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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : AVERYANOV E. M.
Заглавие : POLARIZED LUMINESCENCE SPECTRUM OF IMPURITY LIQUID-CRYSTAL - THE DEGENERATION LIFTED AND RENEWED BY RELAXATION
Место публикации : Zhurnal Eksperimentalnoi Teor. Fiz.: MEZHDUNARODNAYA KNIGA, 1993. - Vol. 103, Is. 6. - P2018-2038. - ISSN 0044-4510
Примечания : Cited References: 45
Предметные рубрики: RESOLVED FLUORESCENCE DEPOLARIZATION
UNIAXIAL MOLECULAR SAMPLES
NEMATIC ORDER PARAMETERS
EXCITED-STATES
SPECTROSCOPY
MEMBRANES
FLUOROPHORES
ORIENTATION
TRANSITION
DYES
Аннотация: The general molecular-statistical approach is proposed for the analysis or the polarized luminescence spectrum for impurity molecule of an arbitrary symmetry in the nematic liquid crystal matrix. On the particular example of uniaxial molecules the influence of features of the molecular electron structure, orientational statistics, molecular dynamics, and features of the anisotropic intermolecular coupling upon the positions of maxima v(if)(t) of impurity fluorescence polarized bands J(ij)(t) is studied. For the first time it is shown that all these factors significantly affect the degree of spectrum v(ij)(t) degeneration. For t not-equal 0, relaxation of excited impurity molecule subsystem toward the orientational distribution lifts a partial degeneration of spectrum v(ij), occuring at t not-equal 0, and renews partial or total degeneration of spectrum v(ij) in the limit t = infinity. In the lack of the spectrum v(ij) degeneration for t = 0 the relaxation may restore partial degeneration for t not-equal 0 as a function of the features of electron structure of molecules. The results of work explain the familiar experimental data on the number of independent component v(ij) and relation between them, on dependence of v(ij) upon the order of matrix and impurity subsystem, on the mutual relation in the positions of impurity band polarized component in the absorption and fluorescence spectra.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ovchinnikov S. G.
Заглавие : Density of hole-doped states in strongly correlated electron-systems of copper oxides
Разночтения заглавия :авие SCOPUS: Density of hole-doped states in strongly correlated electron systems of copper oxides
Место публикации : Phys. Rev. B. - 1994. - Vol. 49, Is. 14. - P.9891-9897. - ISSN 0163-1829, DOI 10.1103/PhysRevB.49.9891
Примечания : Cited References: 34
Предметные рубрики: DYNAMIC PROPERTIES
SUPERCONDUCTIVITY
GAP
LA2CUO4
BI2SR2CACU2O8
PHOTOEMISSION
SPECTROSCOPY
SPECTRA
MODEL
BAND
Аннотация: A generalized tight-binding method to calculate quasiparticle band structure and density of states in strongly correlated systems is presented. The band structures of undoped and weakly hole-doped CuO2 layer are calculated. The insulator gap has a charge transfer nature with a minor contribution from a Cu-O Coulomb interaction. Doping results in the appearance of an in-gap state with a simultaneous decrease of the density of states at the band edges in agreement with small cluster results and experimental data.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : AVERYANOV E. M.
Заглавие : STATIONARY SPECTRUM OF ADMIXED LIQUID-CRYSTAL POLARIZED FLUORESCENCE
Место публикации : Zhurnal Eksperimentalnoi Teor. Fiz.: MEZHDUNARODNAYA KNIGA, 1994. - Vol. 106, Is. 3. - P767-779. - ISSN 0044-4510
Примечания : Cited References: 29
Предметные рубрики: LOCAL FIELD
SPECTROSCOPY
PARAMETERS
DYES
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Peng J. L., Bulcock S., Belobrov P. I., Bursill L. A.
Заглавие : Surface bonding states of nano-crystalline diamond balls
Место публикации : Int. J. Mod. Phys. B: WORLD SCIENTIFIC PUBL CO PTE LTD, 2001. - Vol. 15, Is. 31. - P4071-4085. - ISSN 0217-9792, DOI 10.1142/S0217979201007865
Примечания : Cited References: 20
Предметные рубрики: PLASMON RESPONSE
POWDER
SPECTROSCOPY
MICROSCOPY
SILICON
SI(111)
Ключевые слова (''Своб.индексиров.''): diamond--article--crystal structure--electron--energy transfer--nanoparticle--particulate matter--structure analysis--surface property--transmission electron microscopy
Аннотация: The rough surface of nano-crystalline diamond spheres induces surface electronic states which appear as a broadened pre-peak over approx. 15 eV at the C K-edge energy threshold for carbon in the parallel electron energy loss spectrum (PEELS). This appears to be at least partially due to 1s-pi* transitions, although typically the latter occupy a range of only 4 eV for the sp(2) edge of highly-oriented pyrollytic graphite (HOPG). No pi* electrons appear in the conduction band inside the diamond particles, where all electrons are sp(3) hybridized. PEELS data were also obtained from a chemical vapour deposited diamond film (CVDF) and gem-quality diamond for comparison with the spectra of nano-diamonds. The density of sp(2) and sp(3) states on the surface of diamond nano-crystals is calculated for simple structural models of the diamond balls, including some conjecture about surface structures. The results are used to interpret the sp(2)/sp(3) ratios measured from the PEELS spectra recorded as scans across the particles. Surface roughness at the atomic scale was also examined using high-resolution transmission electron microscopy (HRTEM) and electron nano-diffraction patterns were used to confirm the crystal structures.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Belyaev B. A., Drokin N. A., Shabanov V. F., Shepov V. N.
Заглавие : High-frequency dielectric spectra from liquid crystals of series nCB and nOCB
Место публикации : Tech. Phys.: AMER INST PHYSICS, 2002. - Vol. 47, Is. 4. - P470-473. - ISSN 1063-7842, DOI 10.1134/1.1470597
Примечания : Cited References: 8
Предметные рубрики: DECIMETER WAVELENGTH RANGE
RELAXATION
SPECTROSCOPY
PHASES
Аннотация: The design of a resonant frequency-tunable high-sensitivity microstrip sensor is suggested. The permittivity dispersion of liquid crystals of two homologic series, alkylcyanobiphenyls (7CB and 8CB) and alkyloxycyanobiphenyls (7OCB and 8OCB), is studied at frequencies of 100-900 MHz. The dielectric spectra are shown to be the sum of the Debye relaxation and dielectric resonances observed at f approximate to 160, 280, 360, 450, 550, and 650 MHz. The dielectric resonances are present in the spectra of all the samples in both the nematic and isotropic phase. The substitution of an oxygen atom (series nOCB) for a carbon atom (series nCB) in liquid crystal molecules has a minor effect on the dielectric resonance frequencies but changes the resonance intensities and splits some of the resonance lines. (C) 2002 MAIK "Nauka / Interperiodica".
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kliava J., Edelman I. S., Potseluyko A. M., Petrakovskaja E. A., Berger R., Bruckental I., Yeshurun Y., Malakhovskii A. V., Zarubina Y. V.
Заглавие : Magnetic and optical properties and electron paramagnetic resonance of gadolinium-containing oxide glasses
Место публикации : J. Phys.: Condens. Matter: IOP PUBLISHING LTD, 2003. - Vol. 15, Is. 40. - P6671-6681. - ISSN 0953-8984, DOI 10.1088/0953-8984/15/40/005
Примечания : Cited References: 30
Предметные рубрики: ABSORPTION-SPECTRA
FARADAY-ROTATION
SPIN-RESONANCE
IONS
GD3+
SPECTROSCOPY
BEHAVIOR
GD-3
Ключевые слова (''Своб.индексиров.''): doping (additives)--electronic structure--glass--lanthanum compounds--light absorption--magnetic susceptibility--oxides--paramagnetic resonance--positive ions--rate constants--substitution reactions--absorption band--gadolinium containing oxide glasses--positive weiss constants--gadolinium compounds
Аннотация: Magnetic susceptibility, electron paramagnetic resonance (EPR) and optical absorption have been studied in a glass system 20La(2)O(3)-22Al(2)O(3)-23B(2)O(3)-35(SiO2 + GeO2) with a part of La2O3 substituted by Gd2O3 in different concentrations. Positive Weiss constants have been found in more heavily doped glasses and ascribed to clustering of Gd3+ ions. Computer simulations of the EPR spectra show that the short-range ordering in the environment of the Gd3+ ions is well preserved. The relative distribution widths of the ligand coordinates are less than 2%. In the more heavily doped glasses the EPR spectra are superpositions of signals arising from isolated ions and ferromagnetic clusters. The increase of Gd3+ concentration is shown to change substantially the strong optical absorption edge while only small changes of f-f absorption band characteristics are observed. This difference is associated with the different effect of the Gd ion clustering on the mechanisms of the strong absorption in the ultraviolet region and the f-f absorption.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Vtyurin A. N., Goryainov S. V., Zamkova N. G., Zinenko V. I., Krylov A. S., Krylova S. N., Shefer A. D.
Заглавие : Hydrostatic pressure-induced phase transitions in RbMnCl3: Raman spectra and lattice dynamics
Место публикации : Phys. Solid State: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2004. - Vol. 46, Is. 7. - P1301-1310. - ISSN 1063-7834, DOI 10.1134/1.1778456
Примечания : Cited References: 16
Предметные рубрики: CRYSTALS
SPECTROSCOPY
Аннотация: Raman scattering spectra of RbMnCl3 are measured at room temperature under high hydrostatic pressure. The results are interpreted based on first principles lattice dynamics calculations. The experimental data obtained correlate with the calculations in the low frequency domain but disagree slightly in the region of high-frequency vibrations. The transition from the hexagonal to the cubic perovskite phase observed earlier (near 0.7 GPa) was confirmed, and new transitions to lower symmetry distorted phases were discovered (at 1.1 and 5 GPa). (C) 2004 MAIK "Nauka / Interperiodica".
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Вид документа : Статья из сборника (однотомник)
Шифр издания :
Автор(ы) : Vtyurin A. N., Goryainov S. V., Krylov A. S., Krylova S. N., Shefer A. D., Zamkova N. G., Zinenko V. I.
Заглавие : Raman spectra and pressure-induced lattice instabilities in RbMnCl3 crystal
Разночтения заглавия :авие SCOPUS: Raman spectra and pressure-induced lattice instabilities in RbMnCl 3 crystal
Место публикации : 11th International Conference on Phonon Scattering in Condensed Matter (PHONONS 2004) (JUL 25-30, 2004, St Petersburg, RUSSIA): WILEY-V C H VERLAG GMBH, 2004. - 11th International Conference on Phonon Scattering in Condensed Matter (PHONONS 2004) (JUL 25-30, 2004, St Petersburg, RUSSIA). - P3097-3100. - ISBN 3-527-40588-7, DOI 10.1002/pssc.200405332
Примечания : Cited References: 14
Предметные рубрики: PHASE-TRANSITION
SPECTROSCOPY
Ключевые слова (''Своб.индексиров.''): frequencies--hydrostatic pressure--mathematical models--parameter estimation--raman scattering--spectrometers--stability--ambient conditions--anomalies--lattice instabilities--structural units--rubidium compounds
Аннотация: Raman scattering spectra of the RbMnCl3 crystal have been studied under ambient conditions and under high hydrostatic pressure. The results produced have been interpreted with the ab initio model. The experimental data agree well with the estimated values in the low frequency range and show a slightly worse agreement at higher frequencies. A phase transition from the hexagonal phase to the perovskite phase predicted earlier within the same model was observed under high pressure (above 0.7 GPa) and new transitions to lower symmetry phases were found at higher pressures (1.1 GPa and 5 GPa). (C) 2004 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kliava J., Malakhovskii A. V., Edelman I. S., Potseluyko A. M., Petrakovskaja E. A., Melnikova S.V., Zarubina T. V., Petrovskii G., Bruckental Y., Yeshurun Y.
Заглавие : Unusual magnetic transitions and nature of magnetic resonance spectra in oxide glasses containing gadolinium
Место публикации : Phys. Rev. B: AMER PHYSICAL SOC, 2005. - Vol. 71, Is. 10. - Ст.104406. - ISSN 1098-0121, DOI 10.1103/PhysRevB.71.104406
Примечания : Cited References: 40
Предметные рубрики: ELECTRON-PARAMAGNETIC-RESONANCE
BORATE GLASSES
IONS
BEHAVIOR
GD3+
SPECTROSCOPY
SYSTEMS
GD-3+
FIELD
SHAPE
Ключевые слова (''Своб.индексиров.''): gadolinium--glass--lanthanide--oxide--anisotropy--article--chemical structure--concentration response--electron spin resonance--energy--magnetism--molecular physics--nanoparticle--phase transition--refraction index--temperature sensitivity
Аннотация: Magnetic susceptibility, electron paramagnetic resonance (EPR), and optical properties have been studied in a glass system {20La(2)O(3)-22Al(2)O(3)-23B(2)O(3)-35(SiO2+GeO2)} with a part of La2O3 substituted by Gd2O3 in different concentrations. Positive Weiss constants have been found in the more heavily doped glasses and ascribed to clustering of Gd3+ ions. Two magnetic phase transitions at 55 and 12 K were detected and ascribed, respectively, to ferromagnetic and antiferromagnetic clusters containing Gd ions. The overall shape of the EPR spectra shows the presence of clustering at the higher Gd contents. At low temperatures the cluster-related resonance signal is altered in shape, indicating an onset of magnetic anisotropy field. This signal is convincingly fitted to superparamagnetic resonance arising from ferromagnetic nanoparticles. The clustering, depending on the Gd concentration, correlates with a significant shift to lower energies of the strong optical absorption band edge, ascribed to a charge transfer transition between Gd ions. A nonmonotonous change of refractive index with the increase of the Gd content indicates changes in the glass matrix and in Gd cluster structure.
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Arkhipkin V. G., Timofeev I. V.
Заглавие : Electromagnetically induced transparency and controlling the time shape of laser pulses
Место публикации : Dokl. Phys.: MAIK Nauka-Interperiodica / Springer, 2005. - Vol. 50, Is. 4. - P.165-168. - ISSN 1028-3358, DOI 10.1134/1.1922553
Примечания : Cited References: 14
Предметные рубрики: SPECTROSCOPY
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11.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Popova M. N., Chukalina E. P., Stanislavchuk T. N., Malkin B. Z., Zakirov A. R., Antic-Fidancev E., Popova E. A., Bezmaternykh L. N., Temerov V. L.
Заглавие : Optical spectra, crystal-field parameters, and magnetic susceptibility of multiferroic NdFe3(BO3)(4)
Разночтения заглавия :авие SCOPUS: Optical spectra, crystal-field parameters, and magnetic susceptibility of multiferroic Nd Fe3 (B O3) 4
Место публикации : Phys. Rev. B: AMERICAN PHYSICAL SOC, 2007. - Vol. 75, Is. 22. - Ст.224435. - ISSN 1098-0121, DOI 10.1103/PhysRevB.75.224435
Примечания : Cited References: 22
Предметные рубрики: IRON BORATE GDFE3(BO3)(4)
CRYSTALLIZATION
SPECTROSCOPY
LASER
ND3+
Аннотация: We report high-resolution optical absorption spectra for NdFe3(BO3)(4) trigonal single crystal, which is known to exhibit a giant magnetoelectric effect below the temperature of magnetic ordering T-N=33 K. The analysis of the temperature-dependent polarized spectra reveals the energies and, in some cases, symmetries and exchange splittings of Nd3+ 84 Kramers doublets. We perform crystal-field calculations starting from the exchange-charge model, obtain a set of six real crystal-field parameters, and calculate wave functions and magnetic g factors. In particular, the values g(perpendicular to)=2.385 and g(parallel to)=1.376 were found for the Nd3+ ground-state doublet. We obtain B-loc=7.88 T and parallel to J(FN)parallel to=0.48 K for the values of the local effective magnetic field at liquid-helium temperatures at the Nd3+ site and the Nd-Fe exchange integral, respectively, using the experimentally measured Nd3+ ground-state splitting of 8.8 cm(-1). To check the reliability of our set of crystal-field parameters, we model the magnetic susceptibility data from literature. A dimer containing two nearest-neighbor iron ions in the spiral chain is considered to partly account for quasi-one-dimensional properties of iron borates, and then the mean-field approximation is used. The results of calculations with the exchange parameters for Fe3+ ions J(nn)=-6.25 K (intrachain interactions) and J(nnn)=-1.92 K (interchain interactions) obtained from fitting agree well with the experimental data.
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12.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Malakhovskii A. V., Sokolov A. E., Sukhachev A. L., Temerov V. L., Stolbovaya N. A., Edelman I. S.
Заглавие : Magnetic circular dichroism and optical absorption in TmAl3(BO3)(4)
Разночтения заглавия :авие SCOPUS: Magnetic circular dichroism and optical absorption in TmAl 3(BO3)4
Место публикации : Phys. Solid State: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2007. - Vol. 49, Is. 1. - P34-38. - ISSN 1063-7834, DOI 10.1134/S1063783407010076
Примечания : Cited References: 19
Предметные рубрики: SINGLE-CRYSTALS
SPECTROSCOPY
TRANSITIONS
HUNTITE
GROWTH
Аннотация: The polarized spectra of absorption and magnetic circular dichroism in a TmAl3(BO3)(4) single crystal are studied in the re-ion of H-3(6) - F-3(4), H-3(6) - F-3(3),and H-3(3) - F-3(2) electronic transitions in e Tm3+ ion. The structure of the spectra is interpreted qualitatively. It is shown that the magnetic circular dichroism of the H-3(6) - F-3(4) transition is determined by the contribution from the splitting of the ground state, whereas the magnetic circular dichroism of the H-3(6) - F-3(3) transition is governed by the contribution from the splitting of an excited state in a trigonal crystal field.
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13.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kuz'menko A. M., Mukhin A. A., Ivanov V. Y., Kadomtseva A. M., Lebedev S. P., Bezmaternykh L. N.
Заглавие : Antiferromagnetic Resonance and Dielectric Properties of Rare-earth Ferroborates in the Submillimeter Frequency Range
Место публикации : J. Exp. Theor. Phys.: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2011. - Vol. 113, Is. 1. - P113-120. - ISSN 1063-7761, DOI 10.1134/S106377611105013X
Примечания : Cited References: 27. - This work was supported by the Russian Foundation for Basic Research, project no. 10-02-00846.
Предметные рубрики: GDFE3(BO3)(4)
SPECTROSCOPY
CRYSTAL
Ключевые слова (''Своб.индексиров.''): antiferromagnetic resonance--basic parameters--effective anisotropy constant--ferroborates--ferroics--ferromagnetic orderings--frequency ranges--magnetic interactions--magnetoresonance--millimeter frequency range--rare earth ions--submillimeters--antiferromagnetic materials--crystallography--erbium--europium--ferromagnetic resonance--ion exchange--magnetic anisotropy--magnetic devices--magnetic structure--permittivity--resonance--antiferromagnetism
Аннотация: The magnetoresonance and dielectric properties of a number of crystals of a new family of multiferroics, namely, rare-earth ferroborates RFe(3)(BO(3))(4) (R = Y, Eu, Pr, Tb, Tb(0.25)Er(0.75)), are studied in the submillimeter frequency range (nu = 3-20 cm(-1)). Ferroborates with R = Y, Tb, and Eu exhibit permittivity jumps at temperatures of 375, 198, and 58 K, respectively, which are caused by the R32 - P3(1)2(1) phase transition. Antiferromagnetic resonance (AFMR) modes in the subsystem of Fe(3+) ions are detected in the range of antiferromagnetic ordering (T T(N)
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14.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Aver'yanov E. M.
Заглавие : Local field anisotropy in Langmuir-Blodgett films of cadmium arachidate
Место публикации : Phys. Solid State: MAIK NAUKA/INTERPERIODICA/SPRINGER, 2011. - Vol. 53, Is. 12. - P2492-2494. - ISSN 1063-7834, DOI 10.1134/S1063783411120031
Примечания : Cited References: 9
Предметные рубрики: SPECTROSCOPY
Аннотация: Lorentz tensor and local field tensor components for uniaxial Langmuir-Blodgett films of cadmium arachidate from 3 to 100 nm thick on silver, polymethyl methacrylate, and glass substrates have been experimentally determined using the data on the film refractive index dispersion in the visible range. The constraints from below on the mean value and anisotropy of the molecular polarizability caused by the intermolecular interactions in the film have been established.
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15.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Chzhan A. V., Patrin G. S., Kiparisov S. Y., Seredkin V. A., Burkova L. V., Velikanov D. A.
Заглавие : Magnetic and magneto-optical properties of Co-P films prepared by chemical deposition
Место публикации : J. Magn. Magn. Mater. - 2011. - Vol. 323, Is. 20. - P.2493-2496. - OCT. - ISSN 0304-8853, DOI 10.1016/j.jmmm.2011.05.024
Примечания : Cited Reference Count: 22. - Гранты: This study was supported by the Russian Foundation for Basic Research, Project no. 08-02-00397a and the departmental target program Development of Scientific Potential of Higher Education, 2009-2010, Project no. 2.1.1./4399.Финансирующая организация: Russian Foundation for Basic Research [08-02-00397a]; departmental target program Development of Scientific Potential of Higher Education [2.1.1./4399]
Предметные рубрики: SPECTROSCOPY
THICKNESS
COBALT
Ключевые слова (''Своб.индексиров.''): co-p films--chemically deposition--the polar kerr and faraday effects--hysteresis loops--chemically deposition--cop films--hysteresis loops--the polar kerr and faraday effects--chemical deposition--chemically deposition--co films--cop films--film magnetization--film surface morphology--incident light--magnetic and magneto-optical properties--magnetic layers--polar kerr effect--polar-kerr--polycrystalline--underlayers--chemical analysis--faraday effect--hysteresis loops--kerr magnetooptical effect--light reflection--magnetic materials--optical kerr effect--palladium--cobalt
Аннотация: Features in the formation of chemically deposited polycrystalline Co-P films with thicknesses of a few nanometers are established by analyzing film surface morphology and variation in the film magnetization. It is shown that in the thickness range below 30 nm the polar Kerr effect value OK changes nonmonotonically and depends on a wavelength of the incident light. For the films thicker than 30 nm, this value depends weakly on both the thickness and the wavelength. These features in the OK behavior are attributed to the Faraday effect, which is revealed at small thicknesses upon light reflection from the lower surface of a magnetic layer. It is found that the Faraday effect in the Co-P films exceeds that in the Co films by a factor of more than two. This effect is assumed to be caused by the presence of a Pd underlayer in the samples under study. (C) 2011 Elsevier BY. All rights reserved.
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16.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Drokin N. A., Kokourov G. A., Glushchenko G. A., Osipova I. V., Maslennikov A. N., Churilov G. N.
Заглавие : Effect of electrode material on impedance spectra of metal-polyethylene structures with carbon nanotubes
Место публикации : Phys. Solid State: MAIK Nauka-Interperiodica / Springer, 2012. - Vol. 54, Is. 4. - P.844-848. - ISSN 1063-7834, DOI 10.1134/S1063783412040063
Примечания : Cited References: 15. - This study was supported by the Ministry of Education and Science of the Russian Federation within the framework of the Russian Federal Targeted Program "Scientific and Scientific-Pedagogical Human Resources for the Innovative Russia in 2009-2011" and the Presidium of the Russian Academy of Sciences (integration project no. 27.1).
Предметные рубрики: SPECTROSCOPY
Аннотация: The effect of an electrode material on electrical properties of a composite material based on super-high-molecular polyethylene (SHMPE) filled with carbon nanotubes has been studied using impedance spectroscopy. Using the method of replacing the sample by an equivalent electric circuit, it has been found that, depending on the electrode material, a blocking barrier with high active resistance and a space charge region adjacent to it arise in the interface region. It has been shown that the barrier height is controlled by surface electronic states of SHMPE and weakly depends on the electron work function of metal electrodes (Bardeen barrier). The characteristic times of electrical relaxation characterizing bulk and interface regions of the composite under study have been determined.
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17.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Sokolov A. E., Edelman I. S., Zabluda V. N., Petrakovskaya E. A., Aleksandrovsky A. S., Shubin A. A., Trukhan S. N., Mart'yanov O. N.
Заглавие : Magneto-optical activity of crude oil and its heavy fractions
Место публикации : Opt. Spectrosc.: MAIK Nauka-Interperiodica / Springer, 2012. - Vol. 112, Is. 5. - P.755-762. - ISSN 0030-400X, DOI 10.1134/S0030400X12050165
Примечания : Cited References: 18. - This work was performed under Interdisciplinary Integration Project no. 118 of the Siberian Branch of the Russian Academy of Sciences (2009-2011).
Предметные рубрики: MAGNETIC CIRCULAR-DICHROISM
SINGLE-CRYSTALS
SPECTROSCOPY
EPR
ABSORBENCY
PORPHYRIN
SYSTEMS
Аннотация: We have experimentally studied optical and magneto-optical spectra of solutions of crude oils of different origin and their heavy fractions in the visible spectral range. Magnetic circular dichroism of oil in the wavelength range similar to 550 nm has been revealed. We show that the shape of the spectra of this dichroism depends on the origin of crude oil, with the magnetic dichroism magnitude being proportional to the concentration of the oil in the solution. A comparison of the data of magneto-optical spectroscopy with electron paramagnetic resonance spectra and chemical composition of samples has allowed us to conclude that the observed magneto-optical activity is determined by the occurrence of VO2+ complexes in the oil samples. The revealed magneto-optical activity of crude oil can form the basis of a unique method of analysis of the composition and properties of oils of different origin and heavy fractions thereof.
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18.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Val'kov V. V., Aksenov S. V., Ulanov E. A.
Заглавие : Effects of multiple reflection in the process of inelastic electron transport through an anisotropic magnetic atom
Коллективы : Presidium of the Russian Academy of Sciences; Ministry of Education and Science of Russian Federation [16.740.11.0644]; Russian Foundation for Basic Research [12-02-31130, 13-02-00523, 13-02-98013]; Council of the President of the Russian Federation for Support of Young Scientists and Leading Scientific Schools [MK-526.2013.2, SP-6361.2013.5]
Место публикации : JETP Letters. - 2013. - Vol. 98, Is. 7. - P.403-409. - ISSN 0021-3640, DOI 10.1134/S0021364013200162
Примечания : Cited References: 27. - This work was supported by the Presidium of the Russian Academy of Sciences (program "Quantum Mesoscopic and Disordered Systems"), the Ministry of Education and Science of Russian Federation (state contract no. 16.740.11.0644, federal program "Human Capital for Science and Education in Innovative Russia" for 2009-2013), and the Russian Foundation for Basic Research (project nos. 12-02-31130, 13-02-00523, and 13-02-98013). S. V. A. is grateful to the Council of the President of the Russian Federation for Support of Young Scientists and Leading Scientific Schools, project nos. MK-526.2013.2 and SP-6361.2013.5.
Предметные рубрики: QUANTUM
SPECTROSCOPY
STATE
Аннотация: The effect of multiple reflection in the process of electron transport on the current-voltage characteristics of an adsorbed magnetic atom with single-ion anisotropy has been investigated. All orders of the perturbation theory with respect to the parameter of coupling between the contacts and the multilevel impurity have been taken into account by the Keldysh diagram technique with the use of Hubbard operators. It has been shown that the current-voltage characteristics of the system in a strongly nonequilibrium regime contains regions of negative differential conductance. The ways of enhancing this effect are discussed.
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19.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Val'kov V. V., Aksenov S. V., Ulanov E. A.
Заглавие : Inelastic tunnel transport of electrons through an anisotropic magnetic structure in an external magnetic field
Коллективы : Russian Foundation for Basic Research [13-02-00523, 13-02-98013, 14-02-31280]; Russian Federation [MK-526-526.2013.2, SP-6361.2013.5]
Место публикации : J. Exp. Theor. Phys.: MAIK Nauka-Interperiodica / Springer, 2014. - Vol. 119, Is. 1. - P.124-137. - ISSN 1063-7761, DOI 10.1134/S1063776114060065. - ISSN 1090-6509
Примечания : Cited References: 35. - This work was performed under the Program "Quantum Mesoscopic and Disordered Systems" of the Presidium of the Russian Academy of Sciences and supported financially by the Russian Foundation for Basic Research (project nos. 13-02-00523, 13-02-98013, and 14-02-31280). The work of one of coauthors (S. V. A.) was supported by grant no. MK-526-526.2013.2 of the President of the Russian Federation and scholarship SP-6361.2013.5 of the President of the Russian Federation.
Предметные рубрики: SINGLE-MOLECULE
SPECTROSCOPY
ATOM
STATE
Аннотация: Quantum transport of electrons through a magnetic impurity located in an external magnetic field and affected by a substrate is considered using the Keldysh diagram technique for the Fermi and Hubbard operators. It is shown that in a strongly nonequilibrium state induced by multiple reflections of electrons from the impurity, the current-voltage (I-V) characteristic of the system contains segments with a negative conductivity. This effect can be controlled by varying the anisotropy parameter of the impurity center as well as the parameters of coupling between the magnetic impurity and metal contacts. The application of the magnetic field is accompanied by an increase in the number of Coulomb steps in the I-V curve of the impurity. The effect of appreciable magnetoresistance appears in this case. We demonstrate the possibility of switching between magnetic impurity states with different total spin projection values in the regime of asymmetric coupling of this impurity with the contacts.
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20.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Krylov A. S., Sofronova S. N., Kolesnikova E. M., Ivanov Y. N., Sukhovsky A. A., Goryainov S. V., Ivanenko A. A., Shestakov N. P., Kocharova A. G., Vtyurin A. N.
Заглавие : Experimental and theoretical methods to study structural phase transition mechanisms in K3WO3F3 oxyfluoride
Коллективы : Russian Foundation for Basic Research [4828.2012.2, 12-02-31205]; Federal Special Program "Scientific and scientific-pedagogical staff of innovative Russia" [8379]
Место публикации : J. Solid State Chem. - 2014. - Vol. 218. - P.32-37. - ISSN 0022-4596, DOI 10.1016/j.jssc.2014.05.028. - ISSN 1095-726X
Примечания : Cited References: 21. - The Authors are grateful to Prof. Zinenko V.I. for constructive discussion of the results. The work has been done with financial support of the Russian Foundation for Basic Research projects nos. 4828.2012.2, 12-02-31205; Federal Special Program "Scientific and scientific-pedagogical staff of innovative Russia" project no. 8379.
Предметные рубрики: LATTICE-DYNAMICS
RAMAN-SCATTERING
ELPASOLITE
(NH4)3WO3F3
SPECTROSCOPY
CRYSTALS
Ключевые слова (''Своб.индексиров.''): raman spectroscopy--ir spectroscopy--nmr spectroscopy--high hydrostatic pressure--oxyfluorides--lattice dynamics calculations
Аннотация: The results of structural phase transitions mechanisms study in K3WO3F3oxyfluoride are represented by different experimental and theoretical methods. The structural phase transition anomalies at T1=452 K and T2=414 K of Raman and IR spectra have been analyzed. Using vibrational spectroscopy methods, the NMR-experiment has been done to clarify the nature of found phase transitions: displacive types or order-disorder types. The model of “disordered” crystal was proposed, and the results of lattice dynamics calculation in frameworks of the generalized Gordon–Kim method of ordered (R3) and “disordered” crystals were compared. The high pressure phases were studied by the Raman technique too.
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