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Effect of intramolecular interaction on Time Growth of Second Moment of Multiple-Quantum NMR in Solids [Text] / V. E. Zobov, A. A. Lundin // Int. Conf. "Resonances in Condensed Matter" : Book of abstracts. - 2011. - PTh06

Доп.точки доступа:
Zobov, V.E.; Lundin, A.A.; "Resonances in Condensed Matter", International Conference(2011 ; Jun. ; 21-25 ; Kazan, Russia)
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    Lundin, A. A.
    Asymptotic similarity of time correlation functions and shape of the 13C and 29Si NMR spectra in diamond and silicon / A. A. Lundin, V. E. Zobov // J. Exp. Theor. Phys. - 2018. - Vol. 127, Is. 2. - P. 305-315, DOI 10.1134/S1063776118080216. - Cited References: 47. - We thank V.A. Atsarkin, V.V. Demidov, F.S. Dzheparov, and E. B. Feldman for the discussion of our results. This work was supported by a subsidy allocated by the Institute of Chemical Physics of the Russian Academy of Science for the State assignment, theme 0082-2018-0005, code TSITIS AAAA-A18-118020690203. . - ISSN 1063-7761. - ISSN 1090-6509
Рубрики:
SPIN SYSTEMS
   LINE-SHAPES
   RELAXATION
   SOLIDS
   PARAMAGNETS
   RESONANCE
Аннотация: Based on the proposed theory, we have investigated the shape of the NMR absorption spectra for 13C and 29Si nuclei in diamond and silicon crystals attributable to the internuclear dipole–dipole interaction. In accordance with the available experimental data, we have considered both crystals with a 100% content of magnetoactive isotopes and crystals with a comparatively low dilution by nonmagnetic nuclei. The time correlation functions (the first of which is the Fourier transform of the NMR spectrum) arising in an infinite chain of coupled differential equations are shown to be mutually similar with a slight time delay. The proposed theory allows the spectrum to be calculated analytically. The results obtained agree satisfactorily with the experimental ones. It is noted that the mutual similarity of the time correlation functions is probably a corollary of the development of dynamical chaos in the system.

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Публикация на русском языке Лундин, Андрей Арнольдович. Асимптотическое подобие временных корреляционных функций и форма спектров ЯМР 13C и 29Si в алмазе и кремнии [Текст] / А. А. Лундин, В. Е. Зобов // Журн. эксперим. и теор. физ. - 2018. - Т. 154 Вып. 2. - С. 354–367

Держатели документа:
Russian Acad Sci, Semenov Inst Chem Phys, Vorobevskoe Sh 26, Moscow 117977, Russia.
Russian Acad Sci, Kirensky Inst Phys, Fed Res Ctr, Krasnoyarsk Sci Ctr,Siberian Branch, Akademgorodok 50, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Zobov, V. E.; Зобов, Владимир Евгеньевич; Institute of Chemical Physics of the Russian Academy of Science [0082-2018-0005, TSITIS AAAA-A18-118020690203]
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    Lundin, A. A.
    Decoherence-induced stabilization of the multiple-quantum NMR-spectrum width / A. A. Lundin, V. E. Zobov // Appl. Magn. Reson. - 2016. - Vol. 47, Is. 7. - P. 701-710, DOI 10.1007/s00723-016-0770-z. - Cited References:26 . - ISSN 0937-9347. - ISSN 1613-7507
   Перевод заглавия: Cтабилизация ширины многоквантового спектра ЯМР вследствие затухания

РУБ Physics, Atomic, Molecular & Chemical + Spectroscopy
Рубрики:
SIMULATIONS
   DYNAMICS
   SYSTEMS
   SOLIDS
Аннотация: The time dependence of an increase in the number of correlated spins in cluster was calculated for a particular variant of multiple-quantum (MQ) nuclear magnetic resonance spectroscopy using an effective two-quantum Hamiltonian that includes conventional secular nuclear dipole-dipole interaction as a weak perturbation at the stage of correlation preparation. It was shown that the cluster size grows steadily, while the width of the MQ spectrum stabilizes because the decay rates of the spectral components located at different areas of the MQ spectrum are different. The MQ bandwidth was also calculated as a function of the preparation time for various perturbation strengths. The results obtained are in excellent agreement with the experimental data reported in Alvarez and Suter (Phys Rev A 84:012320, 2011).

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Держатели документа:
Russian Acad Sci, Semenov Inst Chem Phys, Ul Kosygina 4, Moscow 117977, Russia.
Russian Acad Sci, Kirensky Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Zobov, V. E.; Зобов, Владимир Евгеньевич
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Lundin, A. A.
Multiple-quantum NMR spectroscopy and quantum information delocalization in solids in the presence of magnetic fields inhomogeneities / A. A. Lundin, V. E. Zobov // International Conference “Magnetic Resonance – Current State and Future Perspectives” (EPR-75) : book of abstracts. - Kazan, 2019. - P. 30. - Cited References: 5

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Держатели документа:
N.N. Semenov Institute of Chemical Physics, RAS
Kirensky Institute of Physics, Federal Research Center KSC SB RAS, Krasnoyarsk, Russia

Доп.точки доступа:
Zobov, V. E.; Зобов, Владимир Евгеньевич; Лундин, Андрей Арнольдович; "Magnetic Resonance - Current State and Future Perspectives", International Conference(2019 ; Sept. ; 23-27 ; Kazan, Russia); Казанский (Приволжский) федеральный университет; Казанский физико-технический институт им. Е. К. Завойского Казанского научного центра РАН
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Lundin, A. A.
Order dependence of the profile of the intensities of multiple-quantum coherences / A. A. Lundin, V. E. Zobov // J. Exp. Theor. Phys. - 2015. - Vol. 120, Is. 5. - P. 762-771, DOI 10.1134/S1063776115040093. - Cited References:62 . - ISSN 1063. - ISSN 1090-6509. -

РУБ Physics, Multidisciplinary
Рубрики:
PARAMAGNETIC SPIN SYSTEMS
   FREE-INDUCTION DECAY
   NMR-SPECTRA
   AUTOCORRELATION FUNCTIONS
   FLUCTUATION SPECTRUM
   TEMPERATURE DYNAMICS
   LINE-SHAPE
   SOLIDS
   IRREVERSIBILITY
   BEHAVIOR
Аннотация: A modification of the widespread phenomenological model theory of multiple-quantum (MQ) nuclear magnetic resonance spectra of a single cluster of correlated spins has been developed. In contrast to the mentioned theory, the size distribution of such clusters has been consistently taken into account. To obtain the distribution, solutions for the amplitudes of the expansion in the complete set of orthogonal operators are used. Expressions specifying the dependence of the profile of the intensities of MQ coherences on their number n (order) have been obtained. The total form of the dependence has been evaluated by means of the numerical implementation of the resulting expressions. The asymptotic expressions for large n values (wings of the spectrum) have been obtained analytically by the saddle-point method. It has been shown that the dependence under study has a Gaussian central part and exponential wings. The results obtained are in agreement with the previous calculations for some model systems and existing experimental data.

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Публикация на русском языке Лундин, Андрей Арнольдович. Зависимость профиля интенсивностей многоквантовых когерентностей от порядков [Текст] / А. А. Лундин, В. Е. Зобов // Журн. эксперим. и теор. физ. : Наука, 2015. - Т. 147 Вып. 5. - С. 885-895

Держатели документа:
Russian Acad Sci, Semenov Inst Chem Phys, Moscow 117977, Russia.
Russian Acad Sci, Akademgorodok, Kirensky Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia.

Доп.точки доступа:
Zobov, V. E.; Зобов, Владимир Евгеньевич
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Lundin, A. A.
Solid-state NMR free induction decay, simulated by the system of classical magnetic moments and quantum correlations / A. A. Lundin, V. E. Zobov // Russ. J. Phys. Chem. B. - 2021. - Vol. 15, Is. 5. - P. 839-847, DOI 10.1134/S1990793121050079. - Cited References: 34. - This study was carried out as part of state assignment 0082-2019-0001 (registration number AAAA-A19-119012890064-7) . - ISSN 1990-7931. - ISSN 1990-7923

РУБ Physics, Atomic, Molecular & Chemical
Рубрики:
HIGH-TEMPERATURE DYNAMICS
   HEISENBERG-MODEL
   SPIN SIMULATIONS
   SHAPE
Кл.слова (ненормированные):
spin -- paramagnetic -- quantum technology -- spin dynamics -- quantum computing
Аннотация: In the past decade, nuclear magnetic resonance (NMR) has been actively used to study the basic principles of quantum computers. It is assumed that quantum correlations play a significant role in their performance. They exist at both low and high temperatures. At the same time, the time correlation functions of nuclear spin systems of solids determine the observed signals in traditional NMR implementations. The separation of such signals into quantum and classical components has not previously been carried out and will be performed in this study for the most important of the correlational functions observed in magnetic resonance: the free induction decay (FID).

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Публикация на русском языке Лундин, Андрей Арнольдович. Сигнал свободной прецессии ЯМР твердого тела, его моделирование посредством системы классических магнитных моментов и квантовые корреляции [Текст] / А. А. Лундин, В. Е. Зобов // Химич. физика. - 2021. - Т. 40 № 9. - С. 41-49

Держатели документа:
Russian Acad Sci, Semenov Fed Res Ctr Chem Phys, Moscow, Russia.
Russian Acad Sci, Siberian Branch, Krasnoyarsk Sci Ctr, Kirensky Inst Phys,Fed Res Ctr, Krasnoyarsk, Russia.

Доп.точки доступа:
Zobov, V. E.; Зобов, Владимир Евгеньевич; [AAAA-A19-119012890064-7]
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    Lundin, A. A.
    The stabilization of width of multiple-quantum NMR spectrum induced by decoherence / A. A. Lundin, V. E. Zobov // Int. conf. "Spin physics, spin chem., and spin technol.". - 2015. - P. 112. - Библиогр.: 4 назв.
   Перевод заглавия: Стабилизация ширины многоквантового спектра ЯМР вследствие затухания

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Доп.точки доступа:
Zobov, V. E.; Зобов, Владимир Евгеньевич; Лундин, Андрей Арнольдович; "Spin physics, spin chemistry, and spin technology", Internnational conference(2015 ; Jun. ; 1-5 ; Saint Peterburg); Физико-технический институт им. А.Ф. Иоффе РАН; Казанский физико-технический институт им. Е. К. Завойского Казанского научного центра РАН"Инно-мир", центр межрегионального инновационного развития
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Zobov, V. E.
Decay of Multispin Multiple-Quantum Coherent States in the NMR of a Solid and the Stabilization of Their Intensity Profile with Time / V. E. Zobov, A. A. Lundin // J. Exp. Theor. Phys. - 2011. - Vol. 113, Is. 6. - P. 1006-1014, DOI 10.1134/S1063776111140111. - Cited References: 27 . - ISSN 1063-7761

РУБ Physics, Multidisciplinary

Кл.слова (ненормированные):
Cluster sizes -- Coherent state -- Decay rate -- Effective size -- Experimental data -- Intensity profiles -- Coherent light -- Decay (organic) -- Stabilization
Аннотация: Variations, experimentally observed in [14], in the intensity profiles of multiple-quantum (MQ) coherences in the presence of two special types of perturbations are explained on the basis of the theory, earlier developed by the authors, of the growth of the effective size of correlated clusters (the number of correlated spins) and the relaxation of MQ coherent states [23]. The intensity and the character of perturbation were controlled by the experimenters. It is shown that the observed stabilization of profiles with time is not associated with the stabilization of the cluster size. Quite the contrary, a cluster of correlated spins monotonically grows, while the observed variations in the intensity profile and its stabilization with time are attributed to the dependence of the decay rate of an MQ coherence on its order (its position in the MQ spectrum). The results of the theory are in good agreement with the experimental data.

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Держатели документа:
[Zobov, V. E.] Russian Acad Sci, LV Kirensky Phys Inst, Siberian Branch, Krasnoyarsk 660036, Russia
[Lundin, A. A.] Russian Acad Sci, NN Semenov Chem Phys Inst, Moscow 117977, Russia
ИФ СО РАН
Kirensky Institute of Physics, Russian Academy of Sciences, Siberian Branch, Krasnoyarsk, 660036, Russian Federation
Semenov Institute of Chemical Physics, Russian Academy of Sciences, Moscow, 117977, Russian Federation

Доп.точки доступа:
Lundin, A. A.; Зобов, Владимир Евгеньевич
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Zobov, V. E.
Decay of multispin multiquantum coherent states in the NMR of a solid / V. E. Zobov, A. A. Lundin // J. Exp. Theor. Phys. - 2011. - Vol. 112, Is. 3. - P. 451-459, DOI 10.1134/S1063776111020129. - Cited References: 24 . - ISSN 1063-7761

РУБ Physics, Multidisciplinary
Рубрики:
SYSTEMS
SPECTRA
Кл.слова (ненормированные):
Adiabatic approximations -- Andersons -- Coherent state -- Dynamic phenomena -- Experimental data -- Local fields -- Model-based -- Radiospectroscopy -- Relaxation functions -- Spin precession -- Theoretical result -- Two-component -- Coherent light
Аннотация: A model based on the Anderson adiabatic approximation, which is widely used for describing various aspects of dynamic phenomena in conventional radiospectroscopy, is proposed for describing the decay of multispin multiquantum coherent states in a solid. The coherent state relaxation function is represented by the product of two functions corresponding to spin precession in a two-component local field with a correlated and an uncorrelated component. Theoretical results of this study explain the experimental data reported in a number of publications and are in good agreement with these data.

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Держатели документа:
[Zobov, V. E.] Russian Acad Sci, Kirenskii Inst Phys, Siberian Branch, Krasnoyarsk 660036, Russia
[Lundin, A. A.] Russian Acad Sci, NN Semenov Chem Phys Inst, Moscow 117977, Russia
ИФ СО РАН
Kirenskii Institute of Physics, Siberian Branch, Russian Academy of Sciences, Krasnoyarsk 660036, Russian Federation
Semenov Institute of Chemical Physics, Russian Academy of Sciences, Moscow 117977, Russian Federation

Доп.точки доступа:
Lundin, A. A.; Зобов, Владимир Евгеньевич
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10.

Zobov, V. E.
Dependence of the relaxation rate of coherent states on the number of correlated spins and the order of coherence / V. E. Zobov, A. A. Lundin // JETP Lett. - 2023. - Vol. 117, Is. 12. - P. 932-937, DOI 10.1134/S0021364023601525. - Cited References: 29. - This work was supported by the Ministry of Science and Higher Education of the Russian Federation (state assignment no. 122040500060-4) . - ISSN 0021-3640. - ISSN 1090-6487
Аннотация: The relaxation of the components of the multiple-quantum NMR spectrum of a solid under the effect of the dipole–dipole interactions during the evolution period is considered. It is taken into account that clusters of dynamically correlated spins of different sizes are formed in the preparatory period, and their degradation depends on their size and coherence order. To calculate the size distribution function of clusters and their degradation function, a physical model including relaxation processes is developed. Using this model, an analytical result for a multiple-quantum spectrum is obtained. Agreement is obtained between the theoretical and experimental dependences of the coherence degradation rates in adamantane scaled by the square root of the average cluster size. The parameters of the above functions are found from the comparison of these dependences.

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Публикация на русском языке Зобов, Владимир Евгеньевич. Зависимость скорости релаксации когерентных состояний от числа коррелированных спинов и порядка когерентности [Текст] / В. Е. Зобов, А. А. Лундин // Письма в ЖЭТФ. - 2023. - Т. 117 Вып. 12. - С. 929-934

Держатели документа:
Kirensky Institute of Physics, Federal Research Center KSC, Siberian Branch, Russian Academy of Sciences, Krasnoyarsk, 660036, Russian Federation
Semenov Institute of Chemical Physics, Russian Academy of Sciences, Moscow, 117977, Russian Federation

Доп.точки доступа:
Lundin, A. A.; Зобов, Владимир Евгеньевич
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