantum NMR and a time-dependent growth of the number of multispin correlations in solids / V. E. Zobov, A. A. Lundin // J. Exp. Theor. Phys. - 2006. - Vol. 103, Is. 6. - P. 904-916, DOI 10.1134/S1063776106120089. - Cited References: 39 . - ISSN 1063-7761

РУБ Physics, Multidisciplinary
Рубрики:
NUCLEAR-MAGNETIC-RESONANCE
   LINE-SHAPE
   SPIN SYSTEMS
   DYNAMICS
   SPECTRA
   COHERENCES
   STATE
   BEHAVIOR
   CRYSTAL
   MODEL
Кл.слова (ненормированные):
Correlation methods -- Mathematical models -- Nuclear magnetic resonance spectroscopy -- Spectrum analysis -- Time series analysis -- Four-spin time correlation -- Multispin correlations -- Second moment -- Time power series -- Quantum theory
Аннотация: The time evolution of multispin correlations (the growth of the number of correlated spins as a function of time) can be observed directly using the multiple-quantum nuclear magnetic resonance spectroscopy of solids. A quantity related to this number, namely, the second moment of the intensity distribution of coherences of different orders in the multiple-quantum spectrum can be calculated using the theory proposed in this work. An approach to the calculation of the four-spin time correlation function through which this moment is expressed is developed. The main sequences of contributions in the expansion of this function into a time power series are summed using the approximation of a large number of neighbors both for systems with a secular dipole-dipole interaction and for systems with a nonsecular effective interaction. An exponential dependence of is obtained. The value of is additionally calculated using an expansion in terms of orthogonal operators for three model examples corresponding to different limiting realizations of spin systems. It is shown that the results of the microscopic theory at least qualitatively agree with both the results obtained for model examples and experimental results obtained recently for adamantane.

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Держатели документа:
Russian Acad Sci, Siberian Div, Kirenskii Inst Phys, Krasnoyarsk 660036, Russia
Russian Acad Sci, Semenov Inst Chem Phys, Moscow 117977, Russia
ИФ СО РАН
Kirenskii Institute of Physics, Siberian Division, Russian Academy of Sciences, Krasnoyarsk, 660036, Russian Federation
Semenov Institute of Chemical Physics, Russian Academy of Sciences, Moscow, 117977, Russian Federation

Доп.точки доступа:
Lundin, A. A.; Зобов, Владимир Евгеньевич
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    Zobov, V. E.
    Reversible and Irreversible propagation of quantum information and its manifestation in multiple-quantum NMR spectra in solids / V. E. Zobov, A. A. Lundin // J. Exp. Theor. Phys. - 2020. - Vol. 131, Is. 2. - P. 273-279, DOI 10.1134/S1063776120060096. - Cited References: 33. - This work was supported by the Ministry of Science and Higher Education of the Russian Federation within the State Task 0082-2019-0001 (State Registration Number AAAA-A19-119012890064-7) . - ISSN 1063-7761. - ISSN 1090-6509
Рубрики:
DYNAMICS
   LOCALIZATION
   SIMULATIONS
   COHERENCES
Аннотация: On the basis of the earlier developed statistical theory of the growth of the effective size of correlated clusters (the number of correlated spins), an expression for the shape of the multiple-quantum (MQ) NMR spectrum is obtained that takes into account the loss of coherence in a spin system due, for example, to the controlled intervention of the experimenter. It is shown that the scrambling and decoherence processes in the MQ spectrum of the multiparticle system of a solid are not separated, unlike the corresponding spectra of some large isolated molecules [27] in a solution. The relations obtained allow one to extract the necessary information about the above processes (scrambling and decoherence) from the dependence of the MQ spectra on experimental parameters.

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Публикация на русском языке Зобов, Владимир Евгеньевич. Обратимое и необратимое распространение квантовой информации и проявление его в спектрах многоквантового ЯМР в твердом теле [Текст] / В. Е. Зобов, А. А. Лундин // Журн. эксперим. и теор. физ. - 2020. - Т. 158 Вып. 2. - С. 300-308

Держатели документа:
RAS, Fed Res Ctr, Kirensky Inst Phys, KSC,SB, Krasnoyarsk 660036, Russia.
Russian Acad Sci, Semenov Inst Chem Phys, Moscow 117977, Russia.

Доп.точки доступа:
Lundin, A. A.; Зобов, Владимир Евгеньевич; Ministry of Science and Higher Education of the Russian Federation [0082-2019-0001, AAAA-A19-119012890064-7]
}
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    Zobov, V. E.
    On the control of the spread of quantum information in multiple quantum NMR spectroscopy of solids / V. E. Zobov, A. A. Lundin // Proceedings of the International Conference "Micro- and Nanoelectronics – 2021". ICMNE – 2021 : book of abstracts : Oct. 4-8, 2021, Moscow - Zvenigorod, Russia. - 2021. - Ст. q3-02. - P. 149. - Cited References: 5
   Перевод заглавия: О контроле распространением квантовой информации в многоквантовой ЯМР спектроскопии твердых тел

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Доп.точки доступа:
Lundin, A. A.; Лундин, Андрей Арнольдович; Зобов, Владимир Евгеньевич; "Micro- and Nano-Electronics", International Conference(2021 ; Oct. ; Zvenigorod); "Микро- и наноэлектроника", международная конференция(2021 ; окт. ; Звенигород); Квантовая информатика, симпозиум(2021 ; окт. ; Звенигород)Российская академия наук; Физико-технологический институт имени К.А. Валиева РАН
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    Zobov, V. E.
    Nonequidistant multipulse sequence for study of slow atomic motions in solids // Proceedings of the 1st soviet-indian symposium on actual problems of magnetic resonance spectroscopy of inorganic materials. - Dushanbe, 1982. - P. 204-205. - Библиогр.: 5
   Перевод заглавия: Тезисы докладов I советско-индийского симпозиума "Актуальные проблемы магнитной резонансной спектроскопии неорганических материалов"

Держатели документа:
Институт физики им. А.В. Киренского СО РАН

Доп.точки доступа:
Moskvich, Yu. N.; Москвич, Юрий Николаевич; Ponomarenko, A. V.; Пономаренко, Александр Валентинович; Зобов, Владимир Евгеньевич; Soviet-indian symposium on actual problems of magnetic resonance spectroscopy of inorganic materials(1 ; 1982 ; Sept. 29-Oct. 2 ; Dushanbe); Академия наук СССР; Indian national academy of sciences; Академия наук Таджикской ССР
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Zobov, V. E.
Multiple-quantum NMR spectroscopy and quantum information spreading control in the spin systems of solids / V. E. Zobov, A. A. Lundin // J. Exp. Theor. Phys. - 2022. - Vol. 135, Is. 5. - P. 752-761, DOI 10.1134/S1063776122110139. - Cited References: 49. - This work was supported within the State assignment of the Ministry of Science and Higher Education of the Russian Federation (registration number 1021051201992-1) . - ISSN 1063-7761. - ISSN 1090-6509
Аннотация: Multiple-quantum (MQ) solid-state NMR spectroscopy allows the growth of multiple-spin correlations and, thus, the spreading of quantum information in the object under study to be observed. Recently, in [11] it was proposed to control this process through a controlled perturbation added to the effective Hamiltonian that causes degradation of correlated spin clusters with a rate determined by the number of spins K in a cluster. However, this perturbation can also lead to degradation whose rate is determined by the coherence order M. In this paper, to investigate the influence of a small added perturbation, we used an expansion into orthogonal operators that allowed the cluster size distribution to be taken into account. In our calculations we realized a simple model with known amplitudes of the expansion into a complete set of orthogonal operators in the absence of a perturbation. We performed numerical calculations of the “preparation time” dependences of the MQ spectra, their second moments, and the coherence orders at which the MQ spectra decrease by a factor of e as well as the average correlated spin cluster sizes K¯. The coherence-order-dependent contribution to the degradation is shown to change the shape of the MQ spectrum. In particular, as the preparation time increases, the MQ spectrum can be stabilized, while the growth of K¯ is retained. Due to the change in the shape of the MQ spectrum, the relations of its characteristics to the number K¯ change compared to those for the Gaussian function (traditionally used to process the experiments). These changes should be taken into account when studying the spreading of quantum information through MQ spectroscopy.

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Публикация на русском языке Зобов, Владимир Евгеньевич. Многоквантовая ЯМР-спектроскопия и управление распространением квантовой информации в спиновых системах твердых тел [Текст] / В. Е. Зобов, А. А. Лундин // Журн. эксперим. и теор. физ. - 2022. - Т. 162 Вып. 5. - С. 778-789

Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, 660036, Krasnoyarsk, Russia
Semenov Federal Research Center for Chemical Physics, Russian Academy of Sciences, 117977, Moscow, Russia

Доп.точки доступа:
Lundin, A. A.; Зобов, Владимир Евгеньевич
}
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Zobov, V. E.
Effect of intramolecular interaction on time growth of second moment of multiple quantum NMR in solids / V. E. Zobov, A. A. Lundin // INTERNATIONAL CONFERENCE ON RESONANCES IN CONDENSED MATTER: ALTSHULER100. Ser. Journal of Physics Conference Series : IOP PUBLISHING LTD, 2011. - Vol. 324: International Conference on Resonances in Condensed Matter (JUN 21-25, 2011, Kazan, RUSSIA). - Ст. 12010, DOI 10.1088/1742-6596/324/1/012010. - Cited References: 12 . - ISBN 1742-6588

РУБ Physics, Condensed Matter
Рубрики:
COHERENCES
DYNAMICS
Кл.слова (ненормированные):
Dipole dipole interactions -- Double-quantum -- Intramolecular interactions -- Multiple quantum NMR -- Nuclear spin system -- Quantum spectrum -- Rate increase -- Second moments -- Solids containing methyl groups -- Time dependence -- Functional groups -- Quantum optics -- Solids -- Spin dynamics -- Hamiltonians
Аннотация: The time dependence of the NMR multiple quantum spectrum in solids containing methyl groups is investigated. We studied both of types of the nuclear spin systems: namely linking by secular part of the mutual dipole-dipole interaction and linking by effective double quantum Hamiltonian. It is revealed for the first type of systems the rate with the time of the growing up of the second moment when intramolecular interaction is present becomes less in compare with situation when a strong intramolecular interaction is absent. On the contrary for the second type of Hamiltonian the above rate increases.

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Держатели документа:
[Zobov, V. E.] Russian Acad Sci, LV Kirensky Phys Inst, Siberian Branch, Krasnoyarsk 660036, Russia
ИФ СО РАН
L.V. Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences, 660036, Krasnoyarsk, Russian Federation
N.N. Semenov Institute of Chemical Physics, RAS, 117977, Moscow, Russian Federation

Доп.точки доступа:
Lundin, A. A.; Зобов, Владимир Евгеньевич
}
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    Zobov, V. E.
    Effect of degradation processes caused by a small perturbation on the growth of the average cluster size of correlated spins in multiple quantum NMR spectroscopy of solids / V. E. Zobov, A. A. Lundin // Appl. Magn. Reson. - 2021. - Vol. 52. Is. 7. - P. 879–892, DOI 10.1007/s00723-021-01342-1. - Cited References: 33. - The study is funded by the Ministry of Science and Higher Education of the Russian Federation in the framework of the State assignment, State registration number AAAA-A19-119012890064-7 . - ISSN 0937-9347
   Перевод заглавия: Влияние процессов деградации, вызванных малым возмущением, на рост среднего размера кластера коррелированных спинов в многоквантовой ЯМР спектроскопии твердых тел
Кл.слова (ненормированные):
Nuclear magnetic resonance spectroscopy -- Average size -- Cluster sizes -- Degradation process -- Multiple quantum NMR spectroscopy -- Orthogonal operators -- Over-complete -- Small perturbations -- Velocity ratio -- Cluster analysis
Аннотация: Multiple quantum (MQ) NMR spectroscopy of solids allows one to observe the growth and decay of multispin correlations. As a rule, the average size of the cluster of correlated spins is extracted from the width of the MQ spectrum. In the present article, the size distribution of such clusters is explored. To obtain the above distribution, the solutions for the amplitudes of the decomposition over complete sets of orthogonal operators for the two different models were used. By means of these models, we have taken into account the dependence of cluster degradation (the degradation of a cluster means, e.g., destruction of correlations in cluster or loss of particles in it) through two positions. The first one defines by the cluster size while the second one depends on the MQ coherence order of the cluster. It is shown that in dependence of the relation the rates of these degradation processes, the width of the MQ spectrum carries different information. If the first process is faster that the second one, then the width of the MQ spectrum is still determined by the average cluster size. When the velocity ratio becomes inverse, the width of the MQ spectrum takes on a smaller value, which is a consequence of the faster degradation of the MQ spectrum components with large orders of coherence.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Semenov Institute of Chemical Physics, Russian Academy of Sciences, Moscow, 117977, Russian Federation

Доп.точки доступа:
Lundin, A. A.; Зобов, Владимир Евгеньевич
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Zhandun, V. S.
Lattice dynamics, ferroelectric and antiferroeelctric instabilities, and the ferroelectric phase transition in disordered PbB(1/2)' B(1/2)'' O(3) (B ' = Ga, In, Lu; B '' = Nb, Ta) solid solutions / V. S. Zhandun, N. G. Zamkova, V. I. Zinenko // J. Exp. Theor. Phys. - 2008. - Vol. 106, Is. 6. - P. 1109-1117, DOI 10.1134/S1063776108060101. - Cited References: 29 . - ISSN 1063-7761

РУБ Physics, Multidisciplinary
Рубрики:
STATISTICAL-MECHANICS
   PEROVSKITES
   CRYSTALS
   ORDER
   RELAXOR
   BATIO3
   PBTIO3
Кл.слова (ненормированные):
Crystal lattices -- Ferroelectricity -- Lattice vibrations -- Solids -- Ferroelectric (barium strontium titanate) -- Ferroelectric phase transitions -- Lattice (CO) -- Lattice dynamics -- Vibration spectrum -- Ferroelectric materials
Аннотация: The lattice vibration spectra, rf permittivity, and dynamic Born charges of disordered PbB(1/2)'B(1/2)'' O(3) (B' = Ga, In, Lu; B '' = Nb, Ta) solid solutions are calculated in terms of the generalized Gordon-Kim model. All the compounds are found to have soft modes related to the center (Gamma(15)) and boundary point R (R(15)) of the Brillouin zone; the frequencies of these modes are close. The ferroelectric phase transition temperatures and the spontaneous polarization in the ferroelectric phase are calculated for the solid solutions using a model Hamiltonian in the local mode approximation and the Monte Carlo method. These temperatures for the tantalum compounds are found to be higher than for the niobium compounds, and temperature t(s) increases with the atomic number of ion B'. A model where the antiferroelectric state is related to the condensation of modes Gamma(15) and R(15) is proposed. It is found that, for all compounds except for PbSc(1/2)Nb(1/2)O(3) and PbSc(1/2)Ta(1/2)O(3), the ferroelectric phase, which is only related to the condensation of mode R(15), and the antiferroelectric phase have similar energies. In PbIn(1/2)Ta(1/2)O(3), the antiferroelectric phase turns out to be energetically favorable.

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Держатели документа:
[Zhandun, V. S.
Zamkova, N. G.
Zinenko, V. I.] Russian Acad Sci, LV Kirensky Phys Inst, Siberian Branch, Krasnoyarsk 660036, Russia
ИФ СО РАН
Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences, Krasnoyarsk 660036, Russian Federation

Доп.точки доступа:
Zamkova, N. G.; Замкова, Наталья Геннадьевна; Zinenko, V. I.; Зиненко, Виктор Иванович; Жандун, Вячеслав Сергеевич
}
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    Vorotynov, A. M.
    Uniaxial and basal plane anisotropy caused by Cr2+ impurity ions in CrBO3 crystals / A. M. Vorotynov, S. G. Ovchinnikov, V. V. Rudenko // J. Phys. Chem. Solids. - 2018. - Vol. 123. - P. 389-392, DOI 10.1016/j.jpcs.2018.08.016. - Cited References: 14 . - ISSN 0022-3697
   Перевод заглавия: Одноосная и базисная анизотропия вызванная примесью ионов Cr2+ в кристаллах CrBO3
Кл.слова (ненормированные):
Anisotropy -- Chromium compounds -- Crystal impurities -- Ions -- Single crystals
Аннотация: IIn this study, the uniaxial and basal anisotropy governed by Cr2+ impurity ions was treated based on the Cr2+– BO3 3− ion vacancy model using single ion approximation. The anomalous behavior of the basal anisotropy at low temperatures was predicted.

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Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Russian Federation

Доп.точки доступа:
Ovchinnikov, S. G.; Овчинников, Сергей Геннадьевич; Rudenko, V. V.; Руденко, Валерий Васильевич; Воротынов, Александр Михайлович
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10.

Val'kov, V. V.
Energy structure of high-temperature superconductors with the intersite Coulomb interaction / V. V. Val'kov, M. M. Korovushkin // Eur. Phys. J. B. - 2009. - Vol. 69, Is. 2. - P. 219-227, DOI 10.1140/epjb/e2009-00141-4. - Cited References: 26. - This study was supported by the program "Quantum physics of condensed matter"of the Presidium of the Russian Academy of Sciences (RAS); the Russian Foundation for Basic Research (project no. 07-02-00226); the Siberian Branch of RAS (Interdisciplinary Integration project no. 53). One of authors (M. K.) would like to acknowledge the support of the Dynasty Foundation. . - ISSN 1434-6028

РУБ Physics, Condensed Matter
Рубрики:
HIGH-TC SUPERCONDUCTIVITY
   SINGLE-BAND
   ELECTRON CORRELATIONS
   CU OXIDES
   J MODEL
   DERIVATION
Кл.слова (ненормированные):
Strongly correlated electron systems; heavy fermions -- Narrow-band systems; intermediate-valence solids -- Cuprate superconductors -- Strongly correlated electron systems heavy fermions -- Narrow-band systems intermediate-valence solids -- Cuprate superconductors -- Emery model -- Energy structures -- Fermi state -- Integrated density -- Root mean squares -- Spectral intensity -- Copper compounds -- Corundum -- Coulomb interactions -- Electrons -- Fermions -- High temperature superconductors -- Oxide superconductors -- Superconductivity
Аннотация: The effect of the intersite Coulomb interaction of fermions on the ground state and energy structure of high-temperature superconductors is considered within the three-band Emery model using an extended basis of the irreducible operators orthogonal on Mori. The proposed theory allows prediction of bands of the fluctuation states whose spectral intensity grows with an increase in the root-mean-square fluctuations of the occupation numbers. The increase in these fluctuations in high-temperature superconductors upon doping plays a key role in redistribution of the integrated density of the Fermi states.

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Держатели документа:
[Val'kov, V. V.
Korovushkin, M. M.] RAS, Siberian Branch, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
[Val'kov, V. V.] Siberian Fed Univ, Krasnoyarsk 660041, Russia
ИФ СО РАН
L.V. Kirensky Institute of Physics, Siberian Branch, RAS, Krasnoyarsk 660036, Russian Federation
Siberian Federal University, Krasnoyarsk 660041, Russian Federation

Доп.точки доступа:
Korovushkin, M. M.; Коровушкин, Максим Михайлович; Вальков, Валерий Владимирович; Russian Academy of Sciences; Russian Foundation for Basic Research [07-02-00226]; RAS; Dynasty Foundation
}
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