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    State-of-art plasmonic photonic crystals based on self-assembled nanostructures / A. Yadav, N. Yadav, V. Agrawal [et al.] // J. Mater. Chem. C. - 2021. - Vol. 9, Is. 10. - P. 3368-3383, DOI 10.1039/d0tc05254j. - Cited References: 127. - All the authors acknowledge the respective department for providing facilities and resources. We acknowledge funding support from Taishan Scholar scheme of Shandong Province, China (ts 20190401). SPP and SVK acknowledge support of the Ministry of Science and Higher Education of Russian Federation, project no. FSRZ-2020-0008 . - ISSN 2050-7526. - ISSN 2050-7534
   Перевод заглавия: Плазмонные фотонные кристаллы на основе самоорганизующихся наноструктур: современное состояние проблемы

РУБ Materials Science, Multidisciplinary + Physics, Applied

Аннотация: Controlled self-assembly of plasmonic photonic nanostructures provides a cost-effective and efficient methodology to expand plasmonic photonic nano-platforms with unique, tunable, and coupled optical characteristics. Keeping advantages and challenges in view, this review highlights contemporary advancements towards the development of self-assembly of a plasmonic photonic nanostructure using a colloidal solution and a self-assembly modeling technique along with exploring novel optical properties and associated prospects. The potential applications of self-assembled plasmonic photonic nano-systems to investigate next-generation optoelectronic devices, the need to reduce and increase scaling up aspects, and improve the performance, are also covered briefly in the review. The need of considerable efforts for the design and development towards establishing novel cost-effective methods to fabricate controlled self-assembled smart nano-plasmonic platforms is also highlighted in this mini-review. Key confronting issues that precisely limit the self-assemblies of photonic nanostructures and desired integration with other device components, mainly including uniformity within miniaturized devices are also discussed. This review will serve as a guideline and platform to plan advanced research in developing self-assembled plasmonic photonic nano-systems to investigate smart functional optical devices.

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Держатели документа:
Shandong Univ Technol, Ctr Adv Laser Mfg CALM, Zibo 255000, Peoples R China.
Southeast Univ, Sch Phys, Nanjing 211189, Peoples R China.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Krasnoyarsk 660036, Russia.
Bundelkhand Inst Engn & Technol, Dept Appl Sci, Jhansi, Uttar Pradesh, India.
Natl Univ Singapore, Nanosci & Nanotechnol Initiat, 10 Kent Ridge, Singapore 119260, Singapore.

Доп.точки доступа:
Yadav, A.; Yadav, N.; Agrawal, V.; Polyutov, S. P.; Tsipotan, A. S.; Karpov, S. V.; Карпов, Сергей Васильевич; Slabko, V. V.; Yadav, V. S.; Wu, Y. L.; Zheng, H. Y.; RamaKrishna, S.; Taishan Scholar scheme of Shandong Province, China [20190401]; Ministry of Science and Higher Education of Russian Federation [FSRZ-2020-0008]
}
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    Plasmonic lattice Kerker effect in ultraviolet-visible spectral range / V. S. Gerasimov, A. E. Ershov, R. G. Bikbaev [et al.] // Phys. Rev. B. - 2021. - Vol. 103, Is. 3. - Ст. 035402, DOI 10.1103/PhysRevB.103.035402. - Cited References: 66. - The research was supported by the Ministry of Science and High Education of Russian Federation, Project No. FSRZ-2020-0008, by RFBR, Krasnoyarsk Territory and Krasnoyarsk Regional Fund of Science, project number 20-42-240003 and by the Russian Science Foundation (Project No. 18-13-00363) (numerical calculations of phase dependences and corresponding research), A. E. acknowledges the grant of the President of the Russian Federation, agreement No. 075–15–2019–676 . - ISSN 2469-9950
   Перевод заглавия: Эффект Керкера на плазмонной решетке в ультрафиолетовой и видимой области спектра
Кл.слова (ненормированные):
Aluminum -- Dielectric materials -- Geometry -- Nanostructures -- Plasmons -- Surface plasmon resonance
Аннотация: Mostly forsaken, but revived after the emergence of all-dielectric nanophotonics, the Kerker effect can be observed in a variety of nanostructures from high-index constituents with strong electric and magnetic Mie resonances. A necessary requirement for the existence of a magnetic response limits the use of generally nonmagnetic conventional plasmonic nanostructures for the Kerker effect. In spite of this, we demonstrate here the emergence of the lattice Kerker effect in regular plasmonic Al nanostructures. Collective lattice oscillations emerging from the delicate interplay between Rayleigh anomalies and localized surface plasmon resonances both of electric and magnetic dipoles, and electric and magnetic quadrupoles result in suppression of the backscattering in a broad spectral range. Variation of geometrical parameters of Al arrays allows for tailoring the lattice Kerker effect throughout UV and visible wavelength ranges, which is close to impossible to achieve using other plasmonic or all-dielectric materials. It is argued that our results set the ground for wide ramifications in the plasmonics and further application of the Kerker effect.

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Держатели документа:
Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Institute of Computational Modelling of the Siberian Branch, Russian Academy of Sciences, Krasnoyarsk, 660036, Russian Federation
L. V. Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Institute of Optics, University of Rochester, Rochester, NY 14627, United States

Доп.точки доступа:
Gerasimov, V. S.; Ershov, A. E.; Bikbaev, R. G.; Бикбаев, Рашид Гельмединович; Rasskazov, I. L.; Isaev, I. L.; Semina, P. N.; Kostyukov, A. S.; Zakomirnyi, V. I.; Polyutov, S. P.; Karpov, S. V.; Карпов, Сергей Васильевич
}
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Thermoelectric and Plasmonic Properties of Metal Nanoparticles Linked by Conductive Molecular Bridges / A. S. Fedorov, P. O. Krasnov, M. A. Visotin [et al.] // Phys. Status Solidi B. - 2020. - Vol. 257, Is. 12. - Ст. 2000249, DOI 10.1002/pssb.202000249. - Cited References: 53. - This study was supported by the Russian Science Foundation, project no. 16-13-00060 (thermoelectric properties), and by the Ministry of Science and High Education of the Russian Federation, project no. FSRZ-2020-0008 (plasmonic properties) . - ISSN 0370-1972. - ISSN 1521-3951

РУБ Physics, Condensed Matter
Рубрики:
POLYMERS
ARRAYS
RANGE
Кл.слова (ненормированные):
charge transfer plasmons -- density functional theory -- nanoparticles -- thermoelectric properties
Аннотация: Thermoelectric and plasmonic properties of systems comprising small golden nanoparticles (NPs) linked by narrow conductive polymer bridges are studied using the original hybrid quantum-classical model. The bridges are considered here to be either conjugated polyacetylene, polypyrrole, or polythiophene chain molecules terminated by thiol groups. The parameters required for the model are obtained using density functional theory and density functional tight-binding simulations. Charge-transfer plasmons in the considered dumbbell structures are found to possess frequency in the infrared region for all considered molecular linkers. The appearance of plasmon vibrations and the existence of charge flow through the conductive molecule, with manifestation of quantum properties, are confirmed using frequency-dependent polarizability calculations implemented in the coupled perturbed Kohn-Sham method. To study the thermoelectric properties of the 1D periodical systems, a universal equation for the Seebeck coefficient is derived. The phonon part of the thermal conductivity for the periodical -NP-S-C8H8- system is calculated by the classical molecular dynamics. The thermoelectric figure of meritZTis calculated by considering the electrical quantum conductivity of the systems in the ballistic regime. It is shown that forAu309nanoparticles connected by polyacetylene, polypyrrole, or polythiophene chains atT = 300 K, the ZTvalue is {0.08;0.45;0.40}, respectively.

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Держатели документа:
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
RAS, Kirensky Inst Phys, KSC, SB, Krasnoyarsk 660036, Russia.
Tomsk State Univ, Tomsk 634050, Russia.

Доп.точки доступа:
Fedorov, A. S.; Федоров, Александр Семенович; Krasnov, Pavel O.; Visotin, M. A.; Высотин, Максим Александрович; Tomilin, F. N.; Томилин, Феликс Николаевич; Polyutov, Sergey P.; Russian Science FoundationRussian Science Foundation (RSF) [16-13-00060]; Ministry of Science and High Education of the Russian Federation; FSRZ-2020-0008 (plasmonic properties)
}
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Substrate-mediated lattice Kerker effect in Al metasurfaces / A. S. Kostyukov, A. E. Ershov, R. G. Bikbaev [et al.] // J. Opt. Soc. Am. B. - 2021. - Vol. 38, Is. 9. - P. C78-C83, DOI 10.1364/JOSAB.427939. - Cited References: 62. - Funding. Russian Foundation for Basic Research, Krasnoyarsk Territory and Krasnoyarsk Regional Fund of Science (20-42-240003); Ministry of Science and Higher Education of the Russian Federation (FSRZ-2020-0008) . - ISSN 0740-3224
Кл.слова (ненормированные):
Plasmonic nanoparticles -- Refractive index -- Half-space environment -- Non-homogeneous -- Regular array -- Sensing applications -- Surface lattice -- Theoretical treatments -- Two-dimensional arrays -- Wavelength ranges -- Geometry
Аннотация: Surface lattice resonances (SLRs) emerging in regular arrays of plasmonic nanoparticles (NPs) are known to be exceptionally sensitive to the homogeneity of the environment. It is considered necessary to have a homogeneous environment for engineering narrowband SLRs, while in a half-space environment, SLRs rapidly vanish as the contrast between the refractive indices of the substrate and superstrate increases. From this conventional wisdom, it is apparent that the delicate lattice Kerker effect emerging from SLRs and resonances on constituent NPs should be difficult to achieve in a non-homogeneous environment. Using a rigorous theoretical treatment with multipolar decomposition, we surprisingly find and explain a narrowband substrate-mediated lattice Kerker effect in two-dimensional arrays of Al nanocylinders in a half-space geometry. We propose to use this effect for sensing applications and demonstrate its broad tunability across the UV/Vis wavelength range.

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Держатели документа:
International Research Center of Spectroscopy and Quantum Chemistry-IRC SQC, Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Institute of Computational Modelling of the Siberian Branch of the Russian Academy of Sciences, Krasnoyarsk, 660036, Russian Federation
L. V. Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
The Institute of Optics, University of Rochester, Rochester, NY 14627, United States

Доп.точки доступа:
Kostyukov, A. S.; Ershov, A. E.; Bikbaev, R. G.; Бикбаев, Рашид Гельмединович; Gerasimov, V. S.; Rasskazov, I. L.; Karpov, S. V.; Карпов, Сергей Васильевич; Polyutov, S. P.
}
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Plasmonic enhancement of local fields in ultrafine metal nanoparticles / L. K. Sorensen, A. D. Utyushev, V. I. Zakomirnyi [et al.] // J. Phys. Chem. C. - 2021. - Vol. 125, Is. 5. - P. 13900-13908, DOI 10.1021/acs.jpcc.1c01424. - Cited References: 65. - The work was supported by the Russian Science Foundation (project no. 18-13-00363). L.K.S acknowledges the support of Carl Tryggers Stifetelse, project CTS 18-441 . - ISSN 1932-7447
Кл.слова (ненормированные):
Crystal structure -- Electric fields -- Electromagnetic fields -- Metal nanoparticles -- Plasmonics -- Discrete interaction -- External fields -- High symmetry -- Metallic nanoparticles -- Nanoscale particles -- Near field imaging -- Optical response -- Plasmon field -- Plasmonic nanoparticles
Аннотация: We present an analysis of ultrafine metallic nanoparticles (1-15 nm) with respect to electromagnetic field generation by plasmonic excitations. A number of structures with different symmetries and geometries are studied in order to analyze the distributions of plasmonically generated near-electric fields and the concentration of hot and cold spots around the particles. The study is made possible by the recent development of an extended discrete interaction model (Ex-DIM) where the explicit dependency of the plasmonic spectra on the structure and composition of particles in the range of 1-15 nm is accounted for. With the Ex-DIM, the optical response of the internal crystal structure of the nanoscale particles can be visualized, thereby making it possible to predict the dependence of the generated local fields with respect to the position of the particles relative to the external field polarization. The results indicate rather surprising concentrations of the plasmon fields in very confined hot spots also in cases when the particles retain a high symmetry. The consequence of the findings of this study when using small symmetric nanoparticles for near-field imaging is briefly discussed.

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Держатели документа:
Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala, SE-751 20, Sweden
Department of Theoretical Chemistry and Biology, School of Engineering Sciences in Chemistry, Biotechnology and Health, Royal Institute of Technology, Stockholm, SE-10691, Sweden
International Research Center of Spectroscopy and Quantum Chemistry, Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Institute of Computational Modelling, Federal Research Center Ksc Sb Ras, Krasnoyarsk, 660036, Russian Federation
L. V. Kirensky Institute of Physics, Federal Research Center Ksc Sb Ras, Krasnoyarsk, 660036, Russian Federation
Federal Siberian Research Clinical Centre under Fmba of Russia, Krasnoyarsk, 660037, Russian Federation

Доп.точки доступа:
Sorensen, L. K.; Utyushev, A. D.; Zakomirnyi, V. I.; Gerasimov, V. S.; Ershov, A. E.; Polyutov, S. P.; Karpov, S. V.; Карпов, Сергей Васильевич; Agren, H.
}
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    Multipolar lattice resonances in plasmonic finite-size metasurfaces / A. S. Kostyukov, I. L. Rasskazov, V. S. Gerasimov [et al.] // Photonics. - 2021. - Vol. 8, Is. 4. - Ст. 109, DOI 10.3390/photonics8040109. - Cited References: 66. - The reported study was funded by the Russian Science Foundation project number 19-72-00066 . - ISSN 2304-6732
   Перевод заглавия: Мультипольные решеточные резонансы в плазмонных метаповерхностях конечных размеров

РУБ Optics

Кл.слова (ненормированные):
lattice resonance -- plasmonics -- multipoles -- nanoparticle
Аннотация: Collective lattice resonances in regular arrays of plasmonic nanoparticles have attracted much attention due to a large number of applications in optics and photonics. Most of the research in this field is concentrated on the electric dipolar lattice resonances, leaving higher-order multipolar lattice resonances in plasmonic nanostructures relatively unexplored. Just a few works report exceptionally high-Q multipolar lattice resonances in plasmonic arrays, but only with infinite extent (i.e., perfectly periodic). In this work, we comprehensively study multipolar collective lattice resonances both in finite and in infinite arrays of Au and Al plasmonic nanoparticles using a rigorous theoretical treatment. It is shown that multipolar lattice resonances in the relatively large (up to 6400 nanoparticles) finite arrays exhibit broader full width at half maximum (FWHM) compared to similar resonances in the infinite arrays. We argue that our results are of particular importance for the practical implementation of multipolar lattice resonances in different photonics applications.

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Держатели документа:
Siberian Fed Univ, Int Res Ctr Spect & Quantum Chem IRC SQC, Krasnoyarsk 660041, Russia.
Univ Rochester, Inst Opt, Rochester, NY 14627 USA.
Russian Acad Sci, Siberian Branch, Inst Computat Modelling, Krasnoyarsk 660036, Russia.
Fed Res Ctr KSC SB RAS, LV Kirensky Inst Phys, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Kostyukov, Artem S.; Rasskazov, Ilia L.; Gerasimov, Valeriy S.; Polyutov, Sergey P.; Karpov, S. V.; Карпов, Сергей Васильевич; Ershov, Alexander E.; Russian Science FoundationRussian Science Foundation (RSF) [19-72-00066]
}
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Extended Discrete Interaction Model: Plasmonic Excitations of Silver Nanoparticles / V. I. Zakomirnyi [et al.] // J. Phys. Chem. C. - 2019. - Vol. 123, Is. 47. - P. 28867-28880, DOI 10.1021/acs.jpcc.9b07410. - Cited References: 64. - H.Å. and V.I.Z. acknowledge the support of the Russian Science Foundation (project no. 18-13-00363). L.K.S. acknowledges the support of Carl Tryggers Stifetelse, project no. CTS 18-441. . - ISSN 1932-7447
Кл.слова (ненормированные):
Aspect ratio -- Geometry -- Nanorods -- Optical properties -- Plasmonics -- Silver nanoparticles
Аннотация: We present a new atomistic model for plasmonic excitations and optical properties of metallic nanoparticles, which collectively describes their complete response in terms of fluctuating dipoles and charges that depend on the local environment and on the morphology of the composite nanoparticles. Being atomically dependent, the total optical properties, the complex polarizability, and the plasmonic excitation of a cluster refer to the detailed composition and geometric characteristics of the cluster, making it possible to explore the role of the material, alloy mixing, size, form shape, aspect ratios, and other geometric factors down to the atomic level and making it useful for the design of plasmonic particles with particular strength and field distribution. The model is parameterized from experimental data and, at present, practically implementable for particles up to more than 10 nm (for nanorods even more), thus covering a significant part of the gap between the scales where pure quantum calculations are possible and where pure classical models based on the bulk dielectric constant apply. We utilized the method to both spherical and cubical clusters along with nanorods where we demonstrate both the size, shape, and ratio dependence of plasmonic excitations and connect this to the geometry of the nanoparticles using the plasmon length.

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Держатели документа:
Department of Theoretical Chemistry and Biology, School of Engineering Sciences in Chemistry, Biotechnology and Health, Royal Institute of Technology, Stockholm, SE-10691, Sweden
Federal Siberian Research Clinical Centre under FMBA of Russia, Kolomenskaya 26, Krasnoyarsk, 660037, Russian Federation
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Department of Physics, Kaunas University of Technology, Kaunas, LT-51368, Lithuania
College of Chemistry and Chemical Engineering, Henan University, Kaifeng, Henan 475004, China

Доп.точки доступа:
Zakomirnyi, V. I.; Закомирный, Вадим Игоревич; Rinkevicius, Z.; Baryshnikov, G. V.; Sorensen, L. K.; Agren, H.
}
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Super-efficient laser hyperthermia of malignant cells with core-shell nanoparticles based on alternative plasmonic materials / A. S. Kostyukov [et al.] // J. Quant. Spectrosc. Radiat. Transf. - 2019. - Vol. 236. - Ст. 106599, DOI 10.1016/j.jqsrt.2019.106599. - Cited References: 57. - The reported study was funded by the RF Ministry of Science and Higher Education , the State contract with Siberian Federal University for scientific research in 2017–2019 (Grant No. 3.8896.2017 ); Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science (Grant No.18-42-243023); A.E. thanks the grant of the President of Russian Federation (agreement 075-15-2019-676 ). . - ISSN 0022-4073
Кл.слова (ненормированные):
Plasmonic photothermal therapy -- Conducting oxides -- Nanoparticle -- Nanoshell
Аннотация: New type of highly absorbing core-shell AZO/Au (aluminum doped zinc oxide/gold) and GZO/Au (gallium doped zinc oxide/gold) nanoparticles have been proposed for hyperthermia of malignant cells purposes. Comparative studies of pulsed laser hyperthermia were performed for Au nanoshells with AZO core and traditional SiO2 (quartz) core. We show that under the same conditions, the hyperthermia efficiency in the case of AZO increases by several orders of magnitude compared to SiO2 due to low heat capacity of AZO. Similar results have been obtained for GZO core which has same heat capacity. Calculations for pico-, nano- and sub-microsecond pulses demonstrate that reduced pulse duration results in strong spatial localization of overheated areas around nanoparticles, which ensures the absence of negative effects to the normal tissue. Moreover, we propose new alternative way for the optimization of hyperthermia efficiency: instead of maximizing the absorption of nanoparticles, we enhance the thermal damage effect on the membrane of malignant cell. This strategy allows to find the parameters of nanoparticle and the incident radiation for the most effective therapy.

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Держатели документа:
Siberian Federal UniversityKrasnoyarsk, Russian Federation
Institute of Computational Modeling SB RASKrasnoyarsk, Russian Federation
Siberian State University of Science and TechnologyKrasnoyarsk, Russian Federation
The Institute of Optics, University of RochesterNY, United States
Kirensky Institute of Physics, Federal Research Center KSC SB RASKrasnoyarsk, Russian Federation

Доп.точки доступа:
Kostyukov, A. S.; Ershov, A. E.; Ершов, Александр Евгеньевич; Gerasimov, V. S.; Герасимов, Валерий Сергеевич; Filimonov, S. A.; Rasskazov, I. L.; Karpov, S. V.; Карпов, Сергей Васильевич
}
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    Engineering mode hybridization in regular arrays of plasmonic nanoparticles embedded in 1D photonic crystal / V. S. Gerasimov [et al.] // J. Quant. Spectrosc. Radiat. Transf. - 2019. - Vol. 224. - P. 303-308, DOI 10.1016/j.jqsrt.2018.11.028. - Cited References: 49. - The reported study was funded by Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science (Grant No.18-42-240013); by the RF Ministry of Science and Higher Education, the State contract with Siberian Federal University for scientific research in 2017–2019 (Grant No.3.8896.2017); by the Russian Science Foundation (Project No. 18-13-00363 ) (numerical calculations of Rayleigh anomalies in planar structures and corresponding research). . - ISSN 0022-4073
   Перевод заглавия: Управляемая гибридизация мод двумерной решетки внедренной в одномерный фотонный кристалл
Кл.слова (ненормированные):
Surface lattice resonance -- Photonic crystal -- Optical cavity
Аннотация: We analytically and numerically study coupling mechanisms between 1D photonic crystal (PhC) and 2D array of plasmonic nanoparticles (NPs) embedded in its defect layer. We introduce general formalism to explain and predict the emergence of PhC-mediated Wood–Rayleigh anomalies, which spectral positions agree well with the results of exact simulations with Finite-Difference Time-Domain (FDTD) method. Electromagnetic coupling between localized surface plasmon resonance (LSPR) and PhC-mediated Wood–Rayleigh anomalies makes it possible to efficiently tailor PhC modes. The understanding of coupling mechanisms in such hybrid system paves a way for optimal design of sensors, light absorbers, modulators and other types of modern photonic devices with controllable optical properties.

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Держатели документа:
Institute of Computational Modeling SB RAS, Krasnoyarsk, 660036, Russian Federation
Institute of Nanotechnology, Spectroscopy and Quantum Chemistry, Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Federal Siberian Research Clinical Centre under FMBA of Russia, Krasnoyarsk, 660037, Russian Federation
Polytechnic Institute, Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
The Institute of Optics, University of Rochester, Rochester, NY 14627, United States
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Siberian State University of Science and Technology, Krasnoyarsk, 660014, Russian Federation

Доп.точки доступа:
Gerasimov, V. S.; Герасимов, Валерий Сергеевич; Ershov, A. E.; Ершов, Александр Евгеньевич; Bikbaev, R. G.; Rasskazov, I. L.; Timofeev, I. V.; Тимофеев, Иван Владимирович; Polyutov, S. P.; Karpov, S. V.; Карпов, Сергей Васильевич
}
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10.

Collective resonances in hybrid photonic-plasmonic nanostructures / A. E. Ershov, R. G. Bikbaev, I. L. Rasskazov [et al.] // J. Phys.: Conf. Ser. - 2020. - Vol. 1461, Is. 1. - Ст. 012046DOI 10.1088/1742-6596/1461/1/012046. - Cited References: 11. - The reported study was funded by Russian Foundation for Basic Research, Government of Krasnoyarsk Territory, Krasnoyarsk Regional Fund of Science (Grant No. 18-42-240013); A.E. thanks the grant of the President of Russian Federation (agreement 075-15-2019-676)
Кл.слова (ненормированные):
Hybrid systems -- Plasmonics -- Time domain analysis -- 1-D photonic crystal -- Defect layers -- Nanodisks -- Periodic arrays -- Plasmonic nanostructures -- Rayleigh anomalies -- Spectral position -- Theoretical modeling -- Finite difference time domain method
Аннотация: We present the theoretical model to predict the spectral position of Rayleigh anomalies emerged in hybrid system consisting of periodic array of plasmonic nanodisks embeded into the middle of defect layer of 1D photonic crystal (PhC). The spectral positions of these new emerged Rayleigh anomalies agree well with the results of exact simulations with Finite-Difference Time-Domain (FDTD) method.

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Держатели документа:
Institute of Computational Modeling SB RAS, Krasnoyarsk, 660036, Russian Federation
Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Siberian State University of Science and Technology, Krasnoyarsk, 660014, Russian Federation
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Institute of Optics, University of Rochester, Rochester, NY 14627, United States

Доп.точки доступа:
Ershov, A. E.; Bikbaev, R. G.; Бикбаев, Рашид Гельмединович; Rasskazov, I. L.; Gerasimov, V. S.; Timofeev, I. V.; Тимофеев, Иван Владимирович; Polyutov, S. P.; Karpov, S. V.; Карпов, Сергей Васильевич; International Conference on Metamaterials and Nanophotonics(4th ; 15 - 19 July 2019 ; St. Petersburg, Russian Federation)
}
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11.

    Processes underlying the laser photochromic effect in colloidal plasmonic nanoparticle aggregates* / A. E. Ershov, V. S. Gerasimov, I. L. Isaev [et al.] // Chin. Phys. B. - 2020. - Vol. 29, Is. 3. - Ст. 037802, DOI 10.1088/1674-1056/ab6551. - Cited References: 38. - Project funded by the Russian Foundation for Basic Research, the Government of the Krasnoyarsk Territory and Krasnoyarsk Regional Fund of Science (Grant 18-42-243023), the RF Ministry of Science and Higher Education, and the State Contract with Siberian Federal University for Scientific Research. A.E. thanks the grant of the President of Russian Federation (agreement 075-15-2019-676). . - ISSN 1674-1056. - ISSN 1741-4199
Рубрики:
SELECTIVE PHOTOMODIFICATION
   LIGHT
   FORCES
   OPTICS
Кл.слова (ненормированные):
nanoparticle -- surface plasmon resonance -- photochromic process -- pulsed laser radiation
Аннотация: We have studied the dynamic and static processes occurring in disordered multiparticle colloidal Ag aggregates with natural structure and affecting their plasmonic absorption spectra under pico- and nanosecond pulsed laser radiations, as well as the physical origin responsible for these processes. We have shown that depending on the duration of the laser pulse, the mechanisms of laser modification of such aggregates can be associated both with changes in the resonant properties of the particles due to their heating and melting (picosecond irradiation mode) and with the particle shifts in the resonant domains of the aggregates (nanosecond pulses) which depend on the wavelength, intensity, and polarization of the radiation. These mechanisms result in formation of a narrow dip in the plasmonic absorption spectrum of the aggregates near the laser radiation wavelength and affect the shape and position of the dip. The effect of polydispersity of nanoparticle aggregates on laser photochromic reaction has been studied.

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Держатели документа:
RAS, SB, Inst Computat Modeling, Krasnoyarsk 660036, Russia.
Siberian Fed Univ, Krasnoyarsk 660041, Russia.
RAS, SB, KSC, Kirensky Inst Phys,Fed Res Ctr, Krasnoyarsk 660036, Russia.
Siberian State Univ Sci & Technol, Krasnoyarsk 660014, Russia.

Доп.точки доступа:
Ershov, A. E.; Gerasimov, V. S.; Isaev, I. L.; Gavrilyuk, A. P.; Karpov, S. V.; Карпов, Сергей Васильевич; Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR); Government of the Krasnoyarsk Territory [18-42-243023]; Krasnoyarsk Regional Fund of Science [18-42-243023]; RF Ministry of Science and Higher Education; Siberian Federal University for Scientific Research; Russian FederationRussian Federation [075-15-2019-676]
}
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12.

Collective resonances in hybrid photonic-plasmonic nanostructures / A. E. Ershov [et al.] // International Conference on Metamaterials and Nanophotonics (METANANO 2019). - St. Petersburg, 2019

Материалы конференции,
Материалы конференции

Доп.точки доступа:
Ershov, A. E.; Ершов, Александр Андреевич; Bikbaev, R. G.; Бикбаев, Рашид Гельмединович; Rasskazov, I. L.; Рассказов, Илья Леонидович; Gerasimov, V. S.; Герасимов, Валерий Сергеевич; Timofeev, I. V.; Тимофеев, Иван Владимирович; Polyutov, S. P.; Karpov, S. V.; Карпов, Сергей Васильевич; International Conference on Metamaterials and Nanophotonics(4 ; 2019 ; July ; 15-19 ; Saint Peresburg); Санкт-Петербургский национальный исследовательский университет информационных технологий, механики и оптики
}
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13.

    Nature of the anomalous size dependence of resonance red shifts in ultrafine plasmonic nanoparticles / L. K. Sorensen, D. E. Khrennikov, V. S. Gerasimov [et al.] // J. Phys. Chem. C. - 2022. - Vol. 126, Is. 39. - P. 16804-16814, DOI 10.1021/acs.jpcc.2c03738. - Cited References: 61. - D.K., V.G., A.E., S.P., and S.K. acknowledge the support by the Russian Science Foundation (project no. 18-13-00363). L.K.S acknowledges the support of Carl Tryggers Stifetelse, project CTS 18-441. The authors also acknowledge the Swedish National Infrastructure for Computing (SNIC) at the High Performance Computing Center North (HPC2N) partially funded by the Swedish Research Council through grant agreement no. 2020/3-29 . - ISSN 1932-7447
   Перевод заглавия: Природа аномальной размерной зависимости резонансных длинноволновых сдвигов в сверхмалых плазмонных наночастицах
Аннотация: Plasmonic red shifts of nanoparticles are commonly used in imaging technologies to probe the character of local environments, and the understanding of their dependence on size, shape, and surrounding media has therefore become an important target for research. The red shift of plasmon resonances changes character at about 8-10 nm of size for spherical gold nanoparticles above this value, the red shift progresses linearly with particle size, while below this size, the red shift changes nonlinearly and more strongly with size. Using an atomistic discrete interaction model, we have studied the special properties of the nanoparticle surface layers and discovered its importance for ultrafine plasmonic nanoparticles and their red shifts. We find that the physical origin for the specific properties inherent to the surface layer of atoms near the nanoparticle boundary is related to the anisotropy of the local environment of atoms in this layer by other atoms. The anisotropy changes the conditions for light-induced nonlocal interactions of neighboring atoms with each other and with the incident radiation compared to the atoms located in the particle core with isotropic nearest surroundings by other atoms. The local anisotropy of the nanoparticle crystal lattice is a geometric factor that increases toward its boundary and that is the most fundamental factor underlying the physical differences between the nanoparticle surface layer and the core material. It is shown that the inflexion point at 8-10 nm is due to a change in the dominant physical origin of the red shift from chaotization of atomically light-induced dipoles within the surface layer in the case of ultrafine nanoparticles to retardation effects for large nanoparticles in which the relative volume of the surface layer decreases rapidly to a negligible value with increasing nanoparticle size. The patterns revealed are the basis for predicting the manifestation of surface layer effects in ultrafine plasmonic nanoparticles of different shapes and composed of different plasmonic materials.

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Держатели документа:
Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala, SE-751 20, Sweden
Department of Theoretical Chemistry and Biology, School of Engineering Sciences in Chemistry, Biotechnology and Health, Royal Institute of Technology, Stockholm, SE-10691, Sweden
University Library, University of Southern Denmark, Odense M, DK-5230, Denmark
International Research Center of Spectroscopy and Quantum Chemistry, Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Federal Research Center KSC SB RAS, Institute of Computational Modelling, Krasnoyarsk, 660036, Russian Federation
Federal Siberian Research Clinical Centre under FMBA of Russia, 26 Krasnoyarsk, Kolomenskaya660037, Russian Federation
Federal Research Center KSC SB RAS, L. V. Kirensky Institute of Physics, Krasnoyarsk, 660036, Russian Federation

Доп.точки доступа:
Sorensen, L. K.; Khrennikov, D. E.; Gerasimov, V. S.; Ershov, A. E.; Polyutov, S. P.; Karpov, S. V.; Карпов, Сергей Васильевич; Agren, H.
}
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14.

    Пятнов, Максим Владимирович.
    Фотоэлектрохимическое расщепление воды наноструктурированным электродом и зеленая водородная энергетика / М. В. Пятнов, И. В. Тимофеев // Фотоника. - 2022. - Т. 16, Вып. 2. - С. 116-125 ; Photonics Rus., DOI 10.22184/1993-7296.FRos.2022.16.2.116.125. - Библиогр.: 28. - Исследование выполнено за счет гранта Российского научного фонда и Красноярского краевого фонда поддержки научной и научно-технической деятельности № 22-22-20078, https://rscf.ru/project/22-22-20078 . - ISSN 1993-7296. - ISSN 2686-844X
   Перевод заглавия: Photoelectrochemical water splitting by a nanostructured electrode and green hydrogen energy
Кл.слова (ненормированные):
плазмонный катализ -- расщепление воды -- фототок -- эффективность преобразования света в водород -- plasmonic catalysis -- water splitting -- photo-induced current -- light-to-hydrogen conversion efficiency
Аннотация: В статье описан перспективный способ получения водорода – фотоэлектрохимическое расщепление воды. Этот подход сочетает непосредственное использование солнечной энергии и низкую стоимость производства фотоэлектрохимических ячеек из широко распространенных на Земле полупроводниковых материалов. Последние достижения в конструировании таких ячеек включают наноструктурирование полупроводниковых электродов плазмонными материалами.
This article describes a promising hydrogen formation method, namely the photoelectrochemical water splitting. This approach combines the direct use of solar energy and low production cost of photoelectrochemical cells using the widely used semiconductor materials. The latest advances in such cell design include nanostructuring of the semiconductor electrodes with plasmonic materials.

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РИНЦ
Держатели документа:
Институт физики им. Л. В. Киренского СО РАН -обособленное подразделение ФИЦ КНЦ СО РАН
Сибирский федеральный университет

Доп.точки доступа:
Тимофеев, Иван Владимирович; Timofeev, I. V.; Pyatnov, M. V.

}
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15.

Plasmonics: Nonlinear optics, negative phase, and transformable transparency / A. K. Popov, S. A. Myslivets, V. M. Shalaev // Proceedings of SPIE - The International Society for Optical Engineering. - 2009. - Vol. 7395. - Ст. 73950Z, DOI 10.1117/12.824836 . - ISBN 0277786X (ISSN); 9780819476852 (ISBN)
Кл.слова (ненормированные):
Backward electromagnetic waves -- Negative-index metamaterials -- Optical parametric amplification -- Quantum control -- Backward electromagnetic waves -- Control fields -- Light wave -- Nanostructured composites -- Negative group velocity -- Negative phase -- Negative-index -- Negative-index metamaterials -- Optical energy transfer -- Optical parametric amplification -- Optical technique -- Plasmonic metamaterials -- Plasmonics -- Quantum control -- Cements -- Electromagnetic wave diffraction -- Electromagnetic wave scattering -- Electromagnetic waves -- Electromagnetism -- Energy transfer -- Light -- Metamaterials -- Nanophotonics -- Nonlinear optics -- Plasmons -- Transparency -- Amplification
Аннотация: The feasibilities and specific features of coherent nonlinear-optical energy transfer from control fields to a negativephase signal are studied, and they are found to stem from the backwardness of electromagnetic waves inherent to negative-index metamaterials. Plasmonic metamaterials that possess negative group velocity for light waves promise a revolutionary breakthrough in nanophotonics. However, strong absorption inherent to such metaldielectric nanocomposites imposes severe limitations on the majority of such applications. Herein we show the feasibility and discuss different nonlinear-optical techniques of compensating such losses, producing transparency, amplification and even generation of negative-phase light waves in originally strongly absorbing microscopic samples of plasmonic metal-dielectric nanostructured composites. © 2009 SPIE.

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Держатели документа:
University of Wisconsin-Stevens Point, 812 Kensington Rd., Neenah, WI 54956, United States
Siberian Federal University, Institute of Physics, Russian Academy of Sciences, 660036 Krasnoyarsk, Russian Federation
Birck Nanotechnology Center, School of Electrical and Computer Engineering, Purdue University, West Lafayette, IN 47907, United States

Доп.точки доступа:
Popov, A.K.; Myslivets, S. A.; Мысливец, Сергей Александрович; Shalaev, V.M.; Plasmonics: Nanoimaging, Nanofabrication, and their Applications V(5 ; 2009 ; Aug. ; 2-6 ; San Diego, CA)
}
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16.

    Polarization-sensitive resonant absorber based on splitted tamm plasmon polariton / A. Y. Avdeeva, R. G. Bikbaev, S. Y. Vetrov [et al.] // Photonics Nanostruc. Fundam. Appl. - 2023. - Vol. 53, Is. 16. - Ст. 101094, DOI 10.1016/j.photonics.2022.101094. - Cited References: 55 . - ISSN 1569-4410. - ISSN 1569-4429
   Перевод заглавия: Поляризационно-чувствительный резонансный поглотитель на основе расщепления таммовского плазмон-поляритона
Кл.слова (ненормированные):
Absorber -- Polarization -- Localization of light -- Tamm plasmon polariton -- Anisotropic nanocomposite -- Plasmonic sensor
Аннотация: The possibility of creating a polarization-sensitive absorber on the basis of the splitting of a Tamm plasmon polariton at the interface between a metallic film and an anisotropic nanocomposite layer conjugated with a photonic crystal is theoretically predicted. The effect of geometrical parameters on the optical absorption spectra under the critical coupling conditions is discussed. It is shown that, changing the polarization of the radiation falling onto the structure along its normal, one can control the absorption at the Tamm plasmon polariton wavelength.

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Держатели документа:
Kirensky Institute of Physics, Krasnoyarsk Scientific Center, Siberian Branch, Russian Academy of Sciences, Krasnoyarsk, 660036, Russian Federation
Siberian Federal University, Krasnoyarsk, 660041, Russian Federation

Доп.точки доступа:
Avdeeva, A. Yu.; Авдеева, Анастасия Юрьевна; Bikbaev, R. G.; Бикбаев, Рашид Гельмединович; Vetrov, S. Ya.; Ветров, Степан Яковлевич; Doyko, R. K.; Timofeev, I. V.; Тимофеев, Иван Владимирович
}
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17.

    Endorsing a hidden plasmonic mode for enhancement of LSPR sensing performance in evolved metal–insulator geometry using an unsupervised machine learning algorithm / N. Bhalla, A. Thakur, I. S. Edelman, R. D. Ivantsov // ACS Phys. Chem. Au. - 2022. - Vol. 2, Is. 6. - P. 459-467, DOI 10.1021/acsphyschemau.2c00033. - Cited References: 35 . - ISSN 2694-2445
   Перевод заглавия: Обнаружение скрытой плазмонной моды для усиления локального поверхностного плазмонного резонанса (ЛППР). Увеличение чувствительности усовершенствованной геометрии металл-изолятор с использованием самообучающегося машинного алгоритма
Дескрипторы: LSPR -- Plasmonics -- PCA -- Deconvolution -- Sensors
Аннотация: Large-area nanoplasmonic structures with pillared metal–insulator geometry, also called nanomushrooms (NM), consist of an active spherical-shaped plasmonic material such as gold as its cap and silicon dioxide as its stem. NM is a geometry which evolves from its precursor, nanoislands (NI) consisting of aforementioned spherical structures on flat silicon dioxide substrates, via selective physical or chemical etching of the silicon dioxide. The NM geometry is well-known to provide enhanced localized surface plasmon resonance (LSPR) sensitivity in biosensing applications as compared to NI. However, precise optical phenomenon behind this enhancement is unknown and often associated with the existence of electric fields in the large fraction of the spatial region between the pillars of NM, usually accessible by the biomolecules. Here, we uncover the association of LSPR enhancement in such geometries with a hidden plasmonic mode by conducting magneto-optics measurements and by deconvoluting the absorbance spectra obtained during the local refractive index change of the NM and NI geometries. By the virtue of principal component analysis, an unsupervised machine learning technique, we observe an explicit relationship between the deconvoluted modes of LSPR, the differential absorption of left and right circular polarized light, and the refractive index sensitivity of the LSPR sensor. Our findings may lead to the development of new approaches to extract unknown properties of plasmonic materials or establish new fundamental relationships between less understood photonic properties of nanomaterials.

https://doi.org/10.1021/acsphyschemau.2c00033
Держатели документа:
Nanotechnology and Integrated Bioengineering Centre (NIBEC), School of Engineering, Ulster University, Jordanstown, Shore Road, Newtownabbey, Northern Ireland BT37 0QB, United Kingdom
Healthcare Technology Hub, Ulster University, Jordanstown, Shore Road, Newtownabbey, Northern Ireland BT37 0QB, United Kingdom
Amity Institute of Nanotechnology, Amity University Haryana, Gurugram, Haryana 122413, India
Kirensky Institute of Physics, FRC KSC Siberian Branch of Russian Academy of Sciences, Krasnoyarsk 660036, Russia

Доп.точки доступа:
Bhalla, Nikhil; Thakur, Atul; Edelman, I. S.; Эдельман, Ирина Самсоновна; Ivantsov, R. D.; Иванцов, Руслан Дмитриевич
}
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18.

    Medium dependent optical response in ultra-fine plasmonic nanoparticles / L. K. Sorensen, D. E. Khrennikov, V. S. Gerasimov [et al.] // Phys. Chem. Chem. Phys. - 2022. - Vol. 24, Is. 39. - P. 24062-24075, DOI 10.1039/d2cp02929d. - Cited References: 52. - DEK, VSG, SVK acknowledge the support of the Russian Science Foundation (project no. 18-13-00363). L. K. S. acknowledges the support of Carl Tryggers Stiftelse, project CTS 18-441. We also acknowledge the Swedish National Infrastructure for Computing (SNIC) at the High Performance Computing Center North (HPC2N) partially funded by the Swedish Research Council through grant agreement no. 2021/3-22 . - ISSN 1463-9084
   Перевод заглавия: Зависимость оптического отклика сверхмалых плазмонных наночастиц от окружающей среды
Аннотация: We study the influence of media on the interaction of ultra-fine plasmonic nanoparticles (≤ 8 nm) with radiation. The important role of the surface layer of the nanoparticles, with properties that differ from the ones in the inner part, is established. Using an atomistic representation of the nanoparticle material and its interaction with light, we find a highly inhomogeneous distribution of the electric field inside and around the particles. It is predicted that with an increase in the refractive index of the ambient medium, the extension of the surface layer of atoms increases, something that also is accompanied by an enhanced red shift of the plasmon resonance band compared to large particles in which the influence of this layer and its relative volume is reduced. It is shown that the physical origin for the formation of a surface layer of atoms near the nanoparticle boundary is related to the anisotropy of the local environment of atoms in this layer which changes the conditions for the interaction of neighboring atoms with each other and with the incident radiation. It is shown that a growth of the refractive index of the ambient medium results in an increase in the local field in the dielectric cavity in which a plasmonic nanoparticle is embedded and which is accompanied by a growth of the amplitude of the plasmon resonance. We predict that in the ultra-fine regime the refractive index sensitivity shows a decreasing trend with respect to size which is opposite to that for larger particles. With the applied atomistic model this work demonstrates close relations between field distributions and properties of ultra-fine nanoparticles.

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Держатели документа:
Department of Physics and Astronomy, Uppsala University, Box 516, SE-751 20 Uppsala, Sweden. lasse.kragh.soerensen@gmail.com
Department of Theoretical Chemistry and Biology, School of Engineering Sciences in Chemistry, Biotechnology and Health, Royal Institute of Technology, Stockholm, SE-10691, Sweden
University Library, University of Southern Denmark, DK-5230 Odense M, Denmark
International Research Center of Spectroscopy and Quantum Chemistry, Siberian Federal University, Krasnoyarsk, 660041, Russian Federation
Institute of Computational Modelling, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation
Federal Siberian Research Clinical Centre under FMBA of Russia, 660037, Kolomenskaya, 26 Krasnoyarsk, Russia
L. V. Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, 660036, Russian Federation

Доп.точки доступа:
Sorensen, L. K.; Khrennikov, D. E.; Gerasimov, V. S.; Ershov, A. E.; Polyutov, S. P.; Karpov, S. V.; Карпов, Сергей Васильевич; Agren, H.
}
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19.

    Part II. Nanobubbles around plasmonic nanoparticles in terms of modern simulation modeling: what makes them kill the malignant cells? / A. S. Kostyukov, I. L. Isaev, A. E. Ershov [et al.] // J. Phys. D. - 2022. - Vol. 55, Is. 17. - Ст. 175402, DOI 10.1088/1361-6463/ac4c1f. - Cited References: 49. - The research was supported by the Ministry of Science and High Education of Russian Federation (Project No. FSRZ-2020-0008), and was funded by RFBR, Krasnoyarsk Territory and Krasnoyarsk Regional Fund of Science, Project No. 20-42-240003 . - ISSN 0022-3727. - ISSN 1361-6463
   Перевод заглавия: Часть II. Нанопузырьки вокруг плазмонных наночастиц с точки зрения современного имитационного моделирования: что заставляет их убивать злокачественные клетки?

РУБ Physics, Applied
Рубрики:
STRESS WAVES
   LASER
   MEMBRANE
   DAMAGE
   DEATH
   LYSIS
Кл.слова (ненормированные):
photothermal effect -- plasmonic nanoparticle -- malignant cell membrane -- pulsed laser radiation -- finite elements analysis -- anticancer therapy -- aptamer
Аннотация: We have established numerically the physical pattern and conditions for formation of nanosized bubbles in aqueous medium around biocompatible plasmonic nanoparticles (NPs) selectively bound to the membrane of the malignant cells by means of DNA-aptamers under the action of picosecond laser radiation. The results obtained are based on the finite volume method and hydrodynamic models underlying the ANSYS Fluent package with extended capabilities. We have found the main features and previously unknown dominant factors of the damage effect on the cell membrane at the moment of the bubble nucleation around the plasmonic NPs of different types taking into account the influence of the closely located membrane. Information on the kinetics of spatial distribution of pressure, temperature and the relative proportion of vapor in the 'nanoparticle-membrane-medium' system have been obtained. The attention is drawn to the advantages of using biocompatible, perfectly absorbing core–shell plasmonic NPs for anti-tumor therapy characterized by an increased mechanical effect on malignant cell membranes at lower laser radiation intensity and the spectral position of their plasmon resonance (λ = 700 nm) in the hemoglobin transparency range. This ensures penetration of laser radiation deep into tissues. The paper is provided with an extensive review of key publications and the state-of-art in this area.

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Держатели документа:
Siberian Fed Univ, Int Res Ctr Spect & Quantum Chem IRC SQC, Krasnoyarsk 660041, Russia.
Russian Acad Sci, Inst Computat Modelling, Siberian Branch, Krasnoyarsk 660036, Russia.
Fed Med Biol Agcy Russian Federat, Fed Siberian Res Clin Ctr, Krasnoyarsk 660037, Russia.
Russian Acad Sci, LV Kirensky Inst Phys, Fed Res Ctr KSC, Siberian Branch, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Kostyukov, A. S.; Isaev, I. L.; Ershov, A. E.; Gerasimov, V. S.; Polyutov, S. P.; Karpov, S. V.; Карпов, Сергей Васильевич; Ministry of Science and High Education of Russian Federation [FSRZ-2020-0008]; RFBRRussian Foundation for Basic Research (RFBR); Krasnoyarsk Territory and Krasnoyarsk Regional Fund of Science [20-42-240003]
}
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20.

    Thermal degradation of optical resonances in plasmonic nanoparticles / L. K. Sorensen, D. E. Khrennikov, V. S. Gerasimov [et al.] // Nanoscale. - 2022. - Vol. 14, Is. 2. - P. 433-447, DOI 10.1039/d1nr06444d. - Cited References: 85. - The work is supported by the Russian Science Foundation (project No. 18-13-00363). L. K. S. acknowledges the support of Carl Tryggers Stifetelse, project CTS 18-441. The authors thank the Krasnoyarsk Regional Center of Research Equipment of Federal Research Center "Krasnoyarsk Science Center SB RAS" for the use of Hitachi S-5500 high-resolution scanning electron microscope for the analysis of nanomaterials. Some of the computations were enabled by resources provided by the Swedish National Infrastructure for Computing (SNIC) at the High Performance Computing Center North (HPC2N) partially funded by the Swedish Research Council through grant agree-ment no. SNIC 2020/3-29. Authors thank Anton Utyushev for technical assistance in preparation of Fig. 3 . - ISSN 2040-3364. - ISSN 2040-3372
   Перевод заглавия: Тепловая деградация оптических резонансов в плазмонных наночастицах

РУБ Chemistry, Multidisciplinary + Nanoscience & Nanotechnology + Materials Science, Multidisciplinary + Physics, Applied
Рубрики:
STABILIZED GOLD NANOPARTICLES
DIPOLE INTERACTION-MODEL
Аннотация: The dependence of plasmon resonance excitations in ultrafine (3-7 nm) gold nanoparticles on heating and melting is investigated. An integrated approach is adopted, where molecular dynamics simulations of the spatial and temporal development of the atoms constituting the nanoparticles generate trajectories out of which system conformations are sampled and extracted for calculations of plasmonic excitation cross sections which then are averaged over the sample configurations for the final result. The calculations of the plasmonic excitations, which take into account the temperature- and size-dependent relaxation of the plasmons, are carried out with a newly developed Extended Discrete Interaction Model (Ex-DIM) and complemented by multilayered Mie theory. The integrated approach clearly demonstrates the conditions for suppression of the plasmons starting at temperatures well below the melting point. We have found a strong inhomogeneous dependence of the atom mobility in the particle crystal lattice increasing from the center to its surface upon the temperature growth. The plasmon resonance suppression is associated with an increase of the mobility and in the amplitude of phonon vibrations of the lattice atoms accompanied by electron-phonon scattering. This leads to an increase in the relaxation constant impeding the plasmon excitation as the major source of the suppression, while the direct contribution from the increase in the lattice constant and its chaotization at melting is found to be minor. Experimental verification of the suppression of surface plasmon resonance is demonstrated for gold nanoparticles on a quartz substrate heated up to the melting temperature and above.

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Держатели документа:
Siberian Fed Univ, Int Res Ctr Spect & Quantum Chem IRC SQC, Krasnoyarsk 660041, Russia.
Royal Inst Technol, Dept Theoret Chem & Biol, SE-10691 Stockholm, Sweden.
Fed Res Ctr KSC SB RAS, Inst Computat Modeling, Krasnoyarsk 660036, Russia.
Fed Res Ctr KSC SB RAS, LV Kirensky Inst Phys, Krasnoyarsk 660036, Russia.
Inst Chem Organometall Cpds, CNR ICCOM, Via G Moruzzi 1, I-56124 Pisa, Italy.
Fed Siberian Res Clin Ctr FMBA Russia, Kolomenskaya 26, Krasnoyarsk 660037, Russia.
Uppsala Univ, Dept Phys & Astron, Box 516, SE-75120 Uppsala, Sweden.

Доп.точки доступа:
Sorensen, Lasse K.; Khrennikov, Daniil E.; Gerasimov, Valeriy S.; Ershov, Alexander E.; Vysotin, M. A.; Высотин, Максим Александрович; Monti, Susanna; Zakomirnyi, Vadim, I; Polyutov, Sergey P.; Agren, Hans; Karpov, S. V.; Карпов, Сергей Васильевич; Russian Science FoundationRussian Science Foundation (RSF) [18-13-00363]; Carl Tryggers Stifetelse [CTS 18-441]; Swedish Research CouncilSwedish Research CouncilEuropean Commission [SNIC 2020/3-29]
}
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