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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Паршин, Александр Михайлович
Заглавие : Отклик гибридно-упорядоченного нематика с поверхностной линией дисклинации на импульс магнитного поля
Место публикации : Жидк. кристаллы и их практич. использ. - 2021. - Т. 21, № 3. - С. 60-67. - ISSN 1991-3966 (ISSN), DOI 10.18083/LCAppl.2021.3.60; Liq. Cryst. Appl. - ISSN 2499-9644 (eISSN)
Примечания : Библиогр.: 23
Предметные рубрики: LIQUID-CRYSTAL
DOMAIN-STRUCTURE
INTERFERENCE
DYNAMICS
BEHAVIOR
FILM
Аннотация: Исследовано оптическое пропускание гибридно-упорядоченного нематического слоя с поверхностной линией дисклинации, деформированного импульсным магнитным полем. Получены выражения для времен реакции на полевое воздействие и релаксации жидкого кристалла к недеформированному состоянию. Время реакции оказалось существенно больше расчетного значения и сопоставимым с длительностью импульса магнитного поля. Выведены зависимости интенсивности света от разности фаз между обыкновенным и необыкновенным лучами с учетом рассеяния. Для процесса релаксации получено хорошее совпадение экспериментальной и расчетной временных зависимостей интенсивности лазерного излучения, прошедшего через весь слой жидкого кристалла, за исключением тонкого переходного приповерхностного слоя. Аномалия хода кривой релаксации в переходном слое рассмотрена в рамках известных модельных представлений.The optical transmission of a hybrid-ordered nematic layer with a surface disclination line, strained by a pulsed magnetic field, is studied. The expressions for the reaction times to the field action and relaxation of a liquid crystal to an untrained state are obtained. The experimental reaction time turned out to be significantly longer than its calculated value and comparable to the magnetic field pulse duration. The light intensity dependences on the phase difference between the ordinary and extraordinary rays, taking into account scattering are derived. For the relaxation process, good agreement is obtained between the experimental and calculated time dependences of the laser radiation intensity transmitted through the entire liquid crystal layer, with the exception of a thin transitional near-surface layer. The anomaly in the course of the relaxation curve run in the transition layer is considered within the framework of the known model concepts.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Orlov V. A., Rudenko, Roman Yu, Prokopenko, Vladimir S., Orlova, Irina N.
Заглавие : Features in the resonance behavior of magnetization in arrays of triangular and square nanodots
Коллективы : Russian Foundation for Basic ResearchRussian Foundation for Basic Research (RFBR) [20-02-00696]
Место публикации : J. Sib. Fed. Univ. Math. Phys. - 2021. - Vol. 14, Is. 5. - P.611-623. - ISSN 1997-1397, DOI 10.17516/1997-1397-2021-14-5-611-623; Журн. СФУ. Матем. и физика. - ISSN 2313-6022(eISSN)
Примечания : Cited References: 23. - This study was supported by the Russian Foundation for Basic Research, project no. 20-02-00696
Предметные рубрики: VORTEX STATE
DYNAMICS
MOTION
EXCITATIONS
Аннотация: Collective modes of the gyrotropic motion of a magnetic vortex core in ordered arrays of triangular and square ferromagnetic film nanodots have been theoretically investigated. The dispersion relations have been derived. The dipole-dipole interaction of the magnetic moments of the magnetic vortex cores of elements has been taken into account in the approximation of a small shift from the equilibrium position. It is shown that the effective rigidity of the magnetic subsystem of triangular elements is noticeably higher than that of the subsystem of square elements of the same linear sizes. The potential application of the polygonal film nanodisks as nanoscalpels for noninvasive tumor cell surgery is discussed.Теоретически исследуются коллективные моды гиротропного движения ядра магнитного вихря в упорядоченных массивах ферромагнитных пленочных наноточек треугольной и квадратной форм. Получены дисперсионные соотношения. Учитывается диполь-дипольное взаимодействие магнитных моментов ядер магнитных вихрей элементов в приближении малого смещения от положения равновесия. Показано, что эффективная жесткость магнитной подсистемы в треугольных элементах заметно больше, чем в квадратных при одинаковых линейных размерах. Обсуждается перспектива использования пленочных нанодисков-многоугольников в качестве "наноскальпелей" для неинвазивной клеточной хирургии опухолей.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zobov V. E., Lundin A. A.
Заглавие : Reversible and Irreversible propagation of quantum information and its manifestation in multiple-quantum NMR spectra in solids
Коллективы : Ministry of Science and Higher Education of the Russian Federation [0082-2019-0001, AAAA-A19-119012890064-7]
Место публикации : J. Exp. Theor. Phys. - 2020. - Vol. 131, Is. 2. - P.273-279. - ISSN 1063-7761, DOI 10.1134/S1063776120060096. - ISSN 1090-6509(eISSN)
Примечания : Cited References: 33. - This work was supported by the Ministry of Science and Higher Education of the Russian Federation within the State Task 0082-2019-0001 (State Registration Number AAAA-A19-119012890064-7)
Предметные рубрики: DYNAMICS
LOCALIZATION
SIMULATIONS
COHERENCES
Аннотация: On the basis of the earlier developed statistical theory of the growth of the effective size of correlated clusters (the number of correlated spins), an expression for the shape of the multiple-quantum (MQ) NMR spectrum is obtained that takes into account the loss of coherence in a spin system due, for example, to the controlled intervention of the experimenter. It is shown that the scrambling and decoherence processes in the MQ spectrum of the multiparticle system of a solid are not separated, unlike the corresponding spectra of some large isolated molecules [27] in a solution. The relations obtained allow one to extract the necessary information about the above processes (scrambling and decoherence) from the dependence of the MQ spectra on experimental parameters.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Liu, Yan Rong, Wu, Yong, Wang, Jian Guo, Vendrell, Oriol, Kimberg V., Zhang, Song Bin
Заглавие : Electron-rotation coupling in diatomics under strong-field excitation
Место публикации : Phys. Rev. A. - 2020. - Vol. 102, Is. 3. - Ст.033114. - ISSN 2469-9926, DOI 10.1103/PhysRevA.102.033114. - ISSN 2469-9934(eISSN)
Примечания : Cited References: 78. - S.B.Z. thanks H. D. Meyer for his helpful instructions of Wigner-DVR in MCTDH. Grants from the National Basic Research Program of China (2017YFA0403200), NSFC (No. 11604197, No. 11974230, and No. 11934004), the Science Challenge Program of China (TZ2018005 and TZ2016005) are acknowledged. V.K. acknowledges financial support from Swedish Research Council (VR) and the Ministry of Science and High Education of Russian Federation, Project No. FSRZ2020-0008.
Предметные рубрики: REAL-TIME OBSERVATION
DYNAMICS
LASER
ULTRAFAST
MOLECULES
Аннотация: he photoexcitation and photodissociation of diatomic molecules by intense pulse lasers has been the subject of extensive investigations over the past decades. However, the usually employed theoretical framework neglects the coupling between the molecular rotational angular momentum (R) and the angular momentum of the electrons projected onto the molecular axis Ω=Λ+Σ, which results in the known Λ-doubling phenomenon in high-resolution electronic spectra of diatomic molecules. While neglecting this coupling is an excellent approximation in the weak-field or perturbative regime owing to the large mass difference between the rotating atoms and the electrons, the approximation breaks down for intense laser pulses because of the repeated Rabi cycling of the electronic transitions, which can have a significant effect on the rotational degrees of freedom of the molecule. By correcting the transition dipole matrix elements and introducing angular basis sets based on Wigner D functions, the conventional theoretical treatment is generalized to a universal description valid for both the weak- and strong-field regimes. The theoretical treatment developed here is applied to the ∣1Σ› to ∣1Π› transitions in diatomic systems. Our results reveal that, for field intensities resulting in about one Rabi cycling for extreme ultraviolet or x-ray transitions, the theoretical predictions by the conventional theoretical frame need to be corrected when considering observables such as the molecular alignment and the angular distribution of the photofragments.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Shi, Xin, Wu, Yong, Wang, Jian Guo, Kimberg V., Zhang, Song Bin
Заглавие : X-ray transient absorption spectroscopy by an ultrashort x-ray-laser pulse in a continuous-wave IR field
Место публикации : Phys. Rev. A. - 2020. - Vol. 101, Is. 2. - Ст.023401. - ISSN 2469-9926, DOI 10.1103/PhysRevA.101.023401. - ISSN 2469-9934(eISSN)
Примечания : Cited References: 56. - Grants from the National Basic Research Program of China (Grant No. 2017YFA0403200), National Natural Science Foundation of China (Grants No. 11604197, No. 11934004, and No. 11974230), the Science Challenge Program of China (Grants No. TZ2018005 and No. TZ2016005), and the Organization Department of CCCPC are acknowledged. V.K. acknowledges financial support from Swedish Research Council within the State Contract of the Ministry of Education and Science of the Russian Federation for Siberian Federal University for Scientific Research in 2017-2019 (Project No. 3.2662.2017)
Предметные рубрики: MOLECULAR NITROGEN
TIME
DYNAMICS
PHASE
SPECTRA
DECAY
Аннотация: X-ray transient absorption spectra (XTAS) of molecules are theoretically investigated in a femtosecond x-ray pump and continuous-wave (cw) infrared (IR)-control scenario. The scheme is exemplified by a CO molecule resonantly pumped into carbon and oxygen core-excited 1s→π∗ states by a weak femtosecond x-ray pulse, while dynamic Stark shifts are induced by the cw IR-control radiation. As a result, significant shoulder structures appear in XTAS showing strong dependence on the phase of IR radiation relative to the envelope of the x-ray pulse. Due to a significant difference in the frequencies of the two pulses, the present XTAS scheme provides much clear interpretation of the dynamic Stark effects as compared to the attosecond UV transient absorption scenario. Within the suggested two-level model, where the total spectrum is decomposed as incoherent superposition of contributions from different vibrational excitations weighted by the Franck-Condon Factors, all spectral structures can be well identified and interpreted in a good agreement with the full-scale molecular simulations. Well-characterized XTAS in the proposed IR-control scheme can be applied for fine phase synchronization between IR and x-ray pulses, highly demanded in modern experiments on x-ray free-electron lasers.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Zobov V. E., Kucherov M. M.
Заглавие : On the effect of an inhomogeneous magnetic field on high-frequency asymptotic behaviors of correlation functions of spin lattices
Место публикации : JETP Letters. - 2018. - Vol. 107, Is. 9. - P.553-557. - ISSN 0021-3640, DOI 10.1134/S002136401809014X. - ISSN 1090-6487(eISSN)
Примечания : Cited References: 39
Предметные рубрики: HEISENBERG PARAMAGNET
SYSTEMS
TIME
RELAXATION
DYNAMICS
SPECTRA
Аннотация: Singular points of spin autocorrelation functions on the imaginary time axis, which determine the arguments of exponential high-frequency asymptotic behaviors, have been analyzed. It has been shown that randomly distributed inhomogeneous magnetic fields expand the wings of spectra of autocorrelation functions and, thereby, intensify the heating of a system subjected to variable magnetic fields, which are used to create effective Hamiltonians or at the saturation of inhomogeneously broadened EPR lines.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Larionov K. V., Popov Z. I., Vysotin M. A., Kvashnin D. G., Sorokin P. B.
Заглавие : Study of the new two-dimensional compound CoC
Коллективы : Russian Science Foundation [17-72-20223]; Ministry of Education and Science of the Russian Federation [14.Y26.31.0005]; Joint Supercomputer Center, Russian Academy of Sciences
Место публикации : JETP Letters. - 2018. - Vol. 108, Is. 1. - P.13-17. - ISSN 0021-3640, DOI 10.1134/S0021364018130106. - ISSN 1090-6487(eISSN)
Примечания : Cited References: 24. - We are grateful to Prof. Gotthard Seifert, Prof. B.P. Sorokin, and Prof. L.A. Chernozatonskii for the discussion of the results. This work was supported by the Russian Science Foundation (project no. 17-72-20223). The calculations were performed with the use of resources of the Computer Cluster, Materials Modeling and Development Laboratory, National University of Science and Technology MISiS (supported by the Ministry of Education and Science of the Russian Federation, project no. 14.Y26.31.0005), and the Joint Supercomputer Center, Russian Academy of Sciences.
Предметные рубрики: TOTAL-ENERGY CALCULATIONS
WAVE BASIS-SET
AB-INITIO
DYNAMICS
Аннотация: A novel quasi-two-dimensional monolayer structure with orthorhombic symmetry based on cobalt carbide, o-CoC, has been considered. This structure supplements a recently discovered family of quasi-two-dimensional compounds based on transition metals. The dynamic stability of a monolayer has been demonstrated. Its mechanical and electronic characteristics have been studied.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kim P. D., Orlov V. A., Rudenko R. Y., Prokopenko V. S., Orlova I. N., Kobyakov A. V.
Заглавие : On the resonant state of magnetization in array of interacting nanodots
Коллективы : Euro-Asian Symposium "Trends in MAGnetism", "Trends in MAGnetism", Euro-Asian Symposium, Институт физики им. Л.В. Киренского Сибирского отделения РАН , Russian Science Foundation [14-15-00805]; Russian Foundation for Basic Research (RFBR) [16-32-00103]
Место публикации : J. Magn. Magn. Mater.: Elsevier Science, 2017. - Vol. 440. - P.171-174. - ISSN 0304-8853, DOI 10.1016/j.jmmm.2016.12.125. - ISSN 1873-4766(eISSN)
Примечания : Cited References:35. - Authors are grateful to V. Ya. Prints for help in preparing dot arrays. Sections 3 and 4 of the work was supported by the Russian Science Foundation, project no. 14-15-00805. Section 2 of the work was supported by Russian Foundation for Basic Research (RFBR) project no. 16-32-00103.
Предметные рубрики: VORTEX
DYNAMICS
VORTICES
Ключевые слова (''Своб.индексиров.''): nanodots--magnetization--dispersion law--tiel's equation
Аннотация: Development of the interpretation of the phenomenon of the lift of the magnetic resonance frequencies degeneracy caused by the magnetostatic interaction in assemblies of nanodisks has been done. The difference of the resonance behavior of magnetic vortexes in a round and rectangular nanodots has been studied experimentally and explained.
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Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Fedorov A. S., Kuzubov A. A., Kholtobina A. S., Kovaleva E. A., Knaup J., Irle S.
Заглавие : Theoretical investigation of molecular and electronic structures of buckminsterfullerene-silicon quantum dot systems
Место публикации : J. Phys. Chem. A: American Chemical Society, 2016. - Vol. 120, Is. 49. - P.9767-9775. - ISSN 1089-5639, DOI 10.1021/acs.jpca.6b06959
Примечания : Cited References:20. - The work was supported by Ministry of Education and Science of Russia (Russian-Japanese joined project, Agreement 14.613.21.0010, ID RFMEFI61314X0010). We are grateful to the Joint Supercomputer Center of Russian Academy of Sciences, Moscow and Siberian Supercomputer Center of SB RAS, Novosibirsk for the opportunity to use their computer clusters to perform the calculations. S.I. acknowledges partial support from a JST CREST grant.
Предметные рубрики: Si
NANOPARTICLES
DYNAMICS
Аннотация: Density functional theory (DFT) and density functional tight binding (DFTB) molecular dynamics Density functional theory (DFT) and density functional tight binding (DFTB) molecular dynamics (DFTB/MD) simulations of embedding and relaxation of buckminsterfullerene C60 molecules chemisorbed on (001) and (111) surfaces and inside bulk silicon lattice were performed. DFT calculations of chemisorbed fullerenes on both surfaces show that the C60 molecule deformation was very small and the C60 binding energies were roughly ∼4 eV. The charge analysis shows that the C60 molecule charges on (001) and (111) surfaces were between −2 and −3.5 electrons, respectively, that correlates well with the number of C–Si bonds linking the fullerene molecule and the silicon surface. DFT calculations of the C60 molecule inside bulk silicon confirm that the C60 molecule remains stable with the deformation energy values of between 11 and 15 eV for geometries with different C60 configurations. The formation of some C–Si bonds causes local silicon amorphization and corresponding electronic charge uptake on the embedded fullerene cages. Charge analysis confirms that a single C60 molecule can accept up to 20 excessive electrons that can be used in practice, wherein the main charge contribution is located on the fullerene’s carbon atoms bonded to silicon atoms. These DFT calculations correlate well with DFTB/MD simulations of the embedding process. In this process, the C60 molecule was placed on the top of the Si(111) surface, and it was further exposed by a stream of silicon dimers, resulting in subsequent overgrowth by silicon.
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10.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Bulgakov E. N., Sadreev A. F.
Заглавие : Spin polarized bound states in the continuum in open Aharonov-Bohm rings with the Rashba spin-orbit interaction
Коллективы : Russian Science Foundation [14-12-00266]
Место публикации : J. Phys.: Condens. Matter: IOP Publishing, 2016. - Vol. 28, Is. 26. - Ст.265301. - ISSN 0953-8984, DOI 10.1088/0953-8984/28/26/265301. - ISSN 1361-648X(eISSN)
Примечания : Cited References:59. - This work has been supported by Russian Science Foundation through grant 14-12-00266. We acknowledge discussions with D N Maksimov and K N Pichugin.
Предметные рубрики: Degenerate states
Nuclear reactions
Unified theory
Quantum
Transport
Dynamics
Decay
Ключевые слова (''Своб.индексиров.''): aharonov-bohm ring--rashba spin-orbit interaction--bound states in the continuum
Аннотация: We consider the trapping of electrons with a definite spin polarization by bound states in the continuum (BSC) in the open Aharonov-Bohm rings in the presence of the Rashba spin-orbit interaction (RSOI). Neglecting the Zeeman term we show the existence of BSCs in the one-dimensional ring when the eigenstates of the closed ring are doubly degenerate. With account of the Zeeman term BSCs occur only at the points of threefold degeneracy. The BSCs are found in the parametric space of flux and RSOI strength in close pairs with opposite spin polarization. Thereby the spin polarization of electrons transmitted through the ring can be altered by minor variation of magnetic or electric field at the vicinity of these pairs. Numerical simulations of the two-dimensional open ring show similar results for the BSCs. Encircling the BSC points in the parametric space of the flux and the RSOI constant gives rise to a geometric phase.
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11.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Lundin A. A., Zobov V. E.
Заглавие : Decoherence-induced stabilization of the multiple-quantum NMR-spectrum width
Место публикации : Appl. Magn. Reson.: Springer, 2016. - Vol. 47, Is. 7. - P.701-710. - ISSN 0937-9347, DOI 10.1007/s00723-016-0770-z. - ISSN 1613-7507(eISSN)
Примечания : Cited References:26
Предметные рубрики: SIMULATIONS
DYNAMICS
SYSTEMS
SOLIDS
Аннотация: The time dependence of an increase in the number of correlated spins in cluster was calculated for a particular variant of multiple-quantum (MQ) nuclear magnetic resonance spectroscopy using an effective two-quantum Hamiltonian that includes conventional secular nuclear dipole-dipole interaction as a weak perturbation at the stage of correlation preparation. It was shown that the cluster size grows steadily, while the width of the MQ spectrum stabilizes because the decay rates of the spectral components located at different areas of the MQ spectrum are different. The MQ bandwidth was also calculated as a function of the preparation time for various perturbation strengths. The results obtained are in excellent agreement with the experimental data reported in Alvarez and Suter (Phys Rev A 84:012320, 2011).
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12.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kolovsky A. R.
Заглавие : Bose-Hubbard Hamiltonian: Quantum chaos approach
Место публикации : Int. J. Mod. Phys. B: World Scientific Publishing, 2016. - Vol. 30, Is. 10. - Ст.1630009. - ISSN 0217-9792, DOI 10.1142/S0217979216300097. - ISSN 1793-6578(eISSN)
Примечания : Cited References:42
Предметные рубрики: Optical lattice
Dynamics
Atoms
States
Model
Ключевые слова (''Своб.индексиров.''): cold atoms in optical lattices--quantum transport--nonlinear dynamics and chaos
Аннотация: We discuss applications of the theory of quantum chaos to one of the paradigm models of many-body quantum physics - the Bose-Hubbard (BH) model, which describes, in particular, interacting ultracold Bose atoms in an optical lattice. After preliminary, pure quantum analysis of the system we introduce the classical counterpart of the BH model and the governing semiclassical equations of motion. We analyze these equations for the problem of Bloch oscillations (BOs) of cold atoms where a number of experimental results are available. The paper is written for nonexperts and can be viewed as an introduction to the field.
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13.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Tsipotan A. S., Gerasimova M. A., Slabko V. V., Aleksandrovsky A. S.
Заглавие : Laser-induced wavelength-controlled self-assembly of colloidal quasi-resonant quantum dots
Коллективы : Grant of Ministry of Education and Science of the Russian Federation [3.1749.2014/K, 214/71]; RFBR [14-02-00219 A]
Место публикации : Opt. Express: Optical Society of America, 2016. - Vol. 24, Is. 10. - P.11145-11150. - ISSN 1094-4087, DOI 10.1364/OE.24.011145
Примечания : Cited References:18. - This research is partially supported by Grant of the Ministry of Education and Science of the Russian Federation for Siberian Federal University (projects No 3.1749.2014/K, 214/71) and RFBR, research project No. 14-02-00219 A.
Предметные рубрики: Organized aggregation
Metal nanoparticles
Optical binding
Dynamics
Field
Аннотация: Self-assembly of colloidal semiconductor quantum dots controlled solely by laser-induced interaction is demonstrated for the first time. Pairs of CdTe nanoparticles are formed under irradiation with nanosecond pulses at wavelengths 555 or 560 nm. Formation of pairs is justified by corresponding changes of absorption spectra. Conditions of the experiment are in excellent agreement with those predicted by the theory of laser-induced dipole-dipole interaction of QDs. The fraction of QDs assembled into pairs is up to 47%. (C) 2016 Optical Society of America
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14.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kim P. D., Orlov V. A., Prokopenko V. S., Zamai S. S., Prints, V. Ya, Rudenko R. Y., Rudenko T. V.
Заглавие : On the low-frequency resonance of magnetic vortices in micro- and nanodots
Коллективы : Siberian Branch of the Russian Academy of Sciences [26]
Место публикации : Phys. Solid State: MAIK Nauka-Interperiodica / Springer, 2015. - Vol. 57, Is. 1. - P.30-37. - ISSN 1063, DOI 10.1134/S1063783415010151. - ISSN 10906460(eISSN)
Примечания : Cited References:57. - This study was supported by the Siberian Branch of the Russian Academyof Sciences within the framework of the Interdisciplinary IntegrationProject No. 26 "Ferromagnetic Film Nanodots: Physics of Phenomena andApplications" (2012-2014).
Предметные рубрики: EASY-PLANE FERROMAGNETS
VORTEX CORE
MAGNON MODES
DYNAMICS
FIELD
Аннотация: The resonance motion of the magnetization of thin cylindrical and parallelepiped micro- and nanodots has been studied theoretically and experimentally. Analytical expressions for the external-field dependence of the resonance frequency of the vortex-structure oscillations have been derived taking into account the inertial and damping coefficients. The external-field dependence of the damping parameter has been found theoretically. The influence of the effective mass of a magnetic vortex on its low-frequency dynamics has been discussed.
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15.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Handunkanda S. U., Curry E. B., Voronov V. N., Said, Ayman H., Guzman-Verri G. G., Brierley R. T., Littlewood P. B., Hancock J. N.
Заглавие : Large isotropic negative thermal expansion above a structural quantum phase transition
Место публикации : Phys. Rev. B: American Physical Society, 2015. - Vol. 92, Is. 13. - Ст.134101. - ISSN 1098, DOI 10.1103/PhysRevB.92.134101. - ISSN 1550235X(eISSN)
Примечания : Cited References:35. - The authors also acknowledge the valuable conversations with Joe Budnick and Gabe Aeppli. Work at the University of Connecticut is supported by National Science Foundation Award No. DMR-1506825. Work at the University of Costa Rica is supported by Vicerrectoria de Investigacion under Project No. 816-B5-220, and work at Argonne National Laboratory is supported by the US Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. R.T.B. acknowledges support from the Yale Prize Postdoctoral Fellowship. The construction of HERIX was partially supported by the NSF under Grant No. DMR-0115852.
Предметные рубрики: SCF3 CRYSTAL
CUBIC SCF3
DYNAMICS
SCATTERING
SRTIO3
Аннотация: Perovskite structured materials contain myriad tunable ordered phases of electronic and magnetic origin with proven technological importance and strong promise for a variety of energy solutions. An always-contributing influence beneath these cooperative and competing interactions is the lattice, whose physics may be obscured in complex perovskites by the many coupled degrees of freedom, which makes these systems interesting. Here, we report signatures of an approach to a quantum phase transition very near the ground state of the nonmagnetic, ionic insulating, simple cubic perovskite material ScF3, and show that its physical properties are strongly effected as much as 100 K above the putative transition. Spatial and temporal correlations in the high-symmetry cubic phase determined using energy- and momentum-resolved inelastic x-ray scattering as well as x-ray diffraction reveal that soft mode, central peak, and thermal expansion phenomena are all strongly influenced by the transition.
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16.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Ershov A. E., Gavrilyuk A. P., Karpov S. V., Semina P. N.
Заглавие : Optodynamic phenomena in aggregates of polydisperse plasmonic nanoparticles
Коллективы : Russian Academy of Sciences [24.29, 24.31, III.9.5, 43, SB RAS-SFU (101)]; Ministry of Education and Science of Russian Federation [14.B37.21.0457]
Место публикации : Appl. Phys. B: Springer, 2014. - Vol. 115, Is. 4. - P.547-560. - ISSN 0946-2171, DOI 10.1007/s00340-013-5636-6. - ISSN 1432-0649
Примечания : Cited References: 48. - Authors are thankful to Prof. V. A. Markel (University of Pennsylvania) for supplying program codes for realization of the coupled dipole method for polydisperse metal nanoparticle aggregates. This research was supported by the Russian Academy of Sciences under the Grants 24.29, 24.31, III.9.5, 43, SB RAS-SFU (101); Ministry of Education and Science of Russian Federation under Contract 14.B37.21.0457.
Предметные рубрики: SMALL-PARTICLE COMPOSITES
OPTICAL-PROPERTIES
NOBLE-METALS
SILVER
ELECTRON
LIQUID
GENERATION
DYNAMICS
FORCES
GOLD
Аннотация: We propose an optodynamical model of interaction of pulsed laser radiation with aggregates of spherical metallic nanoparticles embedded into host media. The model takes into account polydispersity of particles, pair interactions between the particles, dissipation of absorbed energy, heating and melting of the metallic core of particles and of their polymer adsorption layers, and heat exchange between electron and ion components of the particle material as well as heat exchange with the interparticle medium. Temperature dependence of the electron relaxation constant of the particle material and the effect of this dependence on interaction of nanoparticles with laser radiation are first taken into consideration. We study in detail light-induced processes in the simplest resonant domains of multiparticle aggregates consisting of two particles of an arbitrary size in aqueous medium. Optical interparticle forces are realized due to the light-induced dipole interaction. The dipole moment of each particle is calculated by the coupled dipole method (with correction for the effect of higher multipoles). We determined the role of various interrelated factors leading to photomodification of resonant domains and found an essential difference in the photomodification mechanisms between polydisperse and monodisperse nanostructures.
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17.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Krylov A. S., Kolesnikova E. M., Isaenko L. I., Krylova S. N., Vtyurin A. N.
Заглавие : Measurement of Raman-scattering spectra of Rb2KMoO3F3 crystal: Evidence for controllable disorder in the lattice structure
Коллективы : Russian Foundation for Basic Research [11-02-98002-r, 12-02-00056]; integration project SB RAS [28, SS-4828.2012.2]; Federal Special Program "Scientific and scientific-pedagogical staff of innovative Russia" [8379]
Место публикации : Cryst. Growth Des.: American Chemical Society, 2014. - Vol. 14, Is. 3. - P.923-927. - ISSN 1528-7483, DOI 10.1021/cg4008894. - ISSN 1528-7505
Примечания : Cited References: 31. - The authors are grateful to Prof. I. N. Flerov for valuable support and useful discussions. The authors acknowledge stimulating discussions with Dr. S. N. Sofronova and Dr. A. S. Aleksandrovsky. The assistance of Dr. S. Skokov is sincerely appreciated. This work was partly supported by Russian Foundation for Basic Research project nos. 11-02-98002-r and 12-02-00056 and integration project SB RAS no. 28, SS-4828.2012.2 grant, and Federal Special Program "Scientific and scientific-pedagogical staff of innovative Russia" (no. 8379).
Предметные рубрики: PHASE-TRANSITIONS
OXYFLUORIDE
ELPASOLITE
(NH4)3MOO3F3
(NH4)3WO3F3
TEMPERATURE
DYNAMICS
N-2
Cs
Аннотация: The λ-shaped line width broadening anomalies of octahedron group vibrations in Rb2KMoO3F3 disordered crystal have been revealed in the wide temperature range by Raman technique. The line width of Mo-O and Mo-F vibrations in this crystal is connected with the lattice disorder. The dependence of ordering degree passing the phase transition point history has been discovered. Wide temperature-line width area is found below structural phase transition where different lattice disorder can be obtained at a given temperature by varying the rate of sample cooling. The current study demonstrates the ability of a dynamic temperature regime to control ordering processes in crystals. © 2014 American Chemical Society.
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18.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Fialko O., Delattre M.C., Brand J., Kolovsky A. R.
Заглавие : Nucleation in finite topological systems during continuous metastable quantum phase transitions
Место публикации : Phys. Rev. Lett.: American Physical Society, 2012. - Vol. 108, Is. 25. - Ст.250402. - ISSN 0031-9007, DOI 10.1103/PhysRevLett.108.250402
Примечания : Cited References: 31. - We acknowledge stimulating discussions with Jean-Sebastien Caux and Lincoln Carr. A. K. thanks Massey University for hospitality. O. F., M. C. D., and J. B. were supported by the Marsden Fund (Contract No. MAU0910) administrated by the Royal Society of New Zealand.
Предметные рубрики: SYMMETRY-BREAKING
VORTEX NUCLEATION
BROKEN SYMMETRY
THERMALIZATION
SUPERFLUID
DYNAMICS
STATE
Аннотация: Finite topological quantum systems can undergo continuous metastable quantum phase transitions to change their topological nature. Here we show how to nucleate the transition between ring currents and dark soliton states in a toroidally trapped Bose-Einstein condensate. An adiabatic passage to wind and unwind its phase is achieved by explicit global breaking of the rotational symmetry. This could be realized with current experimental technology.
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19.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Krasnov P. O., Eliseeva N. S., Kuzubov A. A.
Заглавие : Interaction of Scandium and Titanium Atoms with a Carbon Surface Containing Five- and Seven-Membered Rings
Коллективы : Ministry of Education and Science of the Russian Federation
Место публикации : J. Exp. Theor. Phys.: MAIK Nauka-Interperiodica / Springer, 2012. - Vol. 114, Is. 1. - P.80-84. - ISSN 1063-7761, DOI 10.1134/S1063776111160059. - ISSN 1090-6509
Примечания : Cited References: 25. - We are grateful to the Joint Supercomputer Center, Russian Academy of Sciences, for the possibility of using the computer cluster for our quantum-chemical calculations. This work was supported by the Ministry of Education and Science of the Russian Federation (federal program "Human Capital for Science and Education in Innovative Russia" for 2009-2013).
Предметные рубрики: MOLECULAR-HYDROGEN COMPLEXES
STORAGE
NANOTUBES
TRANSITION
ENERGY
TEMPERATURE
EXCHANGE
DYNAMICS
METALS
C60
Аннотация: The use of carbon nanotubes coated by atoms of transition metals to store molecular hydrogen is associated with the problem of the aggregation of these atoms, which leads to the formation of metal clusters. The quantum-chemical simulation of cluster models of the carbon surface of a graphene type with scandium and titanium atoms has been performed. It has been shown that the presence of five- and seven-membered rings, in addition to six-membered rings, in these structures makes it possible to strongly suppress the processes of the migration of metal atoms over the surface, preventing their clustering.
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20.

Вид документа : Статья из журнала
Шифр издания :
Автор(ы) : Kolovsky A. R., Mantica G.
Заглавие : Driven Harper model
Место публикации : Phys. Rev. B: American Physical Society, 2012. - Vol. 86, Is. 5. - Ст.54306. - ISSN 1098-0121, DOI 10.1103/PhysRevB.86.054306
Примечания : Cited References: 14. - Computations for this work have been performed on the CSN4 cluster of INFN in Pisa. G. M. acknowledges the support of MIUR-PRIN project "Nonlinearity and disorder in classical and quantum transport processes" and A. K. acknowledges the support of SB RAS project "Dynamics of atomic Bose-Einstein condensates in optical lattices" and RFBR project "Tunneling of the macroscopic quantum states."
Предметные рубрики: MAGNETIC-FIELDS
ELECTRONS
DYNAMICS
Аннотация: We analyze the driven Harper model, which appears in the problem of tight-binding electrons in the Hall configuration (normal to the lattice plane magnetic field plus in-plane electric field). The presence of an electric field extends the celebrated Harper model, which is parametrized by the Peierls phase, into the driven Harper model, which is additionally parametrized by two Bloch frequencies, associated with the two components of the electric field. We show that the eigenstates of the driven Harper model are either extended or localized, depending on the commensurability of the Bloch frequencies. This results holds for both rational and irrational values of the Peierls phase. In the case of incommensurate Bloch frequencies we provide an estimate for the wave-function localization length.
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